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Register a new userRapid Doubling of the Critical Current of YBa$_2$Cu$_3$O$_{7-delta}$ Coated Conductors for Viable High-Speed Industrial Processing
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We demonstrate that 3.5-MeV oxygen irradiation can markedly enhance the in-field critical current of commercial 2nd generation superconducting tapes with an exposure time of just one second per 0.8 cm2. The speed demonstrated here is now at the level required for an industrial reel-to-reel post-processing. The irradiation is made on production line samples through the protective silver coating and does not require any modification of the growth process. From TEM imaging, we identify small clusters as the main source of increased vortex pinning.
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Combined action of weak and strong pinning centers on the vortex lattice complicates magnetic behavior of a superconductor since temperature and magnetic field differently affect weak and strong pinning. In this paper we show that contributions of weak and strong pinning into magnetization of the layered superconductor YBa$_2$Cu$_3$O$_{7-delta}$ can be separated and analyzed individually. We performed a careful analysis of temperature behavior of the relaxed superconducting current $J$ in YBa$_2$Cu$_3$O$_{7-delta}$ films which revealed two components of the current $J = J_1 +J_2$. A simple method of separation of the components and their temperature dependence in low magnetic fields are discussed. We found that $J_1$ is produced by weak collective pinning on the oxygen vacancies in CuO$_2$ planes while $J_2$ is caused by strong pinning on the Y$_2$O$_3$ precipitates. $J_1$ component weakly changes with field and quasi-exponentially decays with temperature, disappearing at $T simeq 30$--40~K. Rapid relaxation of $J_1$ causes formation of the normalized relaxation rate peak at $T simeq 20$~K. $J_2$ component is suppressed by field as $J_2propto B^{-0.54}$ and decays with temperature following to the power law $J_2propto(1 - T/T_mathrm{dp} )^alpha$ where $T_mathrm{dp}$ is the depinning temperature. Detailed comparison of the experimental data with pinning theories is presented.
The ability of high-temperature superconductors (HTSs) to carry very large currents with almost no dissipation makes them irreplaceable for high-power applications. The development and further improvement of HTS-based cables requires an in-depth understanding of the superconducting vortex dynamics in presence of complex pinning landscapes. We present a critical current analysis of a real HTS sample in a magnetic field by combining state-of-the-art large-scale Ginzburg-Landau simulations with reconstructive three-dimensional scanning transmission electron microscopy tomography of the pinning landscape in Dy-doped YBa$_2$Cu$_3$O$_{7-delta}$. This methodology provides a unique look at the vortex dynamics in the presence of a complex pinning landscape, responsible for the high current-carrying capacity characteristic of commercial HTS wires. Our method demonstrates very good functional and quantitative agreement of the critical current between simulation and experiment, providing a new predictive tool for HTS wires design.
Most measurements of critical current densities in YBa$_2$Cu$_3$O$_{7-delta}$ thin films to date have been performed on films where the textit{c}-axis is grown normal to the film surface. With such films, the analysis of the dependence of $j_c$ on the magnetic field angle is complex. The effects of extrinsic contributions to the angular field dependence of $j_c$, such as the measurement geometry and disposition of pinning centres, are convoluted with those intrinsically due to the anisotropy of the material. As a consequence of this, it is difficult to distinguish between proposed FLL structure models on the basis of angular critical current density measurements on textit{c}-axis films. Films grown on mis-cut (vicinal) substrates have a reduced measurement symmetry and thus provide a greater insight into the critical current anisotropy. In this paper previous descriptions of the magnetic field angle dependence of $j_c$ in YBa$_2$Cu$_3$O$_{7-delta}$ are reviewed. Measurements on YBa$_2$Cu$_3$O$_{7-delta}$ thin films grown on a range of vicinal substrates are presented and the results interpreted in terms of the structure and dimensionality of the FLL in YBa$_2$Cu$_3$O$_{7-delta}$. There is strong evidence for a transition in the structure of the flux line lattice depending on magnetic field magnitude, orientation and temperature. As a consequence, a simple scaling law can not, by itself, describe the observed critical current anisotropy in YBa$_2$Cu$_3$O$_{7-delta}$. The experimentally obtained $j_c(theta)$ behaviour of YBCO is successfully described in terms of a kinked vortex structure for fields applied near parallel to the textit{a-b} planes.
Doping is one of the most relevant paths to tune the functionality of cuprates, it determines carrier density and the overall physical properties of these impressive superconducting materials. We present an oxygen doping study of YBa$_2$Cu$_3$O$_{7-delta}$ (YBCO) thin films from underdoped to overdoped state, correlating the measured charge carrier density, $n_textrm{H}$, the hole doping, $p$, and the critical current density, $J_textrm{c}$. Our results show a continuous increase of $J_textrm{c}$ with charge carrier density, reaching 90 MA/cm$^2$ at 5 K for $p$-doping at the Quantum Critical Point (QCP), linked to an increase of the superconducting condensation energy. The ultra-high $J_textrm{c}$ achived corresponds to a third of the depairing current, i.e. a value 60 % higher than ever reported in YBCO films. The overdoped regime is characterized by a sudden increase of $n_textrm{H}$, associated to the reconstruction of the Fermi-surface at the QCP. Overdoping YBCO opens a promising route to extend the current carrying capabilities of REBCO coated conductors for applications.
We have studied the normal-to-superconducting phase transition in optimally-doped YBa$_2$Cu$_3$O$_{7-delta}$ in zero external magnetic field using a variety of different samples and techniques. Using DC transport measurements, we find that the dynamical critical exponent $z=1.54pm0.14$, and the static critical exponent $ u=0.66pm0.10$ for both films (when finite-thickness effects are included in the data analysis) and single crystals (where finite-thickness effects are unimportant). We also measured thin films at different microwave frequencies and at different powers, which allowed us to systematically probe different length scales to avoid finite-thickness effects. DC transport measurements were also performed on the films used in the microwave experiments to provide a further consistency check. These microwave and DC measurements yielded a value of z consistent with the other results, $z=1.55pm0.15$. The neglect of finite-thickness, finite-current, and finite-frequency effects may account for the wide ranges of values for $ u$ and $z$ previously reported in the literature.
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