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Enhancement of the Deuteron-Fusion Reactions in Metals and its Experimental Implications

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 Added by Armin Huke
 Publication date 2008
  fields
and research's language is English




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Recent measurements of the reaction d(d,p)t in metallic environments at very low energies performed by different experimental groups point to an enhanced electron screening effect. However, the resulting screening energies differ strongly for divers host metals and different experiments. Here, we present new experimental results and investigations of interfering processes in the irradiated targets. These measurements inside metals set special challenges and pitfalls which make them and the data analysis particularly error-prone. There are multi-parameter collateral effects which are crucial for the correct interpretation of the observed experimental yields. They mainly originate from target surface contaminations due to residual gases in the vacuum as well as from inhomogeneities and instabilities in the deuteron density distribution in the targets. In order to address these problems an improved differential analysis method beyond the standard procedures has been implemented. Profound scrutiny of the other experiments demonstrates that the observed unusual changes in the reaction yields are mainly due to deuteron density dynamics simulating the alleged screening energy values. The experimental results are compared with different theoretical models of the electron screening in metals. The Debye-H{u}ckel model that has been previously proposed to explain the influence of the electron screening on both nuclear reactions and radioactive decays could be clearly excluded.



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Background: The cross section for forming a heavy evaporation residue in fusion reactions depends on the capture cross section, the fusion probability, PCN, i.e., the probability that the projectile-target system will evolve inside the fission saddle point to form a completely fused system rather than re-separating (quasifission), and the survival of the completely fused system against fission. PCN is the least known of these quantities. Purpose: To measure PCN for the reaction of 101.2 MeV 18O, 147.3 MeV 26Mg, 170.9 MeV 30Si and 195.3 MeV 36S with 197Au. Methods: We measured the fission fragment angular distributions for these reactions and used the formalism of Back to deduce the fusion-fission and quasifission cross sections. From these quantities we deduced PCN for each reaction. Results: The values of PCN for the reaction of 101.2 MeV 18O, 147.3 MeV 26Mg, 170.9 MeV 30Si and 195.3 MeV 36S with 197Au are 0.66, 1.00, 0.06, 0.13, respectively. Conclusions: The new measured values of PCN agree roughly with the semi-empirical system- atic dependence of PCN upon fissility for excited nuclei.
130 - M. Debowski 1997
Double differential cross sections have been measured for pi+ and K+ emitted around midraidity in d+A and He+A collisions at a beam kinetic energy of 1.15 GeV/nucleon. The total pi+ yield increases by a factor of about 2 when using an alpha projectile instead of a deuteron whereas the K+ yield increases by a factor of about 4. According to transport calculations, the K+ enhancement depends both on the number of hadron-hadron collisions and on the energy available in those collisions: their center-of-mass energy increases with increasing number of projectile nucleons.
The prompt gamma ray emission was investigated in the 16A MeV energy region by means of the 36,40Ar+96,92Zr fusion reactions leading to a compound nucleus in the vicinity of 132Ce. We show that the prompt radiation, which appears to be still effective at such a high beam energy, has an angular distribution pattern consistent with a dipole oscillation along the symmetry axis of the dinuclear system. The data are compared with calculations based on a collective bremsstrahlung analysis of the reaction dynamics.
The extraction of detailed nuclear structure information from transfer reactions requires reliable, well-normalized data as well as optical potentials and a theoretical framework demonstrated to work well in the relevant mass and beam energy ranges. It is rare that the theoretical ingredients can be tested well for exotic nuclei owing to the paucity of data. The halo nucleus Be-11 has been examined through the 10Be(d,p) reaction in inverse kinematics at equivalent deuteron energies of 12,15,18, and 21.4 MeV. Elastic scattering of Be-10 on protons was used to select optical potentials for the analysis of the transfer data. Additionally, data from the elastic and inelastic scattering of Be-10 on deuterons was used to fit optical potentials at the four measured energies. Transfers to the two bound states and the first resonance in Be-11 were analyzed using the Finite Range ADiabatic Wave Approximation (FR-ADWA). Consistent values of the spectroscopic factor of both the ground and first excited states were extracted from the four measurements, with average values of 0.71(5) and 0.62(4) respectively. The calculations for transfer to the first resonance were found to be sensitive to the size of the energy bin used and therefore could not be used to extract a spectroscopic factor.
34 - A. Huke , K. Czerski , P. Heide 2007
The investigation of the d+d fusion reactions in metallic environments at sub-Coulomb energies demands especially adapted techniques beyond standard procedures in nuclear physics. The measurements which were performed with an electrostatic accelerator at different self-implanted metallic target materials show an enhancement of the reaction cross-section compared to the gas target experiments. The resulting electron screening energy values are about one order of magnitude larger relative to the gas target experiments and exceed significantly the theoretical predictions. The measurements on deuterium inside metals are heavily affected by the interference of two peculiarities of this system: the possibly very high mobility of deuterium in solids and the formation of surface contamination layers under ion beam irradiation in high vacuum systems. Thorough investigations of these processes show their crucial influence on the interpretation of the experimental raw data. The differential data acquisition and analysis method employed to it is outlined. Non observance of these problems by using standard procedures results in fatal errors for the extraction of the screening energies.
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