Fast polarization switching of light sources is required over a wide spectral range to investigate the symmetry of matter. In this Letter, we report the first experimental demonstration of the crossed-planar undulator technique at a seeded free-electron laser, which holds great promise for the full control and fast switching of the polarization of short-wavelength radiation. In the experiment, the polarization state of the coherent radiation at the 2nd harmonic of the seed laser is switched successfully. The experiment results confirm the theory, and pave the way for applying the crossed-planar undulator technique for the seeded X-ray free electron lasers.
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