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Register a new userLow-energy electronic properties of clean CaRuO$_3$: elusive Landau quasiparticles
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We have prepared high-quality epitaxial thin films of CaRuO$_3$ with residual resistivity ratios up to 55. Shubnikov-de Haas oscillations in the magnetoresistance and a $T^2$ temperature dependence in the electrical resistivity only below 1.5 K, whose coefficient is substantially suppressed in large magnetic fields, establish CaRuO$_3$ as a Fermi liquid (FL) with anomalously low coherence scale. Non-Fermi liquid (NFL) $T^{3/2}$ dependence is found between 2 and 25 K. The high sample quality allows access to the intrinsic electronic properties via THz spectroscopy. For frequencies below 0.6 THz, the conductivity is Drude-like and can be modeled by FL concepts, while for higher frequencies non-Drude behavior, inconsistent with FL predictions, is found. This establishes CaRuO$_3$ as a prime example of optical NFL behavior in the THz range.
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We have carried out extensive comparative studies of the structural and transport properties of CaRuO$_3$ thin films grown under various oxygen pressure. We find that the preferred orientation and surface roughness of the films are strongly affected by the oxygen partial pressure during growth. This in turn affects the electrical and magnetic properties of the films. Films grown under high oxygen pressure have the least surface roughness and show transport characteristics of a good metal down to the lowest temperature measured. On the other hand, films grown under low oxygen pressures have high degree of surface roughness and show signatures of ferromagnetism. We could verify that the low frequency resistance fluctuations (noise) in these films arise due to thermally activated fluctuations of local defects and that the defect density matches with the level of disorder seen in the films through structural characterizations.
Optical conductivity spectra $sigma_1(omega)$ of paramagnetic CaRuO$_3$ are investigated at various temperatures. At T=10 K, it shows a non-Fermi liquid behavior of $sigma_1(omega)sim 1/{omega}^{frac 12}$, similar to the case of a ferromagnet SrRuO$_3$. As the temperature ($T$) is increased, on the other hand, $sigma_1(omega)$ in the low frequency region is progressively suppressed, deviating from the $1/{omega}^{frac 12%}$-dependence. Interestingly, the suppression of $sigma_1(omega)$ is found to scale with $omega /T$ at all temperatures. The origin of the $% omega /T$ scaling behavior coupled with the non-Fermi liquid behavior is discussed.
Temperature-dependent reflectivity measurements on the kagome metal CsV$_3$Sb$_5$ in a broad frequency range of $50-20000$ cm$^{-1}$ down to $T$=10 K are reported. The charge-density wave (CDW) formed below $T_{rm CDW}$ = 94 K manifests itself in a prominent spectral-weight transfer from low to higher energy regions. The CDW gap of 60-75 meV is observed at the lowest temperature and shows significant deviations from an isotropic BCS-type mean-field behavior. Absorption peaks appear at frequencies as low as 200 cm$^{-1}$ and can be identified with interband transitions according to density-functional calculations. The change in the interband absorption compared to KV$_3$Sb$_5$ reflects the inversion of band saddle points between the K and Cs compounds. Additionally, a broader and strongly temperature-dependent absorption feature is observed below 1000 cm$^{-1}$ and assigned to a displaced Drude peak. It reflects localization effects on charge carriers.
Motivated by theory and experiments on strain induced pseudo-Landau levels (LLs) of Dirac fermions in graphene and topological materials, we consider its extension for Bogoliubov quasiparticles (QPs) in a nodal superconductor (SC). We show, using an effective low energy description and numerical lattice calculations for a d-wave SC, that a spatial variation of the electronic hopping amplitude or a spatially varying s-wave pairing component can act as a pseudo-magnetic field for the Bogoliubov QPs, leading to the formation of pseudo-LLs. We propose realizations of this phenomenon in the cuprate SCs, via strain engineering in films or nanowires, or s-wave proximity coupling in the vicinity of a nematic instability, and discuss its signatures in tunneling experiments.
Selenium and tellurium are among the few elements that form $AB$O$_3$ perovskite structures with a four valent ion in the $A$ site. This leads to highly distorted structures and unusual magnetic behavior. Here we investigate the Co and Ni selenite and tellurite compounds, CoSeO$_3$, CoTeO$_3$, NiSeO$_3$ and NiTeO$_3$ using first principles calculations. We find an interplay of crystal field and Jahn-Teller distortions that underpin the electronic and magnetic properties. While all compounds are predicted to show an insulating G-type antiferromagnetic ground state, there is a considerable difference in the anisotropy of the exchange interactions between the Ni and Co compounds. This is related to the Jahn-Teller distortion. Finally, we observe that these four compounds show characteristics generally associated with Mott insulators, even when described at the level of standard density functional theory. These are then dense bulk band or Slater, Mott-type insulators.
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