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Register a new userObservation of resonance fluorescence and the Mollow-triplet from a coherently driven site-controlled quantum dot
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Resonant excitation of solid state quantum emitters has the potential to deterministically excite a localized exciton while ensuring a maximally coherent emission. In this work, we demonstrate the coherent coupling of an exciton localized in a lithographically positioned, site-controlled semiconductor quantum dot to an external resonant laser field. For strong continuous-wave driving we observe the characteristic Mollow triplet and analyze the Rabi splitting and sideband widths as a function of driving strength and temperature. The sideband widths increase linearly with temperature and the square of the driving strength, which we explain via coupling of the exciton to longitudinal acoustic phonons. We also find an increase of the Rabi splitting with temperature, which indicates a temperature induced delocalization of the excitonic wave function resulting in an increase of the oscillator strength. Finally, we demonstrate coherent control of the exciton excited state population via pulsed resonant excitation and observe a damping of the Rabi oscillations with increasing pulse area, which is consistent with our exciton-photon coupling model. We believe that our work outlines the possibility to implement fully scalable platforms of solid state quantum emitters. The latter is one of the key prerequisites for more advanced, integrated nanophotonic quantum circuits.
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We show that resonance fluorescence, i.e. the resonant emission of a coherently driven two-level system, can be realized with a semiconductor quantum dot. The dot is embedded in a planar optical micro-cavity and excited in a wave-guide mode so as to discriminate its emission from residual laser scattering. The transition from the weak to the strong excitation regime is characterized by the emergence of oscillations in the first-order correlation function of the fluorescence, g(t), as measured by interferometry. The measurements correspond to a Mollow triplet with a Rabi splitting of up to 13.3 micro eV. Second-order-correlation measurements further confirm non-classical light emission.
We experimentally demonstrate that the Mollow triplet sidebands of a quantum dot strongly coupled to a cavity exhibit anomalous power induced broadening and enhanced emission when one sideband is tuned over the cavity frequency. We observe a nonlinear increase of the sideband linewidth with excitation power when the Rabi frequency exceeds the detuning between the quantum dot and the cavity, consistent with a recent theoretical model that accounts for acoustic phonon-induced processes between the exciton and the cavity. In addition, the sideband tuned to the cavity shows strong resonant emission enhancement.
We report on the observation of bright emission of single photons under pulsed resonance fluorescence conditions from a single quantum dot (QD) in a micropillar cavity. The brightness of the QD fluorescence is greatly enhanced via the coupling to the fundamental mode of a micropillar, allowing us to determine a single photon extraction efficiency of $(20.7pm0.8)~%$ per linear polarization basis. This yields an overall extraction efficiency of $(41.4pm1.5)~%$ in our device. We observe the first Rabi-oscillation in a weakly coupled quantum dot-micropillar system under coherent pulsed optical excitation, which enables us to deterministically populate the excited QD state. In this configuration, we probe the single photon statistics of the device yielding $g^{(2)}(0)=0.072pm0.011$ at a QD-cavity detuning of $75~mu$eV.
We report the first experimental demonstration of interference-induced spectral line elimination predicted by Zhu and Scully [Phys. Rev. Lett. 76, 388 (1996)] and Ficek and Rudolph [Phys. Rev. A 60, 4245 (1999)]. We drive an exciton transition of a self-assembled quantum dot in order to realize a two-level system exposed to bichromatic laser field and observe nearly complete elimination of the resonance fluorescence spectral line at the driving laser frequency. This is caused by quantum interference between coupled transitions among the doubly dressed excitonic states, without population trapping. We also demonstrate multiphoton ac Stark effect with shifted subharmonic resonances and dynamical modifications of resonance fluorescence spectra by using double dressing.
Intensity squeezing, i.e., photon number fluctuations below the shot noise limit, is a fundamental aspect of quantum optics and has wide applications in quantum metrology. It was predicted in 1979 that the intensity squeezing could be observed in resonance fluorescence from a two-level quantum system. Yet, its experimental observation in solid states was hindered by inefficiencies in generating, collecting and detecting resonance fluorescence. Here, we report the intensity squeezing in a single-mode fibre-coupled resonance fluorescence single-photon source based on a quantum dot-micropillar system. We detect pulsed single-photon streams with 22.6% system efficiency, which show subshot-noise intensity fluctuation with an intensity squeezing of 0.59 dB. We estimate a corrected squeezing of 3.29 dB at the first lens. The observed intensity squeezing provides the last piece of the fundamental picture of resonance fluorescence; which can be used as a new standard for optical radiation and in scalable quantum metrology with indistinguishable single photons.
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