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Register a new userHigh-accuracy optical clock based on the octupole transition in 171Yb+
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We experimentally investigate an optical frequency standard based on the 467 nm (642 THz) electric-octupole reference transition 2S1/2(F=0) -> F7/2(F=3) in a single trapped 171Yb+ ion. The extraordinary features of this transition result from the long natural lifetime and from the 4f136s2 configuration of the upper state. The electric quadrupole moment of the 2F7/2 state is measured as -0.041(5) e(a0)^2, where e is the elementary charge and a0 the Bohr radius. We also obtain information on the differential scalar and tensorial components of the static polarizability and of the probe light induced ac Stark shift of the octupole transition. With a real-time extrapolation scheme that eliminates this shift, the unperturbed transition frequency is realized with a fractional uncertainty of 7.1x10^(-17). The frequency is measured as 642 121 496 772 645.15(52) Hz.
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Despite being a canonical example of quantum mechanical perturbation theory, as well as one of the earliest observed spectroscopic shifts, the Stark effect contributes the largest source of uncertainty in a modern optical atomic clock through blackbody radiation. By employing an ultracold, trapped atomic ensemble and high stability optical clock, we characterize the quadratic Stark effect with unprecedented precision. We report the ytterbium optical clocks sensitivity to electric fields (such as blackbody radiation) as the differential static polarizability of the ground and excited clock levels: 36.2612(7) kHz (kV/cm)^{-2}. The clocks fractional uncertainty due to room temperature blackbody radiation is reduced an order of magnitude to 3 times 10^{-17}.
Time scales consistently provide precise time stamps and time intervals by combining atomic frequency standards with a reliable local oscillator. Optical frequency standards, however, have not been applied to the generation of time scales, although they provide superb accuracy and stability these days. Here, by steering an oscillator frequency based on the intermittent operation of a $^{87}$Sr optical lattice clock, we realized an optically steered time scale TA(Sr) that was continuously generated for half a year. The resultant time scale was as stable as International Atomic Time (TAI) with its accuracy at the $10^{-16}$ level. We also compared the time scale with TT(BIPM16). TT(BIPM) is computed in deferred time each January based on a weighted average of the evaluations of the frequency of TAI using primary and secondary frequency standards. The variation of the time difference TA(Sr) $-$ TT(BIPM16) was 0.79 ns after 5 months, suggesting the compatibility of using optical clocks for time scale generation. The steady signal also demonstrated the capability to evaluate one-month mean scale intervals of TAI over all six months with comparable uncertainties to those of primary frequency standards (PFSs).
We evaluated the static and dynamic polarizabilities of the 5s^2 ^1S_0 and 5s5p ^3P_0^o states of Sr using the high-precision relativistic configuration interaction + all-order method. Our calculation explains the discrepancy between the recent experimental 5s^2 ^1S_0 - 5s5p ^3P_0^o dc Stark shift measurement Delta alpha = 247.374(7) a.u. [Middelmann et. al, arXiv:1208.2848 (2012)] and the earlier theoretical result of 261(4) a.u. [Porsev and Derevianko, Phys. Rev. A 74, 020502R (2006)]. Our present value of 247.5 a.u. is in excellent agreement with the experimental result. We also evaluated the dynamic correction to the BBR shift with 1 % uncertainty; -0.1492(16) Hz. The dynamic correction to the BBR shift is unusually large in the case of Sr (7 %) and it enters significantly into the uncertainty budget of the Sr optical lattice clock. We suggest future experiments that could further reduce the present uncertainties.
The ESA mission Space Optical Clock project aims at operating an optical lattice clock on the ISS in approximately 2023. The scientific goals of the mission are to perform tests of fundamental physics, to enable space-assisted relativistic geodesy and to intercompare optical clocks on the ground using microwave and optical links. The performance goal of the space clock is less than $1 times 10^{-17}$ uncertainty and $1 times 10^{-15} {tau}^{-1/2}$ instability. Within an EU-FP7-funded project, a strontium optical lattice clock demonstrator has been developed. Goal performances are instability below $1 times 10^{-15} {tau}^{-1/2}$ and fractional inaccuracy $5 times 10^{-17}$. For the design of the clock, techniques and approaches suitable for later space application are used, such as modular design, diode lasers, low power consumption subunits, and compact dimensions. The Sr clock apparatus is fully operational, and the clock transition in $^{88}$Sr was observed with linewidth as small as 9 Hz.
Optical frequency comparison of the 40Ca+ clock transition u_{Ca} (2S1/2-2D5/2, 729nm) against the 87Sr optical lattice clock transition u_{Sr}(1S0-3P0, 698nm) has resulted in a frequency ratio u_{Ca} / u_{Sr} = 0.957 631 202 358 049 9(2 3). The rapid nature of optical comparison allowed the statistical uncertainty of frequency ratio u_{Ca} / u_{Sr} to reach 1x10-15 in only 1000s and yielded a value consistent with that calculated from separate absolute frequency measurements of u_{Ca} using the International Atomic Time (TAI) link. The total uncertainty of the frequency ratio using optical comparison (free from microwave link uncertainties) is smaller than that obtained using absolute frequency measurement, demonstrating the advantage of optical frequency evaluation. We report the absolute frequency of ^{40}Ca+ with a systematic uncertainty 14 times smaller than our previous measurement [1].
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