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Register a new userManipulating ionization path in a Stark map: Stringent schemes for the selective field ionization in highly excited Rb Rydberg atoms
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We have developed a quite stringent method in selectivity to ionize the low angular- momentum ($ell$) states which lie below and above the adjacent manifold in highly excited Rb Rydberg atoms. The method fully exploits the pulsed field-ionization characteristics of the manifold states in high slew-rate regime: Specifically the low $ell$ state below (above) the adjacent manifold is firstly transferred to the lowest (highest) state in the manifold via the adiabatic transition at the first avoided crossing in low slew-rate regime, and then the atoms are driven to a high electric field for ionization in high slew-rate regime. These extreme states of the manifold are ionized at quite different fields due to the tunneling process, resulting in thus the stringent selectivity. Two manipulation schemes to realize this method actually are demonstrated here experimentally.
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Pulsed field ionization of high-$n$ (90 $leq n leq$ 150) manifold states in Rb Rydberg atoms has been investigated in high slew-rate regime. Two peaks in the field ionization spectra were systematically observed for the investigated $n$ region, where the field values at the lower peak do not almost depend on the excitation energy in the manifold, while those at the higher peak increase with increasing excitation energy. The fraction of the higher peak component to the total ionization signals increases with increasing $n$, exceeding 80% at $n$ = 147. Characteristic behavior of the peak component and the comparison with theoretical predictions indicate that the higher peak component is due to the tunneling process. The obtained results show for the first time that the tunneling process plays increasingly the dominant role at such highly excited nonhydrogenic Rydberg atoms.
We have studied an ionization of alkali-metal Rydberg atoms by blackbody radiation (BBR). The results of the theoretical calculations of ionization rates of Li, Na, K, Rb and Cs Rydberg atoms are presented. Calculations have been performed for nS, nP and nD states which are commonly used in a variety of experiments, at principal quantum numbers n=8-65 and at the three ambient temperatures of 77, 300 and 600 K. A peculiarity of our calculations is that we take into account the contributions of BBR-induced redistribution of population between Rydberg states prior to photoionization and field ionization by extraction electric field pulses. The obtained results show that these phenomena affect both the magnitude of measured ionization rates and shapes of their dependences on n. A Cooper minimum for BBR-induced transitions between bound Rydberg states of Li has been found. The calculated ionization rates are compared with our earlier measurements of BBR-induced ionization rates of Na nS and nD Rydberg states with n=8-20 at 300 K. A good agreement for all states except nS with n>15 is observed. Useful analytical formulas for quick estimation of BBR ionization rates of Rydberg atoms are presented. Application of BBR-induced ionization signal to measurements of collisional ionization rates is demonstrated.
We analyze how bound-state excitation, electron exchange and the residual binding potential influence above-threshold ionization (ATI) in Helium prepared in an excited $p$ state, oriented parallel and perpendicular to a linearly polarized mid-IR field. Using ab initio B-spline Algebraic Diagrammatic Construction (ADC), and several one-electron methods with effective potentials, including the Schrodinger solver Qprop, modifi
We report on experiments exploring Stark-tuned Forster resonances between Rydberg atoms with unprecedented resolution in the Forster defect. The individual resonances are expected to exhibit different angular dependencies, opening the possibility to tune not only the interaction strength but also the angular dependence of the pair state potentials by an external electric field. We achieve a high resolution by optical Ramsey interferometry for Rydberg atoms combined with electric field pulses. The resonances are detected by a loss of visibility in the Ramsey fringes due to resonances in the interaction. We present measurements of the density dependence as well as of the coherence time at and close to Forster resonances.
We report on the behaviour of the ionization avalanche in an ensemble of ultracold 87Rb atoms coupled to a high lying Rydberg state and investigate extensions to the current model by including the effects of three-body recombination and plasma expansion. To separate the two effects we study the time dependence of the plasma formation at various densities as well as for different nS and nD states. At medium densities and low n we observe the onset of the avalanche as has been reported in other experiments, as well as a subsequent turn-off of the avalanche for longer excitation times, which we associate with plasma expansion. At higher densities and for higher lying Rydberg states we observe a disappearance of the avalanche signature, which we attribute to three-body recombination.
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