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Hyperpolarizability effects in a Sr optical lattice clock

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 Added by Pierre Lemonde
 Publication date 2005
  fields Physics
and research's language is English
 Authors Anders Brusch




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We report the observation of the higher order frequency shift due to the trapping field in a $^{87}$Sr optical lattice clock. We show that at the magic wavelength of the lattice, where the first order term cancels, the higher order shift will not constitute a limitation to the fractional accuracy of the clock at a level of $10^{-18}$. This result is achieved by operating the clock at very high trapping intensity up to $400 $kW/cm$^2$ and by a specific study of the effect of the two two-photon transitions near the magic wavelength.



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Optical clocks benefit from tight atomic confinement enabling extended interrogation times as well as Doppler- and recoil-free operation. However, these benefits come at the cost of frequency shifts that, if not properly controlled, may degrade clock accuracy. Numerous theoretical studies have predicted optical lattice clock frequency shifts that scale nonlinearly with trap depth. To experimentally observe and constrain these shifts in an $^{171}$Yb optical lattice clock, we construct a lattice enhancement cavity that exaggerates the light shifts. We observe an atomic temperature that is proportional to the optical trap depth, fundamentally altering the scaling of trap-induced light shifts and simplifying their parametrization. We identify an operational magic wavelength where frequency shifts are insensitive to changes in trap depth. These measurements and scaling analysis constitute an essential systematic characterization for clock operation at the $10^{-18}$ level and beyond.
We describe the Sr optical lattice clock apparatus at NPL with particular emphasis on techniques used to increase reliability and minimise the human requirement in its operation. Central to this is a clock-referenced transfer cavity scheme for the stabilisation of cooling and trapping lasers. We highlight several measures to increase the reliability of the clock with a view towards the realisation of an optical time-scale. The clock contributed 502 hours of data over a 25 day period (84% uptime) in a recent measurement campaign with several uninterrupted periods of more than 48 hours. An instability of $2times10^{-17}$ was reached after $10^5$ s of averaging in an interleaved self-comparison of the clock.
Optical frequency comparison of the 40Ca+ clock transition u_{Ca} (2S1/2-2D5/2, 729nm) against the 87Sr optical lattice clock transition u_{Sr}(1S0-3P0, 698nm) has resulted in a frequency ratio u_{Ca} / u_{Sr} = 0.957 631 202 358 049 9(2 3). The rapid nature of optical comparison allowed the statistical uncertainty of frequency ratio u_{Ca} / u_{Sr} to reach 1x10-15 in only 1000s and yielded a value consistent with that calculated from separate absolute frequency measurements of u_{Ca} using the International Atomic Time (TAI) link. The total uncertainty of the frequency ratio using optical comparison (free from microwave link uncertainties) is smaller than that obtained using absolute frequency measurement, demonstrating the advantage of optical frequency evaluation. We report the absolute frequency of ^{40}Ca+ with a systematic uncertainty 14 times smaller than our previous measurement [1].
Optical atomic clocks promise timekeeping at the highest precision and accuracy, owing to their high operating frequencies. Rigorous evaluations of these clocks require direct comparisons between them. We have realized a high-performance remote comparison of optical clocks over km-scale urban distances, a key step for development, dissemination, and application of these optical standards. Through this remote comparison and a proper design of lattice-confined neutral atoms for clock operation, we evaluate the uncertainty of a strontium (Sr) optical lattice clock at the 1x10-16 fractional level, surpassing the best current evaluations of cesium (Cs) primary standards. We also report on the observation of density-dependent effects in the spin-polarized fermionic sample and discuss the current limiting effect of blackbody radiation-induced frequency shifts.
Existing optical lattice clocks demonstrate a high level of performance, but they remain complex experimental devices. In order to address a wider range of applications including those requiring transportable devices, it will be necessary to simplify the laser systems and reduce the amount of support hardware. Here we demonstrate two significant steps towards this goal: demonstration of clock signals from a Sr lattice clock based solely on semiconductor laser technology, and a method for finding the clock transition (based on a coincidence in atomic wavelengths) that removes the need for extensive frequency metrology hardware. Moreover, the unexpected high contrast in the signal revealed evidence of density dependent collisions in Sr-88 atoms.
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