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Register a new userEmergent honeycomb lattice in LiZn2Mo3O8
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We introduce the idea of emergent lattices, where a simple lattice decouples into two weakly-coupled lattices as a way to stabilize spin liquids. In LiZn2Mo3O8, the disappearance of 2/3rds of the spins at low temperatures suggests that its triangular lattice decouples into an emergent honeycomb lattice weakly coupled to the remaining spins, and we suggest several ways to test this proposal. We show that these orphan spins act to stabilize the spin-liquid in the $J_1-J_2$ honeycomb model and also discuss a possible 3D analogue, Ba2MoYO6 that may form a depleted fcc lattice.
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Inelastic neutron scattering for temperatures below 30 K from a powder of LiZn2Mo3O8 demonstrates this triangular-lattice antiferromagnet hosts collective magnetic excitations from spin 1/2 Mo3O13 molecules. Apparently gapless (Delta < 0.2 meV) and extending at least up to 2.5 meV, the low energy magnetic scattering cross section is surprisingly broad in momentum space and involves one third of the spins present above 100 K. The data are compatible with the presence of valence-bonds involving nearest-neighbor and next-nearest-neighbor spins forming a disordered or dynamic state.
We explore the possibility of inducing a topological insulator phase in a honeycomb lattice lacking spin-orbit interaction using a metallic (or Fermi gas) environment. The lattice and the metallic environment interact through a density-density interaction without particle tunneling, and integrating out the metallic environment produces a honeycomb sheet with in-plane oscillating long-ranged interactions. We find the ground state of the interacting system in a variational mean-field method and show that the Fermi wave vector, kF, of the metal determines which phase occurs in the honeycomb lattice sheet. This is analogous to the Ruderman-Kittel-Kasuya-Yosida (RKKY) mechanism in which the metals kF determines the interaction profile as a function of the distance. Tuning kF and the interaction strength may lead to a variety of ordered phases, including a topological insulator and anomalous quantum-hall states with complex next-nearest-neighbor hopping, as in the Haldane and the Kane-Mele model. We estimate the required range of parameters needed for the topological state and find that the Fermi vector of the metallic gate should be of the order of 3Pi/8a (with a being the graphene lattice constant). The net coupling between the layers, which includes screening in the metal, should be of the order of the honeycomb lattice bandwidth. This configuration should be most easily realized in a cold-atoms setting with two interacting Fermionic species.
The theoretical inception of the Kitaev honeycomb model has had defining influence on the experimental hunt for quantum spin liquids, bringing unprecedented focus onto the synthesis of materials with bond-directional interactions. Numerous Kitaev materials, which are believed to harbor ground states parametrically close to the Kitaev spin liquid, have been investigated since. Yet, in these materials the Kitaev interaction often comes hand in hand with off-diagonal $Gamma$ interactions -- with the competition of the two potentially giving rise to a magnetically ordered ground state. In an attempt to aid future material investigations, we study the phase diagram of the spin-1/2 Kitaev-$Gamma$ model on the honeycomb lattice. Employing a pseudofermion functional renormalization group approach which directly operates in the thermodynamic limit and captures the joint effect of thermal and quantum fluctuations, we unveil the existence of extended parameter regimes with emergent incommensurate magnetic correlations at finite temperature. We supplement our results with additional calculations on a finite cylinder geometry to investigate the impact of periodic boundary conditions on the incommensurate order, thereby providing a perspective on previous numerical studies on finite systems.
How many magnetic moments periodically arranged on a metallic surface are needed to generate a coherent Kondo lattice behavior? We investigate this fundamental issue within the particle-hole symmetric Kondo lattice model using quantum Monte Carlo simulations. Extra magnetic atoms forming closed shells around the initial impurity induce a fast splitting of the Kondo resonance at the inner shells which signals the formation of composite heavy-fermion bands. The onset of the hybridization gap matches well the enhancement of antiferromagnetic spin correlations in the plane perpendicular to the applied magnetic field, a genuine feature of the coherent Kondo lattice. In contrast, the outermost shell remains dominated by a local Kondo physics with spectral features resembling the single-impurity behavior.
We theoretically propose possible magnetism-induced negative thermal expansion in honeycomb-lattice antiferromagnets with edge-sharing networks of $MX_6$ octahedra where $M$ and $X$ are transition-metal and ligand ions, respectively. In this crystal structure, the nearest-neighbor exchange interaction is composed of two competing contributions, i.e., the antiferromagnetic contribution from a direct 180$^circ$ $M$-$M$ bond and the ferromagnetic contribution from 90$^circ$ $M$-$X$-$M$ bonds, amplitudes of which have different bond-length dependence. Numerical analysis of the spin-lattice model of the honeycomb-lattice antiferromagnets demonstrates that the negative thermal expansion can occur when the system enters the antiferromagnetic phase with lowering temperature so as to maximize the energy gain associated with the bond-length dependent antiferromagnetic exchange interaction. The present work provides a guiding principle for searching new materials and eventually contributes to diversify the family of materials that host the negative thermal expansion originating from the spin-lattice coupling on the honeycomb lattices or related crystal structures.
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