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Register a new userOn the long range correlations of thermodynamic systems out of equilibrium
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Experiments show that macroscopic systems in a stationary nonequilibrium state exhibit long range correlations of the local thermodynamic variables. In previous papers we proposed a Hamilton-Jacobi equation for the nonequilibrium free energy as a basic principle of nonequilibrium thermodynamics. We show here how an equation for the two point correlations can be derived from the Hamilton-Jacobi equation for arbitrary transport coefficients for dynamics with both external fields and boundary reservoirs. In contrast with fluctuating hydrodynamics, this approach can be used to derive equations for correlations of any order. Generically, the solutions of the equation for the correlation functions are non-trivial and show that long range correlations are indeed a common feature of nonequilibrium systems. Finally, we establish a criterion to determine whether the local thermodynamic variables are positively or negatively correlated in terms of properties of the transport coefficients.
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This paper provides an introduction to some stochastic models of lattice gases out of equilibrium and a discussion of results of various kinds obtained in recent years. Although these models are different in their microscopic features, a unified picture is emerging at the macroscopic level, applicable, in our view, to real phenomena where diffusion is the dominating physical mechanism. We rely mainly on an approach developed by the authors based on the study of dynamical large fluctuations in stationary states of open systems. The outcome of this approach is a theory connecting the non equilibrium thermodynamics to the transport coefficients via a variational principle. This leads ultimately to a functional derivative equation of Hamilton-Jacobi type for the non equilibrium free energy in which local thermodynamic variables are the independent arguments. In the first part of the paper we give a detailed introduction to the microscopic dynamics considered, while the second part, devoted to the macroscopic properties, illustrates many consequences of the Hamilton-Jacobi equation. In both parts several novelties are included.
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We study two dimensional stripe forming systems with competing repulsive interactions decaying as $r^{-alpha}$. We derive an effective Hamiltonian with a short range part and a generalized dipolar interaction which depends on the exponent $alpha$. An approximate map of this model to a known XY model with dipolar interactions allows us to conclude that, for $alpha <2$ long range orientational order of stripes can exist in two dimensions, and establish the universality class of the models. When $alpha geq 2$ no long-range order is possible, but a phase transition in the KT universality class is still present. These two different critical scenarios should be observed in experimentally relevant two dimensional systems like electronic liquids ($alpha=1$) and dipolar magnetic films ($alpha=3$). Results from Langevin simulations of Coulomb and dipolar systems give support to the theoretical results.
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