Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userGlass-like slow dynamics in a colloidal solid with multiple ground states
328
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
We study the phase ordering dynamics of a two dimensional model colloidal solid using molecular dynamics simulations. The colloid particles interact with each other with a Hamaker potential modified by the presence of equatorial patches of attractive and negative regions. The total interaction potential between two such colloids is, therefore, strongly directional and has three-fold symmetry. Working in the canonical ensemble, we determine the tentative phase diagram in the density-temperature plane which features three distinct crystalline ground states viz, a low density honeycomb solid followed by a rectangular solid at higher density, which eventually transforms to a close packed triangular structure as the density is increased further. We show that when cooled rapidly from the liquid phase along isochores, the system undergoes a transition to a strong glass while slow cooling gives rise to crystalline phases. We claim that geometrical frustration arising from the presence of many crystalline ground states causes glassy ordering and dynamics in this solid. Our results may be easily confirmed by suitable experiments on patchy colloids.
rate research
Read More
Spin glasses and many-body localization (MBL) are prime examples of ergodicity breaking, yet their physical origin is quite different: the former phase arises due to rugged classical energy landscape, while the latter is a quantum-interference effect. Here we study quantum dynamics of an isolated 1d spin-glass under application of a transverse field. At high energy densities, the system is ergodic, relaxing via resonance avalanche mechanism, that is also responsible for the destruction of MBL in non-glassy systems with power-law interactions. At low energy densities, the interaction-induced fields obtain a power-law soft gap, making the resonance avalanche mechanism inefficient. This leads to the persistence of the spin-glass order, as demonstrated by resonance analysis and by numerical studies. A small fraction of resonant spins forms a thermalizing system with long-range entanglement, making this regime distinct from the conventional MBL. The model considered can be realized in systems of trapped ions, opening the door to investigating slow quantum dynamics induced by glassiness.
We study AKLT models on locally tree-like lattices of fixed connectivity and find that they exhibit a variety of ground states depending upon the spin, coordination and global (graph) topology. We find a) quantum paramagnetic or valence bond solid ground states, b) critical and ordered Neel states on bipartite infinite Cayley trees and c) critical and ordered quantum vector spin glass states on random graphs of fixed connectivity. We argue, in consonance with a previous analysis, that all phases are characterized by gaps to local excitations. The spin glass states we report arise from random long ranged loops which frustrate Neel ordering despite the lack of randomness in the coupling strengths.
We present numerical simulations of a model of cellulose consisting of long stiff rods, representing cellulose microfibrils, connected by stretchable crosslinks, representing xyloglucan molecules, hydrogen bonded to the microfibrils. Within a broad range of temperature the competing interactions in the resulting network give rise to a slow glassy dynamics. In particular, the structural relaxation described by orientational correlation functions shows a logarithmic time dependence. The glassy dynamics is found to be due to the frustration introduced by the network of xyloglucan molecules. Weakening of interactions between rod and xyloglucan molecules results in a more marked reorientation of cellulose microfibrils, suggesting a possible mechanism to modify the dynamics of the plant cell wall.
We use a simple model to extend network models for activated dynamics to a continuous landscape with a well-defined notion of distance and a direct connection to many-body systems. The model consists of a tracer in a high-dimensional funnel landscape with no disorder. We find a non-equilibrium low-temperature phase with aging dynamics, that is effectively equivalent to that of models with built-in disorder, such as Trap Model, Step Model and REM.
We develop a field-theoretic perturbation method preserving the fluctuation-dissipation relation (FDR) for the dynamics of the density fluctuations of a noninteracting colloidal gas plunged in a quenched Gaussian random field. It is based on an expansion about the Brownian noninteracting gas and can be considered and justified as a low-disorder or high-temperature expansion. The first-order bare theory yields the same memory integral as the mode-coupling theory (MCT) developed for (ideal) fluids in random environments, apart from the bare nature of the correlation functions involved. It predicts an ergodic dynamical behavior for the relaxation of the density fluctuations, in which the memory kernels and correlation functions develop long-time algebraic tails. A FDR-consistent renormalized theory is also constructed from the bare theory. It is shown to display a dynamic ergodic-nonergodic transition similar to the one predicted by the MCT at the level of the density fluctuations, but, at variance with the MCT, the transition does not fully carry over to the self-diffusion, which always reaches normal diffusive behavior at long time, in agreement with known rigorous results.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
