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Register a new userPhotoassociation inside an optical dipole trap: absolute rate coefficients and Franck-Condon factors
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We present quantitative measurements of the photoassociation of cesium molecules inside a far-detuned optical dipole trap. A model of the trap depletion dynamics is derived which allows to extract absolute photoassociation rate coefficients for the initial single-photon photoassociation step from measured trap-loss spectra. The sensitivity of this approach is demonstrated by measuring the Franck-Condon modulation of the weak photoassociation transitions into the low vibrational levels of the outer well of the 0g- state that correlates to the 6s+6p3/2 asymptote. The measurements are compared to theoretical predictions. In a magneto-optical trap these transitions have previously only been observed indirectly through ionization of ground state molecules.
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We present studies of strong coupling in single-photon photoassociation of cesium dimers using an optical dipole trap. A thermodynamic model of the trap depletion dynamics is employed to extract absolute rate coefficents. From the dependence of the rate coefficient on the photoassociation laser intensity, we observe saturation of the photoassociation scattering probability at the unitarity limit in quantitative agreement with the theoretical model by Bohn and Julienne [Phys. Rev. A, 60, 414 (1999)]. Also the corresponding power broadening of the resonance width is measured. We could not observe an intensity dependent light shift in contrast to findings for lithium and rubidium, which is attributed to the absence of a p or d-wave shape resonance in cesium.
Laser induced electronic excitations that spontaneously emit photons and decay directly to the initial ground state (optical cycling transitions) are used in quantum information and precision measurement for state initialization and readout. To extend this primarily atomic technique to organic compounds, we theoretically investigate optical cycling of alkaline earth phenoxides and their functionalized derivatives. We find that optical cycle leakage due to wavefunction mismatch is low in these species, and can be further suppressed by using chemical substitution to boost the electron withdrawing strength of the aromatic molecular ligand through resonance and induction effects. This provides a straightforward way to use chemical functional groups to construct optical cycling moieties for laser cooling, state preparation, and quantum measurement.
In recent years, cold atoms could prove their scientific impact not only on ground but in microgravity environments such as the drop tower in Bremen, sounding rockets and parabolic flights. We investigate the preparation of cold atoms in an optical dipole trap, with an emphasis on evaporative cooling under microgravity. Up to $ 1times10^{6} $ rubidium-87 atoms were optically trapped from a temporarily dark magneto optical trap during free fall in the droptower in Bremen. The efficiency of evaporation is determined to be equal with and without the effect of gravity. This is confirmed using numerical simulations that prove the dimension of evaporation to be three-dimensional in both cases due to the anharmonicity of optical potentials. These findings pave the way towards various experiments on ultra-cold atoms under microgravity and support other existing experiments based on atom chips but with plans for additional optical dipole traps such as the upcoming follow-up missions to current and past spaceborne experiments.
Electronic states and vibrons in carbon nanotube quantum dots have in general different location and size. As a consequence, the conventional Anderson-Holstein model, coupling vibrons to the dot total charge only, may no longer be appropriated in general. Here we explicitly address the role of the spatial fluctuations of the electronic density, yielding space-dependent Franck-Condon factors. We discuss the consequent marked effects on transport which are compatible with recent measurements. This picture can be relevant for tunneling experiments in generic nano-electromechanical systems.
One important factor which determines efficiency of loading cold atoms into an optical dipole trap from a magneto-optical trap is the distance between the trap centers. By studying this efficiency for various optical trap depths (2--110 mK) we find that for optimum dipole trap loading, longitudinal displacements up to 15 mm are necessary. An explanation for this observation is presented and compared with other work and a simple analytical formula is derived for the optimum distance between the trap centers.
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