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Register a new userDecay dynamics of quantum dots influenced by the local density of optical states of two-dimensional photonic crystal membranes
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We have performed time-resolved spectroscopy on InAs quantum dot ensembles in photonic crystal membranes. The influence of the photonic crystal is investigated by varying the lattice constant systematically. We observe a strong slow down of the quantum dots spontaneous emission rates as the two-dimensional bandgap is tuned through their emission frequencies. The measured band edges are in full agreement with theoretical predictions. We characterize the multi-exponential decay curves by their mean decay time and find enhancement of the spontaneous emission at the bandgap edges and strong inhibition inside the bandgap in good agreement with local density of states calculations.
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In quantum dot (QD) electron transport experiments additional features can appear in the differential conductance $dI/dV$ that do not originate from discrete states in the QD, but rather from a modulation of the density-of-states (DOS) in the leads. These features are particularly pronounced when the leads are strongly confined low dimensional systems, such as in a nanowire (NW) where transport is one-dimensional and quasi-zero dimensional lead-states can emerge. In this paper we study such lead-states in InAs NWs. We use a QD integrated directly into the NW during the epitaxial growth as an energetically and spatially well-defined tunnel probe to perform $dI/dV$ spectroscopy of discrete bound states in the `left and `right NW lead segments. By tuning a sidegate in close proximity of one lead segment, we can distinguish transport features related to the modulation in the lead DOS and to excited states in the QD. We implement a non-interacting capacitance model and derive expressions for the slopes of QD and lead resonances that appear in two-dimensional plots of $dI/dV$ as a function of source-drain bias and gate voltage in terms of the different lever arms determined by the capacitive couplings. We discuss how the interplay between the lever arms affect the slopes. We verify our model by numerically calculating the $dI/dV$ using a resonant tunneling model with three non-interacting quantum dots in series. Finally, we used the model to describe the measured $dI/dV$ spectra and extract quantitatively the tunnel couplings of the lead segments. Our results constitute an important step towards a quantitative understanding of normal and superconducting subgap states in hybrid NW devices.
This thesis describes capacitance and tunneling experiments performed on two-dimensional electron gas (2DEG) and quantum dot systems. It develops a system of equations that allow determination, by means of capacitance measurements, of the electronic density of states, the electron density, and the chemical potential in a 2DEG. The thesis describes the use of these techniques in the observation of a magnetic field induced energy gap to tunneling in the 2DEG and the single electron addition spectrum in arrays of quantum dots.
In quantum physics, two prototypical model systems stand out due to their wide range of applications. These are the two-level system (TLS) and the harmonic oscillator. The former is often an ideal model for confined charge or spin systems and the latter for lattice vibrations, i.e., phonons. Here, we couple these two systems, which leads to numerous fascinating physical phenomena. Practically, we consider different optical excitations and decay scenarios of a TLS, focusing on the generated dynamics of a single phonon mode that couples to the TLS. Special emphasis is placed on the entropy of the different parts of the system, predominantly the phonons. While, without any decay, the entire system is always in a pure state, resulting in a vanishing entropy, the complex interplay between the single parts results in non-vanishing respective entanglement entropies and non-trivial dynamics of them. Taking a decay of the TLS into account leads to a non-vanishing entropy of the full system and additional aspects in its dynamics. We demonstrate that all aspects of the entropys behavior can be traced back to the purity of the states and are illustrated by phonon Wigner functions in phase space.
Monolayers of transition metal dichalcogenides (TMDCs) have emerged as new optoelectronic materials in the two dimensional (2D) limit, exhibiting rich spin-valley interplays, tunable excitonic effects, and strong light-matter interactions. An essential yet undeveloped ingredient for many photonic applications is the manipulation of its light emission. Here we demonstrate the control of excitonic light emission from monolayer tungsten diselenide (WSe2) in an integrated photonic structure, achieved by transferring one monolayer onto a photonic crystal (PhC) with a cavity. In addition to the observation of greatly enhanced (~60 times) photoluminescence of WSe2 and an effectively coupled cavity-mode emission, we are able to redistribute the emitted photons both polarly and azimuthally in the far field through designing PhC structures, as revealed by momentum-resolved microscopy. A 2D optical antenna is thus constructed. Our work suggests a new way of manipulating photons in hybrid 2D photonics, important for future energy efficient optoelectronics and 2D nano-lasers.
Systems of photonic crystal cavities coupled to quantum dots are a promising architecture for quantum networking and quantum simulators. The ability to independently tune the frequencies of laterally separated quantum dots is a crucial component of such a scheme. Here, we demonstrate independent tuning of laterally separated quantum dots in photonic crystal cavities coupled by in-plane waveguides by implanting lines of protons which serve to electrically isolate different sections of a diode structure.
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