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Register a new userUltrafast laser-induced changes of the magnetic anisotropy in a low-symmetry iron garnet film
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Added by
Alexandra Kalashnikova
Publication date
2015
fields
Physics
and research's language is
English
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We explore a thermal mechanism of changing the anisotropy by femtosecond laser pulses in dielectric ferrimagnetic garnets by taking a low symmetry (YBiPrLu)3(FeGa)5O12 film grown on the (210)-oriented Gd3Ga5O12 substrate as a model media. We demonstrate by means of spectral magneto-optical pump-probe technique and phenomenological analysis, that the magnetization precession in such a film is triggered by laser-induced changes of the growth-induced magnetic anisotropy along with the well-known ultrafast inverse Faraday effect. The change of magnetic anisotropy is mediated by the lattice heating induced by laser pulses of arbitrary polarization on a picosecond time scale. We show that the orientation of the external magnetic field with respect to the magnetization easy plane noticeably affects the precession excited via the anisotropy change. Importantly, the relative contributions from the ultrafast inverse Faraday effect and the change of different growth-induced anisotropy parameters can be controlled by varying the applied magnetic field strength and direction. As a result, the amplitude and the initial phase of the excited magnetization precession can be gradually tuned.
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Laser induced ultrafast demagnetization in ferromagnetic metals was discovered almost 20 years ago, but currently there is still lack of consensus on the microscopic mechanism responsible for the corresponding transfer of angular momentum and energy between electron, lattice and spin subsystems. A distinct, but intrinsically correlated phenomenon occurring on a longer timescale is the magnetization precession after the ultrafast demagnetization process, if a magnetic field is applied to tilt the magnetization vector away from its easy direction, which can be attributed to the change of anisotropy after laser heating. In an in-plane magnetized Pt/Co/Pt thin film with perpendicular interface anisotropy, we found excellent agreement between theoretical prediction with plausible parameters and experimental data measured using time resolved magneto-optical Kerr effect. This agreement confirms that the time evolution of the anisotropy field, which is driven by the interaction between electrons and phonons, determines the magnetization precession completely. A detailed analysis shows that, even though the whole sample is magnetized in-plane, the dynamic interface anisotropy field dictates the initial phase of the magnetization precession, highlighting the significance of the interface anisotropy field in laser induced magnetization precession.
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