(Abridged) Differential astrometry measurements from the Palomar High-precision Astrometric Search for Exoplanet Systems (PHASES) are used to constrain the astrometric orbit of the previously known lesssim 2 day subsystem in the triple system 63 Gem A and have detected a previously unknown 2 year Keplerian wobble superimposed on the visual orbit of the much longer period (213 years) binary system HR 2896. The very small astrometric perturbation caused by the inner pair in 63 Gem A stretches the limits of current astrometric capabilities, but PHASES observations are able to constrain the orientation of the orbit. The two bright stars comprising the HR 2896 long period (213 year) system have a combined spectral type of K0III and the newly detected objects mass estimate places it in the regime of being a M dwarf. The motion of the stars are slow enough that their spectral features are always blended, preventing Doppler studies. The PHASES measurements and radial velocities (when available) have been combined with lower precision single-aperture measurements covering a much longer timeframe to improve the characterization of the long period orbits in both binaries. The visual orbits of the short and long period systems are presented for both systems, and used to calculate two possible values of the mutual inclinations between inner and outer orbits of 152 pm 12 degrees or a less likely value of 31 pm 11 degrees for 63 Gem A and 10.2 pm 2.4 degrees or 171.2 pm 2.8 degrees for HR 2896. The first is not coplanar, whereas the second is either nearly coplanar or anti-coplanar.
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