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Dicke Superradiance in Solids

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 Added by Junichiro Kono
 Publication date 2016
  fields Physics
and research's language is English




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Recent advances in optical studies of condensed matter have led to the emergence of phenomena that have conventionally been studied in the realm of quantum optics. These studies have not only deepened our understanding of light-matter interactions but also introduced aspects of many-body correlations inherent in optical processes in condensed matter systems. This article is concerned with superradiance (SR), a profound quantum optical process predicted by Dicke in 1954. The basic concept of SR applies to a general $N$-body system where constituent oscillating dipoles couple together through interaction with a common light field and accelerate the radiative decay of the system. In the most fascinating manifestation of SR, known as superfluorescence (SF), an incoherently prepared system of $N$ inverted atoms spontaneously develops macroscopic coherence from vacuum fluctuations and produces a delayed pulse of coherent light whose peak intensity $propto N^2$. Such SF pulses have been observed in atomic and molecular gases, and their intriguing quantum nature has been unambiguously demonstrated. Here, we focus on the rapidly developing field of research on SR in solids, where not only photon-mediated coupling but also strong Coulomb interactions and ultrafast scattering exist. We describe SR and SF in molecular centers in solids, molecular aggregates and crystals, quantum dots, and quantum wells. In particular, we will summarize a series of studies we have recently performed on quantum wells in strong magnetic fields. These studies show that cooperative effects in solid-state systems are not merely small corrections that require exotic conditions to be observed; rather, they can dominate the nonequilibrium dynamics and light emission processes of the entire system of interacting electrons.



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In 1954, Dicke predicted that a system of quantum emitters confined to a subwavelength volume would produce a superradiant burst. For such a burst to occur, the emitters must be in the special Dicke state with zero dipole moment. We show that a superradiant burst may also arise for non-Dicke initial states with nonzero dipole moment. Both for Dicke and non-Dicke initial states, superradiance arises due to a decrease in the dispersion of the quantum phase of the emitter state. For non-Dicke states, the quantum phase is related to the phase of long-period envelopes which modulate the oscillations of the dipole moments. A decrease in dispersion of the quantum phase causes a decrease in the dispersion of envelope phases that results in constructive interference of the envelopes and the superradiant burst.
Following the experimental realization of Dicke superradiance in Bose gases coupled to cavity light fields, we investigate the behavior of ultra cold fermions in a transversely pumped cavity. We focus on the equilibrium phase diagram of spinless fermions coupled to a single cavity mode and establish a zero temperature transition to a superradiant state. In contrast to the bosonic case, Pauli blocking leads to lattice commensuration effects that influence self-organization in the cavity light field. This includes a sequence of discontinuous transitions with increasing atomic density and tricritical superradiance. We discuss the implications for experiment.
Motivated by experiments observing self-organization of cold atoms in optical cavities we investigate the collective dynamics of the associated nonequilibrium Dicke model. The model displays a rich semiclassical phase diagram of long time attractors including distinct superradiant fixed points, bistable and multistable coexistence phases and regimes of persistent oscillations. We explore the intrinsic timescales for reaching these asymptotic states and discuss the implications for finite duration experiments. On the basis of a semiclassical analysis of the effective Dicke model we find that sweep measurements over 200ms may be required in order to access the asymptotic regime. We briefly comment on the corrections that may arise due to quantum fluctuations and states outside of the effective two-level Dicke model description.
200 - L. Deng , E.W. Hagley 2010
We study a highly efficient, matter-wave amplification mechanism in a longitudinally-excited, Bose-Einstein condensate and reveal a very large enhancement due to nonlinear gain from a sixmatter- optical, wave-mixing process involving four photons. Under suitable conditions this opticallydegenerate, four-photon process can be stronger than the usual two-photon inelastic light scattering mechanism, leading to nonlinear growth of the observed matter-wave scattering independent of any enhancement from bosonic stimulation. Our theoretical framework can be extended to encompass even higher-order, nonlinear superradiant processes that result in higher-order momentum transfer.
The Dicke model with a weak dissipation channel is realized by coupling a Bose-Einstein condensate to an optical cavity with ultra-narrow bandwidth. We explore the dynamical critical properties of the Hepp-Lieb-Dicke phase transition by performing quenches across the phase boundary. We observe hysteresis in the transition between a homogeneous phase and a self-organized collective phase with an enclosed loop area showing power law scaling with respect to the quench time, which suggests an interpretation within a general framework introduced by Kibble and Zurek. The observed hysteretic dynamics is well reproduced by numerically solving the mean field equation derived from a generalized Dicke Hamiltonian. Our work promotes the understanding of nonequilibrium physics in open many-body systems with infinite range interactions.
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