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Measuring the dynamic structure factor of a quantum gas undergoing a structural phase transition

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 Added by Tobias Donner
 Publication date 2015
  fields Physics
and research's language is English




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The dynamic structure factor is a central quantity describing the physics of quantum many-body systems, capturing structure and collective excitations of a material. In condensed matter, it can be measured via inelastic neutron scattering, which is an energy-resolving probe for the density fluctuations. In ultracold atoms, a similar approach could so far not be applied due to the diluteness of the system. Here, we report on a direct, real-time and non-destructive measurement of the dynamic structure factor of a quantum gas exhibiting cavity-mediated long-range interactions. The technique relies on inelastic scattering of photons, stimulated by the enhanced vacuum field inside a high finesse optical cavity. We extract the density fluctuations, their energy and lifetime while the system undergoes a structural phase transition. We observe an occupation of the relevant quasi-particle mode on the level of a few excitations, and provide a theoretical description of this dissipative quantum many-body system.

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Quantum gases of light, as photons or polariton condensates in optical microcavities, are collective quantum systems enabling a tailoring of dissipation from e.g. cavity loss. This makes them a tool to study dissipative phases, an emerging subject in quantum manybody physics. Here we experimentally demonstrate a non-Hermitian phase transition of a photon Bose-Einstein condensate to a new dissipative phase, characterized by a biexponential decay of the condensates second-order coherence. The phase transition occurs due to the emergence of an exceptional point in the quantum gas. While Bose-Einstein condensation is usually connected to ordinary lasing by a smooth crossover, the observed phase transition separates the novel, biexponential phase from both lasing and an intermediate, oscillatory condensate regime. Our findings pave the way for studies of a wide class of dissipative quantum phases, for instance in topological or lattice systems.
We investigate the dynamic structure factor of a system of Bose particles at zero temperature using quantum Monte Carlo methods. Interactions are modeled using a hard-sphere potential of size $a$ and simulations are performed for values of the gas parameter $na^3$ ranging from the dilute regime up to densities $n$ where the thermodynamically stable phase is a solid. With increasing density we observe a crossover of the dispersion of elementary excitations from a Bogoliubov-like spectrum to a phonon--maxon--roton curve and the emergence of a broad multiphonon contribution accompanying the single-quasiparticle peak. In particular, for $na^3=0.2138$, which corresponds to superfluid $^4$He at equilibrium density, the extracted spectrum turns out to be in good agreement with the experimental energy--momentum dispersion relation in the roton region and for higher momenta. The behavior of the spectral function at the same density in the stable solid and metastable gas phase above the freezing point is also discussed.
We observe a structural phase transition between two configurations of a superradiant crystal by coupling a Bose-Einstein condensate to an optical cavity and applying imbalanced transverse pump fields. We find that this first order phase transition is accompanied by transient dynamics of the order parameter which we measure in real-time. The phase transition and the excitation spectrum can be derived from a microscopic Hamiltonian in quantitative agreement with our experimental data.
The formation of an equilibrium quantum state from an uncorrelated thermal one through the dynamical crossing of a phase transition is a central question of non-equilibrium many-body physics. During such crossing, the system breaks its symmetry by establishing numerous uncorrelated regions separated by spontaneously-generated defects, whose emergence obeys a universal scaling law with the quench duration. Much less is known about the ensuing re-equilibrating or coarse-graining stage, which is governed by the evolution and interactions of such defects under system-specific and external constraints. In this work we perform a detailed numerical characterization of the entire non-equilibrium process, addressing subtle issues in condensate growth dynamics and demonstrating the quench-induced decoupling of number and coherence growth during the re-equilibration process. Our unique visualizations not only reproduce experimental measurements in the relevant regimes, but also provide valuable information in currently experimentally-inaccessible regimes.
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We investigate, both experimentally and theoretically, the quench dynamics of antiferromagnetic spinor Bose-Einstein condensates in the vicinity of a zero temperature quantum phase transition at zero quadratic Zeeman shift q. Both the rate of instability and the associated finite wavevector of the unstable modes - show good agreement with predictions based upon numerical solutions to the Bogoliubov de-Gennes equations. A key feature of this work is inclusion of magnetic field inhomogeneities that smooth the phase transition. Once these were removed, we observed a dramatic sharpening of the transition point, which could then be resolved within a quadratic Zeeman shift of only 1-2 Hz. Our results point to the use of dynamics, rather than equilibrium quantities for high precision measurements of phase transitions in quantum gases.
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