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Register a new userEngineering of Low-Loss Metal for Nanoplasmonic and Metamaterials Applications
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We have shown that alloying a noble metal (gold) with another metal (cadmium), which can contribute two electrons per atom to a free electron gas, can significantly improve the metals optical properties in certain wavelength ranges and make them worse in the other parts of the spectrum. In particular, in the gold-cadmium alloy we have demonstrated a significant expansion of the spectral range of metallic reflectance to shorter wavelengths. The experimental results and the predictions of the first principles theory demonstrate an opportunity for the improvement and optimization of low-loss metals for nanoplasmonic and metamaterials applications.
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Plasmonics allows manipulating light at the nanoscale, but has limitations due to the static nature of nanostructures and lack of tuneability. We propose and theoretically analyse a room-temperature liquid-metal nanodroplet that changes its shape, and therefore tunes the plasmon resonance frequency, due to capillary oscillations. We show the possibility to tune the capillary oscillation frequency of the nanodroplet and to drive the oscillations electrically or mechanically. Employed as a tuneable nanoantenna, the nanodroplet may find applications in sensors, imaging, microscopy, and medicine.
Nanostructured plasmonic metal systems are known to enhance greatly variety of radiative and nonradiative optical processes, both linear and nonlinear, which are due to the interaction of an electron in a molecule or semiconductor with the enhanced local optical field of the surface plasmons. Principally different are numerous many-body phenomena that are due to the Coulomb interaction between charged particles: carriers (electrons and holes) and ions. These include carrier-carrier or carrier-ion scattering, energy and momentum transfer (including the drag effect), thermal equilibration, exciton formation, impact ionization, Auger effects, etc. It is not widely recognized that these and other many-body effects can also be modified and enhanced by the surface-plasmon local fields. A special but extremely important class of such many-body phenomena is constituted by chemical reactions at metal surfaces, including catalytic reactions. Here, we propose a general and powerful theory of the plasmonic enhancement of the many-body phenomena resulting in a closed expression for the surface plasmon-dressed Coulomb interaction. We illustrate this theory by computing this dressed interaction explicitly for an important example of metal-dielectric nanoshells, which exhibits a reach resonant behavior in both the magnitude and phase. This interaction is used to describe the nanoplasmonic-enhanced Foerster energy transfer between nanocrystal quantum dots in the proximity of a plasmonic nanoshell. Catalysis at nanostructured metal surfaces, nonlocal carrier scattering and surface-enhanced Raman scattering are discussed among other effects and applications where the nanoplasmonic renormalization of the Coulomb interaction may be of principal importance.
All-dielectric nanoantennas have recently opened exciting opportunities for functional nanophotonics, owing to their strong optical resonances along with low material loss in the near-infrared range. Pushing these concepts to the visible range is hindered by a larger absorption coefficient of Si and other high-index semiconductors, thus encouraging the search for alternative dielectrics for nanophotonics. In this paper, we employ bandgap engineering to synthesize hydrogenated amorphous Si nanoparticles (a-Si:H NPs) offering ideal features for functional nanophotonics. We observe significant material loss suppression in a-Si:H NPs in the visible range caused by hydrogenation-induced bandgap renormalization, producing resonant modes in single a-Si:H NPs with Q factors up to ~100, in the visible and near-IR range for the first time. In order to demonstrate light-matter interaction enhancement, we realize highly tunable all-dielectric nanoantennas coupling them to photochromic spiropyran (SP) molecules. We show ~70% reversible all-optical tuning of light scattering at the high-Q resonant mode, along with minor tunability when out of resonance. This remarkable all-optical tuning effect is achieved under a low incident light intensity ~3.8 W/cm2 for UV light and ~1.1*10^2 W/cm2 for green light.
Engineering strong p-wave interactions between fermions is one of the challenges in modern quantum physics. Such interactions are responsible for a plethora of fascinating quantum phenomena such as topological quantum liquids and exotic superconductors. In this letter we propose to combine recent developments of nanoplasmonics with the progress in realizing laser-induced gauge fields. Nanoplasmonics allows for strong confinement leading to a geometric resonance in the atom-atom scattering. In combination with the laser-coupling of the atomic states, this is shown to result in the desired interaction. We illustrate how this scheme can be used for the stabilization of strongly correlated fractional quantum Hall states in ultracold fermionic gases.
We demonstrate theoretically that electromagnetically induced transparency can be achieved in metamaterials, in which electromagnetic radiation is interacting resonantly with mesoscopic oscillators rather than with atoms. We describe novel metamaterial designs that can support full dark resonant state upon interaction with an electromagnetic beam and we present results of its frequency-dependent effective permeability and permittivity. These results, showing a transparency window with extremely low absorption and strong dispersion, are confirmed by accurate simulations of the electromagnetic field propagation in the metamaterial.
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