We have investigated low energy nuclear spin excitations in strongly correlated electron compound HoCrO$_3$. We observe clear inelastic peaks at $E = 22.18 pm 0.04$ $mu eV$ in both energy loss and gain sides. The energy of the inelastic peaks remains constant in the temperature range 1.5 - 40 K at which they are observed. The intensity of the inelastic peak increases at first with increasing temperature and then decreases at higher temperatures. The temperature dependence of the energy and intensity of the inelastic peaks is very unusual compared to that observed in other Nd, Co and V compounds. Huge quasielastic scattering appears at higher temperatures presumably due to the fluctuating electronic moments of the Ho ions that get increasingly disordered at higher temperatures.
We investigated the dispersion of nuclear spin waves in Nd$_2$CuO$_4$ by using neutron spin-echo spectroscopy at millikelvin temperatures. Our results show unambiguously the existence of dispersion of nuclear spin waves in Nd$_2$CuO$_4$ at T = 30 mK. A fit of the dispersion data with the spin wave dispersion formula gave the Suhl-Nakamura interaction range to be of the order of 10 {AA}.
Studying the prototypical ferromagnetic superconductor UGe$_2$ we demonstrate the potential of the Modulated IntEnsity by Zero Effort (MIEZE) technique---a novel neutron spectroscopy method with ultra-high energy resolution of at least 1~$mu$eV---for the study of quantum matter. We reveal purely longitudinal spin fluctuations in UGe$_2$ with a dual nature arising from $5f$ electrons that are hybridized with the conduction electrons. Local spin fluctuations are perfectly described by the Ising universality class in three dimensions, whereas itinerant spin fluctuations occur over length scales comparable to the superconducting coherence length, showing that MIEZE is able to spectroscopically disentangle the complex low-energy behavior characteristic of quantum materials.
The electrodynamic response of organic spin liquids with highly-frustrated triangular lattices has been measured in a wide energy range. While the overall optical spectra of these Mott insulators are governed by transitions between the Hubbard bands, distinct in-gap excitations can be identified at low temperatures and frequencies which we attribute to the quantum spin liquid state. For the strongly correlated $beta^{prime}$-EtMe$_3$-Sb-[Pd(dmit)$_2$]$_2$, we discover enhanced conductivity below $175~{rm cm}^{-1}$, comparable to the energy of the magnetic coupling $Japprox 250$ K. For $omegarightarrow 0$ these low-frequency excitations vanish faster than the charge-carrier response subject to Mott-Hubbard correlations, resulting in a dome-shape band peaked at 100~cm. Possible relations to spinons, magnons and disorder are discussed.
We have investigated the ferromagnetic phase transition of elemental Co by high-resolution neutron backscattering spectroscopy. We monitored the splitting of the nuclear levels by the hyperfine field at the Co nucleus. The energy of this hyperfine splitting is identified as the order parameter of the ferromagnetic phase transition. By measuring the temperature dependence of the energy we determined the critical exponent $beta = 0.350 pm 0.002$ and the ferromagnetic Curie temperature of $T_{text{C}} = 1400$~K. The present result of the critical exponent agrees better with the predicted value (0.367) of the 3-dimensional Heisenberg model than that determined previously by NMR.
Exotic spin-multipolar ordering in spin transition metal insulators has so far eluded unambiguous experimental observation. A less studied, but perhaps more feasible fingerprint of multipole character emerges in the excitation spectrum in the form of quadrupolar transitions. Such multipolar excitations are desirable as they can be manipulated with the use of light or electric field and can be captured by means of conventional experimental techniques. Here we study single crystals of multiferroic Sr$_2$CoGe$_2$O$_7$, and show that due to its nearly isotropic nature a purely quadrupolar bimagnon mode appears in the electron spin resonance (ESR) spectra. This non-magnetic spin-excitation couples to the electric field of the light and becomes observable for a specific experimental configuration, in full agreement with a theoretical analysis of the selection rules.
T. Chatterji
,N. Jalarvo
,C.M.N. Kumar
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(2012)
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"Direct observation of low energy nuclear spin excitations in HoCrO$_3$ by high resolution neutron spectroscopy"
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Tapan Chatterji
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