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Register a new userEvolution of the N=50 shell gap energy towards $^{78}$Ni
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Atomic masses of the neutron-rich isotopes $^{76-80}$Zn, $^{78-83}$Ga, $^{80-85}Ge, $^{81-87}$As and $^{84-89}$Se have been measured with high precision using the Penning trap mass spectrometer JYFLTRAP at the IGISOL facility. The masses of $^{82,83}$Ga, $^{83-85}$Ge, $^{84-87}$As and $^{89}$Se were measured for the first time. These new data represent a major improvement in the knowledge of the masses in this neutron-rich region. Two-neutron separation energies provide evidence for the reduction of the N=50 shell gap energy towards germanium Z=32 and a subsequent increase at gallium (Z=31). The data are compared with a number of theoretical models. An indication of the persistent rigidity of the shell gap towards nickel (Z=28) is obtained.
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The evolution of the N=50 gap is analyzed as a function of the occupation of the proton f5/2 and p3/2 orbits. It is based on experimental atomic masses, using three different methods of one or two-neutron separation energies of ground or isomeric states. We show that the effect of correlations, which is maximized at Z=32 could be misleading with respect to the determination of the size of the shell gap, especially when using the method with two-neutron separation energies. From the methods that are the least perturbed by correlations, we estimate the N=50 spherical shell gap in 78Ni. Whether 78Ni would be a rigid spherical or deformed nucleus is discussed in comparison with other nuclei in which similar nucleon-nucleon forces are at play.
Excited levels were attributed to $^{81}_{31}$Ga$_{50}$ for the first time which were fed in the $beta$-decay of its mother nucleus $^{81}$Zn produced in the fission of $^{nat}$U using the ISOL technique. We show that the structure of this nucleus is consistent with that of the less exotic proton-deficient N=50 isotones within the assumption of strong proton Z=28 and neutron N=50 effective shell effects.
New levels were attributed to $^{81}_{31}$Ga$_{50}$ and $^{83}_{32}$Ge$_{51}$ which were fed by the $beta$-decay of their respective mother nuclei $^{81}_{30}$Zn$_{51}$ and $^{83}_{31}$Ga$_{52}$ produced by fission at the PARRNe ISOL set-up installed at the Tandem accelerator of the Institut de Physique Nucleaire, Orsay. We show that the low energy structure of $^{81}_{31}$Ga$_{50}$ and $^{83}_{32}$Ge$_{51}$ can easily be explained within the natural hypothesis of a strong energy gap at N=50 and a doubly-magic character for $^{78}$Ni.
$beta$-decay rates play a decisive role in understanding the nucleosynthesis of heavy elements and are governed by microscopic nuclear-structure information. A sudden shortening of the half-lives of Ni isotopes beyond $N=50$ was observed at the RIKEN-RIBF. This is considered due to the persistence of the neutron magic number $N=50$ in the very neutron-rich Ni isotopes. By systematically studying the $beta$-decay rates and strength distributions in the neutron-rich Ni isotopes around $N=50$, I try to understand the microscopic mechanism for the observed sudden shortening of the half-lives. The $beta$-strength distributions in the neutron-rich nuclei are described in the framework of nuclear density-functional theory. I employ the Skyrme energy-density functionals (EDF) in the Hartree-Fock-Bogoliubov calculation for the ground states and in the proton-neutron Quasiparticle Random-Phase Approximation (pnQRPA) for the transitions. Not only the allowed but the first-forbidden (FF) transitions are considered. The experimentally observed sudden shortening of the half-lives beyond $N=50$ is reproduced well by the calculations employing the Skyrme SkM* and SLy4 functionals. The sudden shortening of the half-lives is due to the shell gap at $N=50$ and cooperatively with the high-energy transitions to the low-lying $0^-$ and $1^-$ states in the daughter nuclei. The onset of FF transitions pointed out around $N=82$ and 126 is preserved in the lower-mass nuclei around $N=50$. This study suggests that needed is a microscopic calculation where the shell structure in neutron-rich nuclei and its associated effects on the FF transitions are selfconsistenly taken into account for predicting $beta$-decay rates of exotic nuclei in unknown region.
Nuclear spins and precise values of the magnetic dipole and electric quadrupole moments of the ground-states of neutron-rich $^{76-78}$Cu isotopes were measured using the Collinear Resonance Ionization Spectroscopy (CRIS) experiment at ISOLDE, CERN. The nuclear moments of the less exotic $^{73,75}$Cu isotopes were re-measured with similar precision, yielding values that are consistent with earlier measurements. The moments of the odd-odd isotopes, and $^{78}_{29}$Cu ($N=49$) in particular, are used to investigate excitations of the assumed doubly-magic $^{78}$Ni core through comparisons with large-scale shell-model calculations. Despite the narrowing of the $Z=28$ shell gap between $Nsim45$ and $N=50$, the magicity of $Z=28$ and $N=50$ is restored towards $^{78}$Ni. This is due to weakened dynamical correlations, as clearly probed by the present moment measurements.
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