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Register a new userFront propagation into unstable and metastable states in Smectic C* liquid crystals: linear and nonlinear marginal stability analysis
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We discuss the front propagation in ferroelectric chiral smectics (SmC*) subjected to electric and magnetic fields applied parallel to smectic layers. The reversal of the electric field induces the motion of domain walls or fronts that propagate into either an unstable or a metastable state. In both regimes, the front velocity is calculated exactly. Depending on the field, the speed of a front propagating into the unstable state is given either by the so-called linear marginal stability velocity or by the nonlinear marginal stability expression. The cross-over between these two regimes can be tuned by a magnetic field. The influence of initial conditions on the velocity selection problem can also be studied in such experiments. SmC$^*$ therefore offers a unique opportunity to study different aspects of front propagation in an experimental system.
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This paper is an introductory review of the problem of front propagation into unstable states. Our presentation is centered around the concept of the asymptotic linear spreading velocity v*, the asymptotic rate with which initially localized perturbations spread into an unstable state according to the linear dynamical equations obtained by linearizing the fully nonlinear equations about the unstable state. This allows us to give a precise definition of pulled fronts, nonlinear fronts whose asymptotic propagation speed equals v*, and pushed fronts, nonlinear fronts whose asymptotic speed v^dagger is larger than v*. In addition, this approach allows us to clarify many aspects of the front selection problem, the question whether for a given dynamical equation the front is pulled or pushed. It also is the basis for the universal expressions for the power law rate of approach of the transient velocity v(t) of a pulled front as it converges toward its asymptotic value v*. Almost half of the paper is devoted to reviewing many experimental and theoretical examples of front propagation into unstable states from this unified perspective. The paper also includes short sections on the derivation of the universal power law relaxation behavior of v(t), on the absence of a moving boundary approximation for pulled fronts, on the relation between so-called global modes and front propagation, and on stochastic fronts.
Non-equilibrium dissipative systems usually exhibit multistability, leading to the presence of propagative domain between steady states. We investigate the front propagation into an unstable state in discrete media. Based on a paradigmatic model of coupled chain of oscillators and populations dynamics, we calculate analytically the average speed of these fronts and characterize numerically the oscillatory front propagation. We reveal that different parts of the front oscillate with the same frequency but with different amplitude. To describe this latter phenomenon we generalize the notion of the Peierls-Nabarro potential, achieving an effective continuous description of the discreteness effect.
Propagating fronts arising from bistable reaction-diffusion equations are a purely deterministic effect. Stochastic reaction-diffusion processes also show front propagation which coincides with the deterministic effect in the limit of small fluctuations (usually, large populations). However, for larger fluctuations propagation can be affected. We give an example, based on the classic spruce-budworm model, where the direction of wave propagation, i.e., the relative stability of two phases, can be reversed by fluctuations.
We develop a theory of Smectic A - Smectic C phase transition with anomalously weak smectic layer contraction. We construct a phenomenological description of this transition by generalizing the Chen-Lubensky model. Using a mean-field molecular model, we demonstrate that a relatively simple interaction potential suffices to describe the transition. The theoretical results are in excellent agreement with experimental data.
General microscopic mechanism of ferroelectric ordering in chiral smectic C* liquid crystals is considered. It is shown that if the mesogenic molecules have a sufficiently low symmetry, the spontaneous polarization is proportional to one of the biaxial vector order parameters of the smectic C phase. This order parameter may be determined by intermolecular interactions which are not sensitive to molecular chirality. At the same time, the polarization is also proportional to a pseudoscalar parameter which vanishes if the molecules are nonchiral. The general statistical theory of ferroelectric ordering is illustrated by two particular models. The first model is based on electrostatic quadrupole-quadrupole interactions, and it enables one to obtain explicit analytical expressions for the spontaneous polarization. In the second model, the molecular chirality and polarity are determined by a pair of off-center nonparallel dipoles. For this case, the spontaneous polarization is calculated numerically as a function of temperature. The theory provides a more general interpretation of the previous approaches including the classical Boulder model.
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