We report the direct frequency measurement of the visible 5s$^2$ $^1$S$_0$-5s 5p$^3$P$_1$ intercombination line of strontium that is considered a possible candidate for a future optical frequency standard. The frequency of a cavity-stabilized laser is locked to the saturated fluorescence in a thermal Sr atomic beam and is measured with an optical-frequency comb-generator referenced to the SI second through a GPS signal. The $^{88}$Sr transition is measured to be at 434 829 121 311 (10) kHz. We measure also the $^{88}$Sr-$^{86}$Sr isotope shift to be 163 817.4 (0.2) kHz.
We present a spectroscopy scheme for the 7-kHz-wide 689-nm intercombination line of strontium. We rely on shelving detection, where electrons are first excited to a metastable state by the spectroscopy laser before their state is probed using the broad transition at 461 nm. As in the similar setting of calcium beam clocks, this enhances dramatically the signal strength as compared to direct saturated fluorescence or absorption spectroscopy of the narrow line. We implement shelving spectroscopy both in directed atomic beams and hot vapor cells with isotropic atomic velocities. We measure a fractional frequency instability $sim 2 times 10^{-12}$ at 1 s limited by technical noise - about one order of magnitude above shot noise limitations for our experimental parameters. Our work illustrates the robustness and flexibility of a scheme that can be very easily implemented in the reference cells or ovens of most existing strontium experiments, and may find applications for low-complexity clocks.
We present the first characterization of the spectral properties of superradiant light emitted from the ultra-narrow, 1 mHz linewidth optical clock transition in an ensemble of cold $^{87}$Sr atoms. Such a light source has been proposed as a next-generation active atomic frequency reference, with the potential to enable high-precision optical frequency references to be used outside laboratory environments. By comparing the frequency of our superradiant source to that of a state-of-the-art cavity-stabilized laser and optical lattice clock, we observe a fractional Allan deviation of $6.7(1)times 10^{-16}$ at 1 second of averaging, establish absolute accuracy at the 2 Hz ($4times 10^{-15}$ fractional frequency) level, and demonstrate insensitivity to key environmental perturbations.
We present a measurement of the absolute frequency of the 5s$^2$ $^1$S$_0$ to 5s5p $^3$P$_0$ transition in $^{87}$Sr, which is a secondary representation of the SI second. We describe the optical lattice clock apparatus used for the measurement, and we focus in detail on how its systematic frequency shifts are evaluated with a total fractional uncertainty of $1 times 10^{-17}$. Traceability to the International System of Units is provided via comparison to International Atomic Time (TAI). Gathering data over 5- and 15-day periods, with the lattice clock operating on average 74$%$ of the time, we measure the frequency of the transition to be 429228004229873.1(5) Hz, which corresponds to a fractional uncertainty of $1 times 10^{-15}$. We describe in detail how this uncertainty arises from the intermediate steps linking the optical frequency standard, through our local time scale UTC(NPL), to an ensemble of primary and secondary frequency standards which steer TAI. The calculated absolute frequency of the transition is in good agreement with recent measurements carried out in other laboratories around the world.
We report a new measurement of the $n=2$ Lamb shift in Muonium using microwave spectroscopy. Our result of $1047.2(2.3)_textrm{stat}(1.1)_textrm{syst}$ MHz comprises an order of magnitude improvement upon the previous best measurement. This value matches the theoretical calculation within one standard deviation allowing us to set limits on CPT violation in the muonic sector, as well as on new physics coupled to muons and electrons which could provide an explanation of the muon $g-2$ anomaly.
High-power and narrow-linewidth laser light is a vital tool for atomic physics, being used for example in laser cooling and trapping and precision spectroscopy. Here we produce Watt-level laser radiation at 457.49 nm and 460.86 nm of respective relevance for the cooling transitions of cadmium and strontium atoms. This is achieved via the frequency doubling of a kHz-linewidth vertical-external-cavity surface-emitting laser (VECSEL), which is based on a novel gain chip design enabling lasing at > 2 W in the 915-928 nm region. Following an additional doubling stage, spectroscopy of the $^1S_0to{}^1P_1$ cadmium transition at 228.89 nm is performed on an atomic beam, with all the transitions from all eight natural isotopes observed in a single continuous sweep of more than 4 GHz in the deep ultraviolet. The absolute value of the transition frequency of Cd-114 and the isotope shifts relative to this transition are determined, with values for some of these shifts provided for the first time