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Register a new userEntanglement-induced Kondo screening in atomic spin chains
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Quantum entanglement permeates the complex ground states of correlated electron materials defying single-particle descriptions. Coupled magnetic atoms have potential as model systems for entanglement in condensed matter giving the opportunity to create artificial many-body states which can be controlled by tuning the underlying interactions. They provide an avenue to unravel the complexities of correlated-electron materials. Here we use low temperature scanning tunnelling microscopy (STM) and atomic manipulation to tune entanglement in chains of magnetic atoms. We find that a Kondo singlet state can emerge from this entanglement. The many electron Kondo state is based on the screening of the entangled spin ground state of the chain by substrate electrons and can be engineered to envelop at least ten magnetic atoms. The concomitant Kondo resonance measured in the differential conductance enables the electric read-out of entanglement. By tuning composition and coupling strength within atomic chains it is possible to create model spin chains with defined entanglement. This lays the foundation for a new class of experiments to construct exotic correlated-electron materials atom by atom.
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We study the time evolution of bi- and tripartite operator mutual information of the time-evolution operator and Paulis spin operators in the one-dimensional Ising model with magnetic field and the disordered Heisenberg model. In the Ising model, the early-time evolution qualitatively follows an effective light cone picture, and the late-time value is well described by Pages value for a random pure state. In the Heisenberg model with strong disorder, we find many-body localization prevents the information from propagating and being delocalized. We also find an effective Ising Hamiltonian describes the time evolution of bi- and tripartite operator mutual information for the Heisenberg model in the large disorder regime.
The Kondo effect is a key many-body phenomenon in condensed matter physics. It concerns the interaction between a localised spin and free electrons. Discovered in metals containing small amounts of magnetic impurities, it is now a fundamental mechanism in a wide class of correlated electron systems. Control over single, localised spins has become relevant also in fabricated structures due to the rapid developments in nano-electronics. Experiments have already demonstrated artificial realisations of isolated magnetic impurities at metallic surfaces, nanometer-scale magnets, controlled transitions between two-electron singlet and triplet states, and a tunable Kondo effect in semiconductor quantum dots. Here, we report an unexpected Kondo effect realised in a few-electron quantum dot containing singlet and triplet spin states whose energy difference can be tuned with a magnetic field. This effect occurs for an even number of electrons at the degeneracy between singlet and triplet states. The characteristic energy scale is found to be much larger than for the ordinary spin-1/2 case.
Using strong-disorder renormalization group, numerical exact diagonalization, and quantum Monte Carlo methods, we revisit the random antiferromagnetic XXZ spin-1/2 chain focusing on the long-length and ground-state behavior of the average time-independent spin-spin correlation function C(l)=upsilon l^{-eta}. In addition to the well-known universal (disorder-independent) power-law exponent eta=2, we find interesting universal features displayed by the prefactor upsilon=upsilon_o/3, if l is odd, and upsilon=upsilon_e/3, otherwise. Although upsilon_o and upsilon_e are nonuniversal (disorder dependent) and distinct in magnitude, the combination upsilon_o + upsilon_e = -1/4 is universal if C is computed along the symmetric (longitudinal) axis. The origin of the nonuniversalities of the prefactors is discussed in the renormalization-group framework where a solvable toy model is considered. Moreover, we relate the average correlation function with the average entanglement entropy, whose amplitude has been recently shown to be universal. The nonuniversalities of the prefactors are shown to contribute only to surface terms of the entropy. Finally, we discuss the experimental relevance of our results by computing the structure factor whose scaling properties, interestingly, depend on the correlation prefactors.
Linear and nonlinear transport of quantum wires is investigated at a magnetic field where spin-split one-dimensional (1D) subbands are equidistant in energy. In this seldom-studied regime, experiments are consistent with a density-dependent energy gap between spin subbands, and with a complete spin polarization of the first 1D subband under a large source-drain bias at zero field.
The ability to make electrical contact to single molecules creates opportunities to examine fundamental processes governing electron flow on the smallest possible length scales. We report experiments in which we controllably stretch individual cobalt complexes having spin S = 1, while simultaneously measuring current flow through the molecule. The molecules spin states and magnetic anisotropy were manipulated in the absence of a magnetic field by modification of the molecular symmetry. This control enabled quantitative studies of the underscreened Kondo effect, in which conduction electrons only partially compensate the molecular spin. Our findings demonstrate a mechanism of spin control in single-molecule devices and establish that they can serve as model systems for making precision tests of correlated-electron theories.
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