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Observation of vortices and hidden pseudogap from scanning tunneling spectroscopic studies of electron-doped cuprate superconductor $Sr_{0.9}La_{0.1}CuO_2$

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 Added by Nai-Chang Yeh
 Publication date 2008
  fields Physics
and research's language is English




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We present the first demonstration of vortices in an electron-type cuprate superconductor, the highest $T_c$ (= 43 K) electron-type cuprate $Sr_{0.9}La_{0.1}CuO_2$. Our spatially resolved quasiparticle tunneling spectra reveal a hidden low-energy pseudogap inside the vortex core and unconventional spectral evolution with temperature and magnetic field. These results cannot be easily explained by the scenario of pure superconductivity in the ground state of high-$T_c$ superconductivity.

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Quasiparticle tunneling spectra of both hole-doped (p-type) and electron-doped (n-type) cuprates are studied using a low-temperature scanning tunneling microscope. The results reveal that neither the pairing symmetry nor the pseudogap phenomenon is universal among all cuprates, and that the response of n-type cuprates to quantum impurities is drastically different from that of the p-type cuprates. The only ubiquitous features among all cuprates appear to be the strong electronic correlation and the nearest-neighbor antiferromagnetic Cu^{2+}-Cu^{2+} coupling in the CuO_2 planes.
The elucidation of the pseudogap phenomenon of the cuprates, a set of anomalous physical properties below the characteristic temperature T* and above the superconducting transition temperature Tc, has been a major challenge in condensed matter physics for the past two decades. Following initial indications of broken time-reversal symmetry in photoemission experiments, recent polarized neutron diffraction work demonstrated the universal existence of an unusual magnetic order below T*. These findings have the profound implication that the pseudogap regime constitutes a genuine new phase of matter rather than a mere crossover phenomenon. They are furthermore consistent with a particular type of order involving circulating orbital currents, and with the notion that the phase diagram is controlled by a quantum critical point. Here we report inelastic neutron scattering results for HgBa2CuO4+x (Hg1201) that reveal a fundamental collective magnetic mode associated with the unusual order, and that further support this picture. The modes intensity rises below the same temperature T* and its dispersion is weak, as expected for an Ising-like order parameter. Its energy of 52-56 meV and its enormous integrated spectral weight render it a new candidate for the hitherto unexplained ubiquitous electron-boson coupling features observed in spectroscopic studies.
The microscopic details of flux line lattice state studied by muon spin rotation is reported in an electron-doped high-$T_{rm c}$ cuprate superconductor, Sr$_{1-x}$La$_{x}$CuO$_{2}$ (SLCO, $x=0.10$--0.15). A clear sign of phase separation between magnetic and non-magnetic phases is observed, where the effective magnetic penetration depth [$lambdaequivlambda(T,H)$] is determined selectively for the latter phase. The extremely small value of $lambda(0,0)$ %versus $T_{rm c}$ and corresponding large superfluid density ($n_s propto lambda^{-2}$) is consistent with presence of a large Fermi surface with carrier density of $1+x$, which suggests the breakdown of the doped Mott insulator even at the optimal doping in SLCO. Moreover, a relatively weak anisotropy in the superconducting order parameter is suggested by the field dependence of $lambda(0,H)$. These observations strongly suggest that the superconductivity in SLCO is of a different class from hole-doped cuprates.
Magneto-optical imaging was used to study the local magnetization in polycrystalline NdFeAsO$_{0.9}$F$_{0.1}$ (NFAOF). Individual crystallites up to $sim200times100times30$ $mu m^{3}$ in size could be mapped at various temperatures. The in-grain, persistent current density is about $jsim10^{5}$ A/cm$^{2}$ and the magnetic relaxation rate in a remanent state peaks at about $T_{m}sim38$ K. By comparison with with the total magnetization measured in a bar-shaped, dense, polycrystalline sample, we suggest that NdFeAsO$_{0.9}$F$_{0.1}$ is similar to a layered high-$T_{c}$, compound such as Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$ and exhibits a $3Dto2D$ crossover in the vortex structure. The 2D Ginzburg parameter is about $Gi^{2D}% simeq10^{-2}$ implying electromagnetic anisotropy as large as $epsilon sim1/30$. Below $T_{m}$, the static and dynamic behaviors are consistent with collective pinning and creep.
We performed scanning tunneling spectroscopic experiments on hole-doped NdBa$_2$Cu$_3$O$_{7-delta}$. The d$I$/d$V$ curves obtained at 4.2 K are asymmetric with clear peak-dip and hump structures. Energy derivatives of these curves show peaks at energies beyond the dip features. Highly precise full potential bandstructure calculations confirm a featureless electronic density of states in that energy region. Our results indicate that tunneling electrons couple to a collective mode in the CuO$_2$ plane.
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