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Register a new userModified Cross-Correlation for Efficient White-Beam Inelastic Neutron Scattering Spectroscopy
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We describe a method of white-beam inelastic neutron scattering for improved measurement efficiency. The method consists of matrix inversion and selective extraction. The former is to resolve each incident energy component from the white-beam data, and the latter eliminates contamination by elastic components, which produce strong backgrounds that otherwise obfuscate the inelastic scattering components. In this method, the optimal experimental condition to obtain high efficiency will strongly depend on the specific aim of the individual experiments.
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We provide a quantitative description of a method to measure neutron-induced fission cross sections in ratio to elastic hydrogen scattering in a white-source neutron beam with the fission Time Projection Chamber. This detector has measured precision fission cross section ratios using actinide references such as $^{235}$U(n,f) and $^{238}$U(n,f). However, by employing a more precise reference such as the H(n,el) cross section there is the potential to further reduce the evaluation uncertainties of the measured cross sections. In principle the fissionTPC could provide a unique measurement by simultaneously measuring both fission fragments and proton recoils over a large solid angle. We investigate one method with a hydrogenous gas target and with the neutron energy determined by the proton recoil kinematics. This method enables the measurement to be performed in a white-source neutron beam and with the current configuration of the fissionTPC. We show that while such a measurement is feasible in the energy range of 0.5 MeV to $sim$10 MeV, uncertainties on the proton detection efficiency and the neutron energy resolution do not allow us to preform a fission ratio measurement to the desired precision. Utilizing either a direct measurement of the neutron time-of-flight for the recoil proton or a mono-energetic neutron source or some combination of both would provide a path to a sub-percent precision measurement.
An instrument and software algorithm is described for the purpose of characterization of large single crystals at the Alignment Facility (ALF) of the ISIS spallation neutron source. We describe a method for both characterizing the quality of the sample and also aligning it in a particular scattering plane. We present a software package written for this instrument and demonstrate its utility by way of an example of the structural characterization of large singles crystals of Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$. We suggest extensions and modifications of characterization instruments for future improved beamlines. It is hoped that this software will be used by the neutron user community for pre characterizing large single crystals for spectroscopy experiments and that future facilities will include such a facility as part of the spectroscopy suite at spallation neutron sources.
Spin waves in the the rare earth orthorferrite YFeO$_3$ have been studied by inelastic neutron scattering and analyzed with a full four-sublattice model including contributions from both the weak ferromagnetic and hidden antiferromagnetic orders. Antiferromagnetic (AFM) exchange interactions of $J_1 = -4.23 pm 0.08$ (nearest-neighbors only) or $J_1 = -4.77 pm 0.08$ meV and $J_2 = -0.21 pm 0.04$ meV lead to excellent fits for most branches at both low and high energies. An additional branch associated with the hidden antiferromagnetic order was observed. This work paves the way for studies of other materials in this class containing spin reorientation transitions and magnetic rare earth ions.
Experiments searching for neutrinoless double beta decay ($0 ubetabeta$) require precise energy calibration and extremely low backgrounds. One of the most popular isotopes for $0 ubetabeta$ experiments is $^{136}$Xe. In support of these experiments, the neutron inelastic scattering properties of this isotope have been measured at the GErmanium Array for Neutron Induced Excitations (GEANIE) at the Los Alamos Neutron Science Center. Time-of-flight techniques are utilized with high-purity germanium detectors to search for inelastic scattering $gamma$ rays for neutron energies between 0.7 and 100 MeV. Limits are set on production of yet-unobserved $gamma$ rays in the energy range critical for $0 ubetabeta$ studies, and measurements are made of multiple $gamma$-ray production cross sections. In particular, we have measured the production of the 1313 keV $gamma$ ray which comes from the transition of the first-excited to ground state of $^{136}$Xe. This neutron-induced $gamma$ line may be useful for a novel energy calibration technique, described in this paper.
Sodium niobate (NaNbO3) exhibits most complex sequence of structural phase transitions in perovskite family and therefore provides as excellent model system for understanding the mechanism of structural phase transitions. We report temperature dependence of inelastic neutron scattering measurements of phonon densities of states in sodium niobate. The measurements are carried out in various crystallographic phases of this material at various temperatures from 300 K to 1048 K. The phonon spectra exhibit peaks centered around 19, 37, 51, 70 and 105 meV. Interestingly, the peak around 70 meV shifts significantly towards lower energy with increasing temperature, while the other peaks do not exhibit an appreciable change. The phonon spectra at 783 K show prominent change and become more diffusive as compared to those at 303 K. In order to better analyze these features, we have performed first principles lattice dynamics calculations based on the density functional theory. The computed phonon density of states is found to be in good agreement with the experimental data. Based on our calculation we are able to assign the characteristic Raman modes in the antiferroelectric phase to the A1g symmetry, which are due to the folding of the T (w=95 cm-1) and delta(w=129 cm-1) points of the cubic Brillouin zone.
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