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Dilute magnetic impurities in a disordered Fermi liquid are considered close to the Anderson metal-insulator transition (AMIT). Critical Power law correlations between electron wave functions at different energies in the vicinity of the AMIT result in the formation of pseudogaps of the local density of states. Magnetic impurities can remain unscreened at such sites. We determine the density of the resulting free magnetic moments in the zero temperature limit. While it is finite on the insulating side of the AMIT, it vanishes at the AMIT, and decays with a power law as function of the distance to the AMIT. Since the fluctuating spins of these free magnetic moments break the time reversal symmetry of the conduction electrons, we find a shift of the AMIT, and the appearance of a semimetal phase. The distribution function of the Kondo temperature $T_{K}$ is derived at the AMIT, in the metallic phase and in the insulator phase. This allows us to find the quantum phase diagram in an external magnetic field $B$ and at finite temperature $T$. We calculate the resulting magnetic susceptibility, the specific heat, and the spin relaxation rate as function of temperature. We find a phase diagram with finite temperature transitions between insulator, critical semimetal, and metal phases. These new types of phase transitions are caused by the interplay between Kondo screening and Anderson localization, with the latter being shifted by the appearance of the temperature-dependent spin-flip scattering rate. Accordingly, we name them Kondo-Anderson transitions (KATs).
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Continuous-Time Quantum Monte Carlo (CT-QMC) method combined with Dynamical Mean Field Theory (DMFT) is used to calculate both Periodic Anderson Model (PAM) and Kondo Lattice Model (KLM). Different parameter sets of both models are connected by the Schrieffer-Wolff transformation. For degeneracy N=2, a special particle-hole symmetric case of PAM at half filling which always fixes one electron per impurity site is compared with the results of the KLM. We find a good mapping between PAM and KLM in the limit of large on-site Hubbard interaction U for different properties like self-energy, quasiparticle residue and susceptibility. This allows us to extract quasiparticle mass renormalizations for the f electrons directly from KLM. The method is further applied to higher degenerate case and to realsitic heavy fermion system CeRhIn5 in which the estimate of the Sommerfeld coefficient is proven to be close to the experimental value.
The low-temperature behavior of the asymmetric single-impurity Anderson model is studied by diagrammatic methods resulting in analytically controllable approximations. We first discuss the ways one can simplify parquet equations in critical regions of singularities in the two-particle vertex. The scale vanishing at the critical point defines the Kondo temperature at which the electron-hole correlation function saturates. We show that the Kondo temperature exists at any filling of the impurity level. A quasiparticle resonance peak in the spectral function, however, forms only in almost electron-hole symmetric situations. We relate the Kondo temperature with the width of the resonance peak. Finally we discuss the existence of satellite Hubbard bands in the spectral function.
The Kondo resonance at the Fermi level is well-established for the electronic structure of Ce (f1 electron) and Yb (f1 hole) based systems. In this work, we report complementary experimental and theoretical studies on the Kondo resonance in Pr-based f2 system, PrTi2Al20. Using Pr 3d-4f resonant photoemission spectroscopy and single impurity Anderson model (SIAM) calculations including the full multiplets of Pr ions, we show that an f2 system can also give rise to a Kondo resonance at the Fermi level. The Kondo resonance peak is experimentally observed through a final-state-multiplet dependent resonance and is reproduced with properly tuned hybridization strength in SIAM calculations.
It is well-known that magnetic impurities can change the symmetry class of disordered metallic systems by breaking spin and time-reversal symmetry. At low temperature these symmetries can be restored by Kondo screening. It is also known that at the Anderson metal-insulator transition, wave functions develop multifractal fluctuations with power law correlations. Here, we consider the interplay of these two effects. We show that multifractal correlations open local pseudogaps at the Fermi energy at some random positions in space. When dilute magnetic impurities are at these locations, Kondo screening is strongly suppressed. We find that when the exchange coupling J is smaller than a certain value J*, the metal-insulator transition point extends to a critical region in the disorder strength parameter and to a band of critical states. The width of this critical region increases with a power of the concentration of magnetic impurities.
Thermodynamic properties are presented for four magnetic impurity models describing delocalized fermions scattering from a localized orbital at an energy-dependent rate $Gamma(epsilon)$ which vanishes precisely at the Fermi level, $epsilon = 0$. Specifically, it is assumed that for small $|epsilon|$, $Gamma(epsilon)propto|epsilon|^r$ with $r>0$. The cases $r=1$ and $r=2$ describe dilute magnetic impurities in unconventional superconductors, ``flux phases of the two-dimensional electron gas, and zero-gap semiconductors. For the nondegenerate Anderson model, the depression of the low-energy scattering rate suppresses mixed valence in favor of local-moment behavior, and leads to a marked reduction in the exchange coupling on entry to the local-moment regime, with a consequent narrowing of the range of parameters within which the impurity spin becomes Kondo-screened. The relationship between the Anderson model and the exactly screened Kondo model with power-law exchange is examined. The intermediate-coupling fixed point identified in the latter model by Withoff and Fradkin (WF) has clear signatures in the thermodynamic properties and in the local magnetic response of the impurity. The underscreened, impurity-spin-one Kondo model and the overscreened, two-channel Kondo model both exhibit a conditionally stable intermediate-coupling fixed point in addition to unstable fixed points of the WF type. In all four models, the presence or absence of particle-hole symmetry plays a crucial role.
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