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Register a new userRevisiting heat capacity of bulk polycrystalline YBa2Cu3O7-{delta}
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In this letter, we present the superconducting property characterization of a phase pure reasonably good quality YBa2Cu3O7-{delta} sample. Studied compound is crystallized in orthorhombic Pmmm space group with lattice parameters a, b, and c are 3.829(2) {AA}, 3.887(1) {AA} and 11.666(3) {AA} respectively. Bulk superconductivity is observed below 90K as evidenced by resistivity and dc/ac magnetization measurements. The resistivity under magnetic field ({rho}TH) measurements showed clearly both the intra-grain and inter-grain transitions, which are supplemented by detailed (varying frequency and amplitude) ac susceptibility studies as well. The upper critical field at 0K i.e., Hc2(0) being determined from {rho}TH measurements with 50% criteria of resistivity drope is ~ 70 Tesla. Studied polycrystalline YBa2Cu3O7-{delta} is subjected to detailed heat capacity (CP) studies. Cp exhibited well defined anomaly at below 90 K, which decreases with applied field. Though the Cp anomaly/peak at Tc reduces with applied field, the same is not completely suppressed in high applied fields of up to 12 Tesla. The Sommerfeld constant ({gamma}) and Debye temperature ({Theta}D) as determined from low temperature fitting of CP(T) data to Sommerfeld-Debye model, are 10.65 mJ/mole-K2 and 312.3 K respectively. The results are compared with existing literature on bulk polycrystalline superconducting YBa2Cu3O7-{delta} sample
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Thin films of optimally-doped (001)-oriented YBa2Cu3O7-{delta} are epitaxially integrated on silicon (001) through growth on a single crystalline SrTiO3 buffer. The former is grown using pulsed-laser deposition and the latter is grown on Si using oxide molecular beam epitaxy. The single crystal nature of the SrTiO3 buffer enables high quality YBa2Cu3O7-{delta} films exhibiting high transition temperatures to be integrated on Si. For a 30 nm thick SrTiO3 buffer, 50 nm thick YBa2Cu3O7-{delta} films that exhibit a transition temperature of ~ 93 K, and a narrow transition width (< 5 K) are achieved. The integration of single crystalline YBa2Cu3O7-{delta} on Si (001) paves the way for the potential exploration of cuprate materials in a variety of applications.
We present an angle-resolved photoelectron spectroscopy study of YBa2Cu3O7-delta films in situ grown by pulsed laser deposition. We have successfully produced underdoped surfaces with ordered oxygen vacancies within the CuO chains resulting in a clear ortho-II band folding of the Fermi surface. This indicates that order within the CuO chains affects the electronic properties of the CuO2 planes. Our results highlight the importance of having not only the correct surface carrier concentration, but also a very well ordered and clean surface in order that photoemission data on this compound be representative of the bulk.
Using spin polarized neutron reflectivity experiments, we demonstrate an unusual proximity behaviour when the superconductor (SC) and the ferromagnet (FM) are coupled through an insulator (I) in YBa2Cu3O7-{delta} (SC)/SrTiO3 (I)/La0.67Sr0.33MnO3 (FM) heterostructures. We have observed an unexpected magnetic modulation at the interface region of the FM below the superconducting transition temperature. The magnetization of the FM layer at the I/FM interface was drastically reduced as compared to the magnetization in the rest of the FM layer. This result indicates that the Cooper pairs tunnel across the insulator and interact with the local magnetization at the interface region (extending ~ 30 {AA}) of the FM causing modification of the magnetization at the interface. This unexpected magnetic behavior cannot be explained on the basis of the existing theoretical models. However, the length scale associated here clearly suggests the long range proximity effect as a result of tunneling of Cooper pairs.
We present a detailed study of the electrical transport properties of YBa2Cu3O7-{delta} thin film. The irreversibility fields ({mu}_0 H_irr), upper critical fields ({mu}_0 H_C2), penetration depths ({lambda}) and coherence lengths ({xi} ) of the YBa2Cu3O7-{delta} materials are deduced from the resistivity curves. Itis observed that {mu}_0 H_irr, {mu}_0 H_C2 and {Delta}Tc of the film strongly depend on the direction and strength of the field. The coherence length {xi} (0) and penetration depth {lambda} (0) values at T = 0 K has been calculated from the irreversibility fields ({mu}_0 H_irr) and upper critical fields ({mu}_0 H_C2) respectively. Based on all the results, the change of the superconducting properties as a function of the magnetic field direction presents the anisotropy of the sample produced.
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