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`Stuckelberg interferometry with ultracold molecules

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 Publication date 2007
  fields Physics
and research's language is English




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We report on the realization of a time-domain `Stuckelberg interferometer, which is based on the internal state structure of ultracold Feshbach molecules. Two subsequent passages through a weak avoided crossing between two different orbital angular momentum states in combination with a variable hold time lead to high-contrast population oscillations. This allows for a precise determination of the energy difference between the two molecular states. We demonstrate a high degree of control over the interferometer dynamics. The interferometric scheme provides new possibilities for precision measurements with ultracold molecules.



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Stuckelberg interferometry describes the interference of two strongly coupled modes during a double passage through an avoided energy level crossing. In this work, we experimentally investigate finite time effects in Stuckelberg interference and provide an exact analytical solution of the Stuckelberg problem. Approximating this solution in distinct limits reveals uncharted parameter regimes of Stuckelberg interferometry. Experimentally, we study these regimes using a purely classical, strongly coupled nanomechanical two-mode system of high quality factor. The classical two-mode system consists of the in-plane and out-of-plane fundamental flexural mode of a high stress silicon nitride string resonator, coupled via electric gradient fields. The dielectric control and microwave cavity enhanced universal transduction of the nanoelectromechanical system allows for the experimental access to all theoretically predicted Stuckelberg parameter regimes. We exploit our experimental and theoretical findings by studying the onset of Stuckelberg interference in dependence of the characteristic system control parameters and obtain characteristic excitation oscillations between the two modes even without the explicit need of traversing the avoided crossing. The presented theory is not limited to classical mechanical two-mode systems but can be applied to every strongly coupled (quantum) two-level system, for example a spin-1/2 system or superconducting qubit.
We report on the first creation of ultracold bosonic heteronuclear molecules of two fermionic species, 6Li and 40K, by a magnetic field sweep across an interspecies s-wave Feshbach resonance. This allows us to associate up to 4x10^4 molecules with high efficiencies of up to 50%. Using direct imaging of the molecules, we measure increased lifetimes of the molecules close to resonance of more than 100 ms in the molecule-atom mixture stored in a harmonic trap.
We examine dark quantum superposition states of weakly bound Rb2 Feshbach molecules and tightly bound triplet Rb2 molecules in the rovibrational ground state, created by subjecting a pure sample of Feshbach molecules in an optical lattice to a bichromatic Raman laser field. We analyze both experimentally and theoretically the creation and dynamics of these dark states. Coherent wavepacket oscillations of deeply bound molecules in lattice sites, as observed in one of our previous experiments, are suppressed due to laser-induced phase locking of molecular levels. This can be understood as the appearance of a novel multilevel dark state. In addition, the experimental methods developed help to determine important properties of our coupled atom / laser system.
273 - B. Deh , C. Marzok , S. Slama 2008
We report on the observation of Bragg scattering of an ultracold Fermi gas of 6Li atoms at a dynamic optical potential. The momentum states produced in this way oscillate in the trap for time scales on the order of seconds, nearly unperturbed by collisions, which are absent for ultracold fermions due to the Pauli principle. In contrast, interactions in a mixture with 87Rb atoms lead to rapid damping. The coherence of these states is demonstrated by Ramsey-type matter wave interferometry. The signal is improved using an echo pulse sequence, allowing us to observe coherence times longer than 100 mus. Finally we use Bragg spectroscopy to measure the in-situ momentum distribution of the 6Li cloud. Signatures for the degeneracy of the Fermi gas can be observed directly from the momentum distribution of the atoms inside the trap.
111 - C. Marzok , B. Deh , S. Slama 2008
We report on the first observation of Bragg scattering of an ultracold $^6$Li Fermi gas. We demonstrate a Ramsey-type matter-wave interferometer based on Bragg diffraction and find robust signatures of persistent matter wave coherences using an echo pulse sequence. Because of the Pauli principle, the diffracted fermions oscillate nearly unperturbed in the trapping potential for long times beyond 2 s. This suggests extremely long coherence times. On these timescales, only the presence of a $^{87}$Rb cloud seems sufficient to induce noticeable perturbations.
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