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Register a new userInterplay of fission modes in mass distribution of light actinide nuclei 225,227Pa
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Fission-fragment mass distributions were measured for 225,227Pa nuclei formed in fusion reactions of 19F + 206, 208Pb around fusion barrier energies. Mass-angle correlations do not indicate any quasi-fission like events in this bombarding energy range. Mass distributions were fitted by Gaussian distribution and mass variance extracted. At below-barrier energies, the mass variance was found to increase with decrease in energy for both nuclei. Results from present work were compared with existing data for induced fission of 224, 226Th and 228U around barrier energies. Enhancement in mass variance of 225, 227Pa nuclei at below-barrier energies shows evidence for presence of asymmetric fission events mixed with symmetric fission events. This is in agreement with the results of mass distributions of nearby nuclei 224, 226Th and 228U where two-mode fission process was observed. Two-mode feature of fission arises due to the shell effects changing the landscape of the potential energy surfaces at low excitation energies. The excitation-energy dependence of the mass variance gives strong evidence for survival of microscopic shell effects in fission of light actinide nuclei 225, 227Pa with initial excitation energy ~30 - 50 MeV.
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A study of photofission on 181Ta nucleus induced by bremsstrahlung photons with endpoint energies of 50 and 3500 MeV has been performed. The fission yields have been measured by using the induced-activity method in an off-line analysis. The absolute photofission cross sections for the tantalum target at 50 and 3500 MeV are found to be 5.4 pm 1.1 microb and 0.77pm0.11 mb, respectively, and the corresponding deduced fissilities are (0.23pm0.05) x 10^{-3} and (2.9 pm 0.9) x 10^{-3}. Mass- and charge-yield distributions were derived from the data. The results were compared with the simulated results from CRISP code for multi-modal fission by assuming symmetrical fission mode.
An analysis of the $^{231}$Pa$(d,3n)$$^{230}$U reaction excitation function at energies around the Coulomb barrier has taken into account the pre-equilibrium and compound-nucleus cross sections corrected for the deuteron-breakup decrease of the total reaction cross section, as well as the inelastic breakup enhancement. The analysis reveals the dominance of the deuteron breakup mechanism unlike a former assessment in this respect of the deuteron-induced fission process.
In this work, we present new experimental data on mass distribution of fission fragments from $^{241}$Am proton-induced fission at $660$ MeV measured at the LNR Phasotron (JINR). The systematic analysis of several measured fragment mass distributions from different fission reactions available in the literature is also presented. The proton-induced fission of $^{241}$Am, $^{237}$Np and $^{238}$U at 26.5, 62.9 and 660 MeV was studied. The proton-induced fission of $^{232}$Th was studied at 26.5, 62.9 and 190 MeV. The fission of $^{208}$Pb also by a proton was investigated at 190, 500 and 1000 MeV. The fission of $^{197}$Au was studied for 190 and 800 MeV protons. Bremsstrahlung reactions with maximum photon energies of 50 and 3500 MeV were studied for $^{232}$Th and $^{238}$U. The framework of the Random Neck Rupture Model was applied in the analysis. The roles of the neutron excess and of the so called fissility parameter were also investigated.
Fission barriers heights and excitation energies of superdeformed isomeric minima are calculated within the microscopic - macroscopic Woods - Saxon model for 75 actinide nuclei for which the experimental data are known. State - of - the - art methods were used: minimization over many deformation parameters for minima and the imaginary water flow on many - deformation energy grid for saddles, including nonaxial and reflection-asymmetric shapes. We obtain 0.82 - 0.94 MeV rms deviation between the calculated and experimental barriers and 0.53 MeV rms error in the excitation of superdeformed minima (SD). Experimental vs theory discrepancies seem to be of various nature and not easy to eliminate, especially if one cares for more than one or two observables. As an example, we show that by strengthening pairing in odd systems one can partially improve agreement in barriers, while spoiling it for masses. We also discuss the thorium anomaly and suggest its possible relation to a different way in which the Ac and Th barriers are derived from experimental data.
The nucleus is one of the most multi-faceted many-body systems in the universe. It exhibits a multitude of responses depending on the way one probes it. With increasing technical advancements of beams at the various accelerators and of detection systems the nucleus has, over and over again, surprised us by expressing always new ways of organized structures and layers of complexity. Nuclear magnetism is one of those fascinating faces of the atomic nucleus we discuss in the present review. We shall not just limit ourselves to presenting the by now very large data set that has been obtained in the last two decades using various probes, electromagnetic and hadronic alike and that presents ample evidence for a low-lying orbital scissors mode around 3 MeV, albeit fragmented over an energy interval of the order of 1.5 MeV, and higher-lying spin-flip strength in the energy region 5 - 9 MeV in deformed nuclei, nor to the presently discovered evidence for low-lying proton-neutron isovector quadrupole excitations in spherical nuclei. To the contrary, we put the experimental evidence in the perspectives of understanding the atomic nucleus and its various structures of well-organized modes of motion and thus enlarge our discussion to more general fermion and bosonic many-body systems.
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