Optical interferometry is amongst the most sensitive techniques for precision measurement. By increasing the light intensity a more precise measurement can usually be made. However, in some applications the sample is light sensitive. By using entangled states of light the same precision can be achieved with less exposure of the sample. This concept has been demonstrated in measurements of fixed, known optical components. Here we use two-photon entangled states to measure the concentration of the blood protein bovine serum albumin (BSA) in an aqueous buffer solution. We use an opto-fluidic device that couples a waveguide interferometer with a microfluidic channel. These results point the way to practical applications of quantum metrology to light sensitive samples.
Plasmonics and metamaterials have recently been shown to allow the control and interaction with non-classical states of light, a rather counterintuitive finding given the high losses typically encountered in these systems. Here, we demonstrate a range of functionalities that are allowed with correlated and entangled photons that are used to illuminate multiple, overlaid patterns on plasmonic metasurfaces. Correlated photons allow to nonlocally determine the pattern that is imaged or, alternatively to un-scramble an image that is otherwise blurred. Entangled photons allow a more important functionality whereby the images imprinted on the metasurface are individually visible only when illuminated with one of the entangled photons. Correlated single photon imaging of functional metasurfaces could therefore promise advances towards the use of nanostructured subwavelength thin devices in quantum information protocols.
With the growing availability of experimental loophole-free Bell tests, it has become possible to implement a new class of device-independent random number generators whose output can be certified to be uniformly random without requiring a detailed model of the quantum devices used. However, all of these experiments require many input bits in order to certify a small number of output bits, and it is an outstanding challenge to develop a system that generates more randomness than is used. Here, we devise a device-independent spot-checking protocol which uses only uniform bits as input. Implemented with a photonic loophole-free Bell test, we can produce 24% more certified output bits (1,181,264,237) than consumed input bits (953,301,640), which is 5 orders of magnitude more efficient than our previous work [arXiv:1812.07786]. The experiment ran for 91.0 hours, creating randomness at an average rate of 3606 bits/s with a soundness error bounded by $5.7times 10^{-7}$ in the presence of classical side information. Our system will allow for greater trust in public sources of randomness, such as randomness beacons, and the protocols may one day enable high-quality sources of private randomness as the device footprint shrinks.
Distributed quantum metrology can enhance the sensitivity for sensing spatially distributed parameters beyond the classical limits. Here we demonstrate distributed quantum phase estimation with discrete variables to achieve Heisenberg limit phase measurements. Based on parallel entanglement in modes and particles, we demonstrate distributed quantum sensing for both individual phase shifts and an averaged phase shift, with an error reduction up to 1.4 dB and 2.7 dB below the shot-noise limit. Furthermore, we demonstrate a combined strategy with parallel mode entanglement and multiple passes of the phase shifter in each mode. In particular, our experiment uses six entangled photons with each photon passing the phase shifter up to six times, and achieves a total number of photon passes N=21 at an error reduction up to 4.7 dB below the shot-noise limit. Our research provides a faithful verification of the benefit of entanglement and coherence for distributed quantum sensing in general quantum networks.
Quantum entangled photons provide a sensitive probe of many-body interactions and offer an unique experimental portal for quantifying many-body correlations in a material system. In this paper, we present a theoretical demonstration of how photon-photon entanglement can be generated via interactions between coupled qubits. Here we develop a model for the scattering of an entangled pair of photons from a molecular dimer. We develop a diagrammatic theory for the scattering matrix and show that one can correlate the von Neumann entropy of the outgoing bi-photon wave function to exciton exchange and repulsion interactions. We conclude by discussing possible experimental scenarios for realizing these ideas.
Many quantum advantages in metrology and communication arise from interferometric phenomena. Such phenomena can occur on ultrafast time scales, particularly when energy-time entangled photons are employed. These have been relatively unexplored as their observation necessitates time resolution much shorter than conventional photon counters. Integrating nonlinear optical gating with conventional photon counters can overcome this limitation and enable subpicosecond time resolution. Here, using this technique and a Franson interferometer, we demonstrate high-visibility quantum interference with two entangled photons, where the one- and two-photon coherence times are both subpicosecond. We directly observe the spectral and temporal interference patterns, measure a visibility in the two-photon coincidence rate of $(85.3pm0.4)%$, and report a CHSH-Bell parameter of $2.42pm0.02$, violating the local-hidden variable bound by 21 standard deviations. The demonstration of energy-time entanglement with ultrafast interferometry provides opportunities for examining and exploiting entanglement in previously inaccessible regimes.