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We observed electromagnetically-induced-transparency-based four-wave mixing (FWM) in the pulsed regime at low light levels. The FWM conversion efficiency of 3.8(9)% was observed in a four-level system of cold 87Rb atoms using a driving laser pulse with a peak intensity of approximately 80 {mu}W/cm^2, corresponding to an energy of approximately 60 photons per atomic cross section. Comparison between the experimental data and the theoretical predictions proposed by Harris and Hau [Phys. Rev. Lett. 82, 4611 (1999)] showed good agreement. Additionally, a high conversion efficiency of 46(2)% was demonstrated when applying this scheme using a driving laser intensity of approximately 1.8 mW/cm^2. According to our theoretical predictions, this FWM scheme can achieve a conversion efficiency of nearly 100% when using a dense medium with an optical depth of 500.
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We develop a general Hamiltonian treatement of spontaneous four-wave mixing in a microring resonator side-coupled to a channel waveguide. The effect of scattering losses in the ring is included, as well as parasitic nonlinear effects including self- and cross-phase modulation. A procedure for computing the output of such a system for arbitrary parameters and pump states is presented. For the limit of weak pumping an expression for the joint spectral intensity of generated photon pairs, as well as the singles-to-coincidences ratio, is derived.
We show that a simple scheme based on nondegenerate four-wave mixing in a hot atomic vapor behaves like a near-perfect phase-insensitive optical amplifier, which can generate bright twin beams with a measured quantum noise reduction in the intensity difference of more than 8 dB, close to the best optical parametric amplifiers and oscillators. The absence of a cavity makes the system immune to external perturbations, and the strong quantum noise reduction is observed over a large frequency range.
Using four-wave mixing in a hot atomic vapor, we generate a pair of entangled twin beams in the microsecond pulsed regime near the D1 line of $^{85}$Rb, making it compatible with commonly used quantum memory techniques. The beams are generated in the bright and vacuum-squeezed regimes, requiring two separate methods of analysis, without and with local oscillators, respectively. We report a noise reduction of up to $3.8pm 0.2$ dB below the standard quantum limit in the pulsed regime and a level of entanglement that violates an Einstein--Podolsky--Rosen inequality.
In this article, we use quantum Langevin equations to provide a theoretical understanding of the non-classical behavior of Kerr optical frequency combs when pumped below and above threshold. In the configuration where the system is under threshold, the pump field is the unique oscillating mode inside the resonator, and triggers the phenomenon of spontaneous four-wave mixing, where two photons from the pump are symmetrically up- and down-converted in the Fourier domain. This phenomenon can only be understood and analyzed from a fully quantum perspective as a consequence of the coupling between the field of the central (pumped) mode and the vacuum fluctuations of the various sidemodes. We analytically calculate the power spectra of the spontaneous emission noise, and we show that these spectra can be either single- or double peaked depending on the parameters of the system. We also calculate as well the overall spontaneous noise power per sidemode, and propose simplified analytical expressions for some particular cases. In the configuration where the system is pumped above threshold, we investigate the phenomena of quantum correlations and multimode squeezed states of light that can occur in the Kerr frequency combs originating from stimulated four-wave mixing. We show that for all stationary spatio-temporal patterns, the side-modes that are symmetrical relatively to the pumped mode in the frequency domain display quantum correlations that can lead to squeezed states of light. We also explicitly determine the phase quadratures leading to photon entanglement, and analytically calculate their quantum noise spectra. We finally discuss the relevance of Kerr combs for quantum information systems at optical telecommunication wavelengths, below and above threshold.
We experimentally determine the quantum discord present in two-mode squeezed vacuum generated by a four-wave mixing process in hot rubidium vapor. The frequency spectra of the discord, as well as the quantum and classical mutual information are also measured. In addition, the effects of symmetric attenuation introduced into both modes of the squeezed vacuum on the discord, the quantum mutual information and the classical correlations are examined experimentally. Finally, we show that due to the multi-spatial-mode nature of the four-wave mixing process, the quantum discord may exhibit sub- or superadditivity depending on which spatial channels are selected.
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