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Register a new userSpin multiplicity and entanglement swapping in radical ion recombinations
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We address the problem of relative frequencies of singlet and triplet recombinations in a multiparticle system, which consists of spin-correlated radical ion pairs. The nonlocal swapping of spin correlations due to cross-recombinations is taken into account. It is shown that this swapping does not contribute to singlet and triplet recombination frequencies in the absence of spin evolution in the correlated pairs.
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The so-called phenomenological kinetic equation for one-pair density operator for spin-selective reactions is defended. We derive this equation from the kinetic equation for density operator of all pairs which are treated as singlet and triplet bosons. There presented some reasons for inconsistency of measurement-like approach to the problem.
We show that the stochastic Schrodinger equation (SSE) provides an ideal way to simulate the quantum mechanical spin dynamics of radical pairs. Electron spin relaxation effects arising from fluctuations in the spin Hamiltonian are straightforward to include in this approach, and their treatment can be combined with a highly efficient stochastic evaluation of the trace over nuclear spin states that is required to compute experimental observables. These features are illustrated in example applications to a flavin-tryptophan radical pair of interest in avian magnetoreception, and to a problem involving spin-selective radical pair recombination along a molecular wire. In the first of these examples, the SSE is shown to be both more efficient and more widely applicable than a recent stochastic implementation of the Lindblad equation, which only provides a valid treatment of relaxation in the extreme-narrowing limit. In the second, the exact SSE results are used to assess the accuracy of a recently-proposed combination of Nakajima-Zwanzig theory for the spin relaxation and Schulten-Wolynes theory for the spin dynamics, which is applicable to radical pairs with many more nuclear spins. An appendix analyses the efficiency of trace sampling in some detail, highlighting the particular advantages of sampling with SU(N) coherent states.
A 2015 experiment by Hanson and Delft colleagues provided further confirmation that the quantum world violates the Bell inequalities, being the first Bell test to close two known experimental loopholes simultaneously. The experiment was also taken to provide new evidence of spooky action at a distance. Here we argue for caution about the latter claim. The Delft experiment relies on entanglement swapping, and our main claim is that this geometry introduces an additional loophole in the argument from violation of the Bell inequalities to action at a distance: the apparent action at a distance may be an artifact of collider bias. In the absence of retrocausality, the sensitivity of such experiments to this Collider Loophole (CL) depends on the temporal relation between the entanglement swapping measurement C and the two measurements A and B between which we seek to infer a causal connection. CL looms large if the C is in the future of A and B, but not if C is in the past. The Delft experiment itself is the intermediate case, in which the separation is spacelike. We argue that this leaves it vulnerable to CL, unable to establish conclusively that it avoids it. An Appendix discusses the implications of permitting retrocausality for the issue of causal influence across entanglement swapping measurements.
We report an experimental demonstration of entanglement swapping over two quantum stages. By successful realizations of two cascaded photonic entanglement swapping processes, entanglement is generated and distributed between two photons, that originate from independent sources and do not share any common past. In the experiment we use three pairs of polarization entangled photons and conduct two Bell-state measurements (BSMs) one between the first and second pair, and one between the second and third pair. This results in projecting the remaining two outgoing photons from pair 1 and 3 into an entangled state, as characterized by an entanglement witness. The experiment represents an important step towards a full quantum repeater where multiple entanglement swapping is a key ingredient.
We show that braiding transformation is a natural approach to describe quantum entanglement, by using the unitary braiding operators to realize entanglement swapping and generate the GHZ states as well as the linear cluster states. A Hamiltonian is constructed from the unitary $check{R}_{i,i+1}(theta,phi)$-matrix, where $phi=omega t$ is time-dependent while $theta$ is time-independent. This in turn allows us to investigate the Berry phase in the entanglement space.
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