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Register a new userMagneto-optical properties of paramagnetic superrotors
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We study the dynamics of paramagnetic molecular superrotors in an external magnetic field. Optical centrifuge is used to create dense ensembles of oxygen molecules in ultra-high rotational states. It is shown for the first time, that the gas of rotating molecules becomes optically birefringent in the presence of magnetic field. The discovered effect of magneto-rotational birefringence indicates preferential alignment of molecular axes along the field direction. We provide an intuitive qualitative model, in which the influence of the applied magnetic field on the molecular orientation is mediated by the spin-rotation coupling. This model is supported by the direct imaging of the distribution of molecular axes, the demonstration of the magnetic reversal of the rotational Raman signal, and by numerical calculations.
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A magneto-optical trap (MOT) of atoms or molecules is studied when two lasers of different detunings and polarization are used. Especially for $Jrightarrow J,J-1$ transitions, a scheme using more than one frequency per transition and different polarization is required to create a significant force. Calculations have been performed with the simplest forms of the $Jrightarrow J-1$ case (i.e. $J=1 rightarrow J=0$) and $Jrightarrow J$ case (i.e. $J=1/2 rightarrow J=1/2$). A one dimensional (1D) model is presented and a complete 3D simulation using rate equations confirm the results. Even in the absence of Zeeman effect in the excited state, where no force is expected in the single laser field configuration, we show that efficient cooling and trapping forces are restored in our configuration. We study this mechanism for the C$_2^-$ molecular anion as a typical example of the interplay between the two simple transitions $J rightarrow J,J-1$.
A new configuration for observation of magneto-optical subnatural-linewidth resonances of electromagnetically induced absorption (EIA) in alkali vapor has been verified experimentally. The configuration includes using two counter-propagating pump and probe light waves with mutually orthogonal linear polarizations, exciting an open optical transition of an alkali atom in the presence of a buffer gas. The main advantage of the novel observation scheme consists in the possibility of obtaining simultaneously high-contrast and quite narrow nonlinear signals. Here a 2.5-cm long rubidium-87 vapor cell filled with Ar buffer gas is used, and the excited optical transition is the F$_g$=2 $to$ F$_e$=1 of the D$_1$ line. The signals registered reach a contrast of 57.7% with a FWHM of 7.2 mG. The contrast with respect to a wide Doppler pedestal well exceeds 100%. To our knowledge, to date this is the best result for EIA resonances in terms of contrast-to-width ratio. In general, the results demonstrate that the new magneto-optical scheme has very good prospects for various applications in quantum metrology, nonlinear optics and photonics.
Arrays of trapped ultracold molecules represent a promising platform for implementing a universal quantum computer. DeMille has detailed a prototype design based on Stark states of polar $^1Sigma$ molecules as qubits. Herein, we consider an array of polar $^2Sigma$ molecules which are, in addition, inherently paramagnetic and whose Hunds case (b) free-rotor states are Bell states. We show that by subjecting the array to combinations of concurrent homogeneous and inhomogeneous electric and magnetic fields, the entanglement of the arrays Stark and Zeeman states can be tuned and the qubit sites addressed. Two schemes for implementing an optically controlled CNOT gate are proposed and their feasibility discussed in the face of the broadening of spectral lines due to dipole-dipole coupling and the inhomogeneity of the electric and magnetic fields.
We present our technique to create a magneto-optical trap for dysprosium atoms using the narrow-line cooling transition at 626$,$nm to achieve suitable conditions for direct loading into an optical dipole trap. The magneto-optical trap is loaded from an atomic beam via a Zeeman slower using the strongest atomic transition at 421$,$nm. With this combination of two cooling transitions we can trap up to $2.0cdot10^8$ atoms at temperatures down to 6$, mu$K. This cooling approach is simpler than present work with ultracold dysprosium and provides similar starting conditions for a transfer to an optical dipole trap.
Optical and magneto-optical properties of ZnMnO films grown at low temperature by Atomic Layer Deposition are discussed. A strong polarization of excitonic photoluminescence is reported, surprisingly observed without splitting or spectral shift of excitonic transitions. Present results suggest possibility of Mn recharging in ZnO lattice. Strong absorption, with onset at about 2.1 eV, is related to Mn 2+ to 3+ photo-ionization. We propose that the observed strong circular polarization of excitonic emission is of a similar character as the one observed by us for ZnSe:Cr.
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