Lee-Yang zeros are points on the complex plane of magnetic field where the partition function of a spin system is zero and therefore the free energy diverges. Lee-Yang zeros and their generalizations are ubiquitous in many-body systems and they fully characterize the analytic properties of the free energy and hence thermodynamics of the systems. Determining the Lee-Yang zeros is not only fundamentally important for conceptual completeness of thermodynamics and statistical physics but also technically useful for studying many-body systems. However, Lee-Yang zeros have never been observed in experiments, due to the intrinsic difficulty that Lee-Yang zeros would occur only at complex values of magnetic field, which are unphysical. Here we report the first observation of Lee-Yang zeros, by measuring quantum coherence of a probe spin coupled to an Ising-type spin bath. As recently proposed, the quantum evolution of the probe spin introduces a complex phase factor, and therefore effectively realizes an imaginary magnetic field on the bath. From the measured Lee-Yang zeros, we reconstructed the free energy of the spin bath and determined its phase transition temperature. This experiment demonstrates quantum coherence probe as a useful approach to studying thermodynamics in the complex plane, which may reveal a broad range of new phenomena that would otherwise be inaccessible if physical parameters are restricted to be real numbers.
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