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Register a new userCoupling Efficiencies in Single Photon On-Demand Sources
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Many quantum computation and communication schemes require, or would significantly benefit from, true sources of single photon on-demand (SPOD). Unfortunately, such sources do not exist. It is becoming increasingly clear that coupling photons out of a SPOD source will be a limiting factor in many SPOD implementations. In particular, coupling these source outputs into optical fibers (usually single mode fibers) is often the preferred method for handling this light. We investigate the practical limits to this coupling as relates to parametric downconversion, an important starting point for many SPOD schemes. We also explored whether it is possible to optimize the engineering of the downconversion sources to improve on this coupling. We present our latest results in this area.
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Spontaneous parametric down-conversion (SPDC) in a laser pumped optical nonlinear medium can produce heralded single photons with a high purity but a very low yield. Improving the yield by increasing the pump power in SPDC inevitably reduces the purity due to excitation of multi-photon events. We propose a scheme to overcome this purity-yield trade-off by suppressing multi-photon events in a cavity-enhanced SPDC via the photon blockade effect. By introducing a strong photon-photon interaction into the intracavity medium and increasing the pump power, we can improve the available single-photon yield to larger than $90%$, while maintaining a high purity of $99%$, towards on-demand generation of single photons through the SPDC process. Our quasi-on-demand SPDC sources may boost single-photon-based quantum information technology.
Photon pairs produced by parametric down-conversion or four-wave mixing can interfere with each other in multiport interferometers, or carry entanglement between distant nodes for use in entanglement swapping. This requires the photons be spectrally pure to ensure good interference, and have high heralding efficiency to know accurately the number of photons involved and to maintain high rates as the number of photons grows. Spectral filtering is often used to remove noise and define spectral properties. For heralded single photons high purity and heralding efficiency is possible by filtering the heralding arm, but when both photons in typical pair sources are filtered, we show that the heralding efficiency of one or both of the photons is strongly reduced even by ideal spectral filters with 100% transmission in the passband: any improvement in reduced-state spectral purity from filtering comes at the cost of lowered heralding efficiency. We consider the fidelity to a pure, lossless single photon, symmetrize it to include both photons of the pair, and show this quantity is intrinsically limited for sources with spectral correlation. We then provide a framework for this effect for benchmarking common photon pair sources, and present an experiment where we vary the photon filter bandwidths and measure the increase in purity and corresponding reduction in heralding efficiency.
Deterministic coupling between photonic nodes in a quantum network is an essential step towards implementing various quantum technologies. The omnidirectionality of free-standing emitters, however, makes this coupling highly inefficient, in particular if the distant nodes are coupled via low numerical aperture (NA) channels such as optical fibers. This limitation requires placing quantum emitters in nanoantennas that can direct the photons into the channels with very high efficiency. Moreover, to be able to scale such technologies to a large number of channels, the placing of the emitters should be deterministic. In this work we present a method for directly locating single free-standing quantum emitters with high spatial accuracy at the center of highly directional bullseye metal-dielectric nanoantennas. We further employ non-blinking, high quantum yield colloidal quantum dots (QDs) for on-demand single-photon emission that is uncompromised by instabilities or non-radiative exciton recombination processes. Taken together this approach results in a record-high collection efficiency of 85% of the single photons into a low NA of 0.5, setting the stage for efficient coupling between on-chip, room temperature nanoantenna-emitter devices and a fiber or a remote free-space node without the need for additional optics.
Quantum emitters coupled to plasmonic resonators are known to allow enhanced broadband Purcell factors, and such systems have been recently suggested as possible candidates for on-demand single photon sources, with fast operation speeds. However, a true single photon source has strict requirements of high efficiency (brightness) and quantum indistinguishability of the emitted photons, which can be quantified through two-photon interference experiments. To help address this problem, we employ and extend a recently developed quantized quasinormal mode approach, which rigorously quantizes arbitrarily lossy open system modes, to compute the key parameters that accurately quantify the figures of merit for plasmon-based single photon sources. We also present a quantized input-output theory to quantify the radiative and nonradiative quantum efficiencies. We exemplify the theory using a nanoplasmonic dimer resonator made up of two gold nanorods, which yields large Purcell factors and good radiative output beta factors. Considering an optically pulsed excitation scheme, we explore the key roles of pulse duration and pure dephasing on the single photon properties, and show that ultrashort pulses (sub-ps) are generally required for such structures, even for low temperature operation. We also quantify the role of the nonradiative beta factor both for single photon and two-photon emission processes. Our general approach can be applied to a wide variety of plasmon systems, including metal-dielectrics, and cavity-waveguide systems, without recourse to phenomenological quantization schemes.
A quantum dot coupled to an optical cavity has recently proven to be an excellent source of on-demand single photons. Typically, applications require simultaneous high efficiency of the source and quantum indistinguishability of the extracted photons. While much progress has been made both in suppressing background sources of decoherence and utilizing cavity-quantum electrodynamics to overcome fundamental limitations set by the intrinsic exciton-phonon scattering inherent in the solid-state platform, the role of the excitation pulse has been often neglected. We investigate quantitatively the factors associated with pulsed excitation that can limit simultaneous efficiency and indistinguishability, including excitation of multiple excitons, multi-photons, and pump-induced dephasing, and find for realistic single photon sources that these effects cause degradation of the source figures-of-merit comparable to that of phonon scattering. We also develop rigorous open quantum system polaron master equation models of quantum dot dynamics under a time-dependent drive which incorporate non-Markovian effects of both photon and phonon reservoirs, and explicitly show how coupling to a high Q-factor cavity suppresses multi-photon emission in a way not predicted by commonly employed models. We then use our findings to summarize the criteria that can be used for single photon source optimization.
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