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Register a new userMagnetic order in CaFe1-xCoxAsF (x = 0, 0.06, 0.12) superconductor compounds
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A Neutron Powder Diffraction (NPD) experiment has been performed to investigate the structural phase transition and magnetic order in CaFe1-xCoxAsF superconductor compounds (x = 0, 0.06, 0.12). The parent compound CaFeAsF undergoes a tetragonal to orthorhombic phase transition at 134(3) K, while the magnetic order in form of a spin-density wave (SDW) sets in at 114(3) K. The antiferromagnetic structure of the parent compound has been determined with a unique propagation vector k = (1,0,1) and the Fe saturation moment of 0.49(5)uB aligned along the long a-axis. With increasing Co doping, the long range antiferromagnetic order has been observed to coexist with superconductivity in the orthorhombic phase of the underdoped CaFe0.94Co0.06AsF with a reduced Fe moment (0.15(5)uB). Magnetic order is completely suppressed in optimally doped CaFe0.88Co0.12AsF. We argue that the coexistence of SDW and superconductivity might be related to mesoscopic phase separation.
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We report an extensive study on the intrinsic bulk electronic structure of the high-temperature superconductor CeFeAsO0.89F0.11 and its parent compound CeFeAsO by soft and hard x-ray photoemission, x-ray absorption and soft-x-ray emission spectroscopies. The complementary surface/bulk probing depth, and the elemental and chemical sensitivity of these techniques allows resolving the intrinsic electronic structure of each element and correlating it with the local structure, which has been probed by extended-x-ray absorption fine structure spectroscopy. The measurements indicate a predominant 4f1 (i.e. Ce3+) initial state configuration for Cerium and an effective valence-band-to-4f charge-transfer screening of the core hole. The spectra also reveal the presence of a small Ce f0 initial state configuration, which we assign to the occurrence of an intermediate valence state. The data reveal a reasonably good agreement with the partial density of states as obtained in standard density functional calculations over a large energy range. Implications for the electronic structure of these materials are discussed.
We present a volume-sensitive high-energy x-ray diffraction study of the underdoped cuprate high temperature superconductor La2-xSrxCuO4 (x = 0.12, Tc=27 K) in applied magnetic field. Bulk short-range charge stripe order with propagation vector q_ch = (0.231, 0, 0.5) is demonstrated to exist below T_ch = 85(10) K and shown to compete with superconductivity. We argue that bulk charge ordering arises from fluctuating stripes that become pinned near boundaries between orthorhombic twin domains.
Polycrystalline NdFeAsO0.88F0.12 superconductors prepared by high pressure (HP) and ambient pressure (AP) method were comparatively studied by magnetization and transport measurements. Upper critical field (Hc2), irreversibility field (Hirr) and the anisotropy parameter were estimated from resistance transition curves. The broadening of transition width was observed, and ascribed to both Hc2 anisotropy and superconductivity inhomogeneity of samples. Magnetic hysteresis loops (MHLs) in low fields were measured to detect the trace of weak-link behavior. The reclosed hysteresis loops in low fields manifest that there are weak-links in both samples. Magnetization critical current density Jcm were derived from MHLs. High-pressure synthesized sample shows higher Jcm. However, by means of direct transport I-V measurements, transport critical current density Jct was very low. The Jct values for two samples are comparable. Large discrepancies between Jcm and Jct also indicate that there are weak-links in both samples. The relative mechanism is discussed in detail.
Charge order has now been observed in several cuprate high-temperature superconductors. We report a resonant inelastic x-ray scattering experiment on the electron-doped cuprate Nd$_{2-x}$Ce$_{x}$CuO$_4$ that demonstrates the existence of dynamic correlations at the charge order wave vector. Upon cooling we observe a softening in the electronic response, which has been predicted to occur for a d-wave charge order in electron-doped cuprates. At low temperatures, the energy range of these excitations coincides with that of the dispersive magnetic modes known as paramagnons. Furthermore, measurements where the polarization of the scattered photon is resolved indicate that the dynamic response at the charge order wave vector primarily involves spin-flip excitations. Overall, our findings indicate a coupling between dynamic magnetic and charge-order correlations in the cuprates.
Polarized beam neutron scattering measurements on a highly perfect crystal of ${rm YBa_2Cu_3O_{6.6}}$ show a distinct magnetic transition with an onset at about 235K, the temperature expected for the pseudogap transition. The moment is found to be about 0.1 $mu_B$ for each sublattice and have a correlation length of at least 75 AA. We found the critical exponent for the magnetic neutron intensity to be 2$beta$ =0.37$pm$ 0.12. This is the proper range for the class of transition that has no specific heat divergence possibly explaining why none is found at the pseudogap transition.
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