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Register a new userSpatiotemporal complexity of electroconvection patterns in nematic liquid crystals
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We investigate a number of complex patterns driven by the electro-convection instability in a planarly aligned layer of a nematic liquid crystal. They are traced back to various secondary instabilities of the ideal roll patterns bifurcating at onset of convection, whereby the basic nemato-hydrodynamic equations are solved by common Galerkin expansion methods. Alternatively these equations are systematically approximated by a set of coupled amplitude equations. They describe slow modulations of the convection roll amplitudes, which are coupled to a flow field component with finite vorticity perpendicular to the layer and to a quasi-homogeneous in-plane rotation of the director. It is demonstrated that the Galerkin stability diagram of the convection rolls is well reproduced by the corresponding one based on the amplitude equations. The main purpose of the paper is, however, to demonstrate that their direct numerical simulations match surprisingly well new experiments, which serves as a convincing test of our theoretical approach.
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Optical methods are most convenient to analyze spatially periodic patterns with wavevector $bm q$ in a thin layer of a nematic liquid crystal. In the standard experimental setup a beam of parallel light with a short wavelength $lambda ll 2 pi/q$ passes the nematic layer. Recording the transmitted light the patterns are either directly visualized by shadowgraphy or characterized more indirectly by the diffraction fringes due to the optical grating effects of the pattern. In this work we present a systematic short-wavelength analysis of these methods for the commonly used planar orientation of the optical axis of liquid crystal at the confining surfaces. Our approach covers general 3D experimental geometries with respect to the relative orientation of $bm q$ and of the wavevector $bm k$ of the incident light. In particular the importance of phase grating effects is emphasized, which are not accessible in a pure geometric optics approach. Finally, as a byproduct we present also an optical analysis of convection rolls in Rayleigh-Benard convection, where the refraction index of the fluid is isotropic in contrast to its uniaxial symmetry in nematic liquid crystals. Our analysis is in excellent agreement with an earlier physical optics approach by Trainoff and Cannell [Physics of Fluids {bf 14}, 1340 (2002)], which is restricted to a 2D geometry and technically much more demanding.
The effect of superimposed ac and dc electric fields on the formation of electroconvection and flexoelectric patterns in nematic liquid crystals was studied. For selected ac frequencies an extended standard model of the electro-hydrodynamic instabilities was used to characterize the onset of pattern formation in the two-dimensional parameter space of the magnitudes of the ac and dc electric field components. Numerical as well as approximate analytical calculations demonstrate that depending on the type of patterns and on the ac frequency, the combined action of ac and dc fields may either enhance or suppress the formation of patterns. The theoretical predictions are qualitatively confirmed by experiments in most cases. Some discrepancies, however, seem to indicate the need to extend the theoretical description.
We present in this paper a detailed analysis of the flexoelectric instability of a planar nematic layer in the presence of an alternating electric field (frequency $omega$), which leads to stripe patterns (flexodomains) in the plane of the layer. This equilibrium transition is governed by the free energy of the nematic which describes the elasticity with respects to the orientational degrees of freedom supplemented by an electric part. Surprisingly the limit $omega to 0$ is highly singular. In distinct contrast to the dc-case, where the patterns are stationary and time-independent, they appear at finite, small $omega$ periodically in time as sudden bursts. Flexodomains are in competition with the intensively studied electro-hydrodynamic instability in nematics, which presents a non-equilibrium dissipative transition. It will be demonstrated that $omega$ is a very convenient control parameter to tune between flexodomains and convection patterns, which are clearly distinguished by the orientation of their stripes.
Motivated by experiments in electroconvection in nematic liquid crystals with homeotropic alignment we study the coupled amplitude equations describing the formation of a stationary roll pattern in the presence of a weakly-damped mode that breaks isotropy. The equations can be generalized to describe the planarly aligned case if the orienting effect of the boundaries is small, which can be achieved by a destabilizing magnetic field. The slow mode represents the in-plane director at the center of the cell. The simplest uniform states are normal rolls which may undergo a pitchfork bifurcation to abnormal rolls with a misaligned in-plane director.We present a new class of defect-free solutions with spatial modulations perpendicular to the rolls. In a parameter range where the zig-zag instability is not relevant these solutions are stable attractors, as observed in experiments. We also present two-dimensionally modulated states with and without defects which result from the destabilization of the one-dimensionally modulated structures. Finally, for no (or very small) damping, and away from the rotationally symmetric case, we find static chevrons made up of a periodic arrangement of defect chains (or bands of defects) separating homogeneous regions of oblique rolls with very small amplitude. These states may provide a model for a class of poorly understood stationary structures observed in various highly-conducting materials (prechevrons or broad domains).
We analyze the existence and stability of two-component vector solitons in nematic liquid crystals for which one of the components carries angular momentum and describes a vortex beam. We demonstrate that the nonlocal, nonlinear response can dramatically enhance the field coupling leading to the stabilization of the vortex beam when the amplitude of the second beam exceeds some threshold value. We develop a variational approach to describe this effect analytically.
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