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Measurements of ultracold neutron lifetimes in solid deuterium

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 Publication date 2001
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and research's language is English




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We present the first measurements of the survival time of ultracold neutrons (UCNs) in solid deuterium SD2. This critical parameter provides a fundamental limitation to the effectiveness of superthermal UCN sources that utilize solid ortho-deuterium as the source material. Superthermal UCN sources offer orders of magnitude improvement in the available densities of UCNs, and are of great importance to fundamental particle-physics experiments such as searches for a static electric dipole moment and lifetime measurements of the free neutron. These measurements are performed utilizing a SD2 source coupled to a spallation source of neutrons, providing a demonstration of UCN production in this geometry and permitting systematic studies of the influence of thermal up-scatter and contamination with para-deuterium on the UCN survival time.



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85 - A.Anghel , T.L.Bailey , G.Bison 2018
Solid deuterium (sD_2) is used as an efficient converter to produce ultracold neutrons (UCN). It is known that the sD_2 must be sufficiently cold, of high purity and mostly in its ortho-state in order to guarantee long lifetimes of UCN in the solid from which they are extracted into vacuum. Also the UCN transparency of the bulk sD_2 material must be high because crystal inhomogeneities limit the mean free path for elastic scattering and reduce the extraction efficiency. Observations at the UCN sources at Paul Scherrer Institute and at Los Alamos National Laboratory consistently show a decrease of the UCN yield with time of operation after initial preparation or later treatment (`conditioning) of the sD_2. We show that, in addition to the quality of the bulk sD_2, the quality of its surface is essential. Our observations and simulations support the view that the surface is deteriorating due to a build-up of D_2 frost-layers under pulsed operation which leads to strong albedo reflections of UCN and subsequent loss. We report results of UCN yield measurements, temperature and pressure behavior of deuterium during source operation and conditioning, and UCN transport simulations. This, together with optical observations of sD_2 frost formation on initially transparent sD_2 in offline studies with pulsed heat input at the North Carolina State University UCN source results in a consistent description of the UCN yield decrease.
Our experiment using gravitationally trapped ultracold neutrons (UCN) to measure the neutron lifetime is reviewed. Ultracold neutrons were trapped in a material bottle covered with perfluoropolyether. The neutron lifetime was deduced from comparison of UCN losses in the traps with different surface-to-volume ratios. The precise value of the neutron lifetime is of fundamental importance to particle physics and cosmology. In this experiment, the UCN storage time is brought closer to the neutron lifetime than in any experiments before:the probability of UCN losses from the trap was only 1% of that for neutron beta decay. The neutron lifetime obtained,878.5+/-0.7stat+/-0.3sys s, is the most accurate experimental measurement to date.
Neutron lifetime is one of the most important physical constants which determines parameters of the weak interaction and predictions of primordial nucleosynthesis theory. There remains the unsolved problem of a 3.9{sigma} discrepancy between measurements of this lifetime using neutrons in beams and those with stored neutrons (UCN). In our experiment we measure the lifetime of neutrons trapped by Earths gravity in an open-topped vessel. Two configurations of the trap geometry are used to change the mean frequency of UCN collisions with the surfaces - this is achieved by plunging an additional surface into the trap without breaking the vacuum. The trap walls are coated with a hydrogen-less fluorine-containing polymer to reduce losses of UCN. The stability of this coating to multiple thermal cycles between 80 K and 300 K was tested. At 80 K, the probability of UCN loss due to collisions with the trap walls is just 1.5% of the probability of beta-decay. The free neutron lifetime is determined by extrapolation to an infinitely large trap with zero collision frequency. The result of these measurements is 881.5 +/- 0.7_stat +/- 0.6_syst s which is consistent with the conventional value of 880.2 +/- 1.0 s presented by the Particle Data Group. Future prospects for this experiment are in further cooling to 10 K which will lead to an improved accuracy of measurement. In conclusion we present an analysis of currently-available data on various measurements of the neutron lifetime.
Ultra-cold neutrons (UCN), neutrons with energies low enough to be confined by the Fermi potential in material bottles, are playing an increasing role in measurements of fundamental properties of the neutron. The ability to manipulate UCN with material guides and bottles, magnetic fields, and gravity can lead to experiments with lower systematic errors than have been obtained in experiments with cold neutron beams. The UCN densities provided by existing reactor sources limit these experiments. The promise of much higher densities from solid deuterium sources has led to proposed facilities coupled to both reactor and spallation neutron sources. In this paper we report on the performance of a prototype spallation neutron-driven solid deuterium source. This source produced bottled UCN densities of 145 +/-7 UCN/cm3, about three times greater than the largest bottled UCN densities previously reported. These results indicate that a production UCN source with substantially higher densities should be possible.
Ultracold neutron (UCN) storage measurements were made in a trap constructed from a 1.3 T Halbach Octupole PErmanent (HOPE) magnet array aligned vertically, using the TES-port of the PF2 source at the Institut Laue-Langevin. A mechanical UCN valve at the bottom of the trap was used for filling and emptying. This valve was covered with Fomblin grease to induce non-specular reflections and was used in combination with a movable polyethylene UCN remover inserted from the top for cleaning of above-threshold UCNs. Loss due to UCN depolarization was suppressed with a minimum 2 mT bias field. Without using the UCN remover, a total storage time constant of $(712 pm 19)$ s was observed; with the remover inserted for 80 s and used at either 80 cm or 65 cm from the bottom of the trap, time constants of $(824 pm 32)$ s and $(835 pm 36)$ s were observed. Combining the latter two values, a neutron lifetime of $tau_{rm n} = (887 pm 39)$ s is extracted after primarily correcting for losses at the UCN valve. The time constants of the UCN population during cleaning were observed and compared to calculations based on UCN kinetic theory as well as Monte-Carlo studies. These calculations are used to predict above-threshold populations of $sim 5%$, $sim 0.5%$ and $sim 10^{-12}%$ remaining after cleaning in the no remover, 80~cm remover and 65~cm remover measurements. Thus, by using a non-specular reflector covering the entire bottom of the trap and a remover at the top of the trap, we have established an effective cleaning procedure for removing a major systematic effect in high-precision $tau_{rm n}$ experiments with magnetically stored UCNs.
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