Unified theory of spiral magnetism in the harmonic-honeycomb iridates {alpha}, {beta}, {gamma} Li2IrO3


Abstract in English

A family of insulating iridates with chemical formula Li$_2$IrO$_3$ has recently been discovered, featuring three distinct crystal structures $alpha,beta,gamma$ (honeycomb, hyperhoneycomb, stripyhoneycomb). Measurements on the three-dimensional polytypes, $beta$- and $gamma$-Li$_2$IrO$_3$, found that they magnetically order into remarkably similar spiral phases, exhibiting a non-coplanar counter-rotating spiral magnetic order with equivalent q=0.57 wavevectors. We examine magnetic Hamiltonians for this family and show that the same triplet of nearest-neighbor Kitaev-Heisenberg-Ising (KJI) interactions reproduces this spiral order on both $beta,gamma$-Li$_2$IrO$_3$ structures. We analyze the origin of this phenomenon by studying the model on a 1D zigzag chain, a structural unit common to the three polytypes. The zigzag-chain solution transparently shows how the Kitaev interaction stabilizes the counter-rotating spiral, which is shown to persist on restoring the inter-chain coupling. Our minimal model makes a concrete prediction for the magnetic order in $alpha$-Li$_2$IrO$_3$.

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