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Two-Impurity Kondo Effect in Double-Quantum-Dot Systems - Effect of Interdot Kinetic Exchange Coupling

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 Added by Wataru Izumida
 Publication date 1999
  fields Physics
and research's language is English




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Tunneling conductance through two quantum dots, which are connected in series to left and right leads, is calculated by using the numerical renormalization group method. As the hopping between the dots increases from very small value, the following states continuously appear; (i) Kondo singlet state of each dot with its adjacent-site lead, (ii) singlet state between the local spins on the dots, and (iii) double occupancy in the bonding orbital of the two dots. The conductance shows peaks at the transition regions between these states. Especially, the peak at the boundary between (i) and (ii) has the unitarity limit value of $2e^{2}/h$ because of coherent connection through the lead-dot-dot-lead. For the strongly correlated cases, the characteristic energy scale of the coherent peak shows anomalous decrease relating to the quantum critical transition known for the two-impurity Kondo effect. The two dots systems give the new realization of the two-impurity Kondo problem.

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The Kondo effect is a key many-body phenomenon in condensed matter physics. It concerns the interaction between a localised spin and free electrons. Discovered in metals containing small amounts of magnetic impurities, it is now a fundamental mechanism in a wide class of correlated electron systems. Control over single, localised spins has become relevant also in fabricated structures due to the rapid developments in nano-electronics. Experiments have already demonstrated artificial realisations of isolated magnetic impurities at metallic surfaces, nanometer-scale magnets, controlled transitions between two-electron singlet and triplet states, and a tunable Kondo effect in semiconductor quantum dots. Here, we report an unexpected Kondo effect realised in a few-electron quantum dot containing singlet and triplet spin states whose energy difference can be tuned with a magnetic field. This effect occurs for an even number of electrons at the degeneracy between singlet and triplet states. The characteristic energy scale is found to be much larger than for the ordinary spin-1/2 case.
We report the observation of Kondo physics in a spin- 3/2 hole quantum dot. The dot is formed close to pinch-off in a hole quantum wire defined in an undoped AlGaAs/GaAs heterostructure. We clearly observe two distinctive hallmarks of quantum dot Kondo physics. First, the Zeeman spin-splitting of the zero-bias peak in the differential conductance is independent of gate voltage. Second, this splitting is twice as large as the splitting for the lowest one-dimensional subband. We show that the Zeeman splitting of the zero-bias peak is highly-anisotropic, and attribute this to the strong spin-orbit interaction for holes in GaAs.
We theoretically investigate the Kondo effect of a T-shaped triple-quantum-dot structure, by means of the numerical renormalization group method. It is found that at the point of electron-hole symmetry, the systems entropy has opportunities to exhibit three kinds of transition processes for different interdot couplings, with the decrease of temperature. This leads to the different pictures of the Kondo physics, including the three-stage Kondo effect. Next when the electron-hole symmetry is broken or the structural parameters are changed, the Kondo resonance can also be observed in the conductance spectrum. However, it shows alternative dependence on the relevant quantities, i.e., the Coulomb interaction and interdot couplings. All these phenomena exhibit the abundant and interesting Kondo physics in this system. We believe that this work can be helpful for further understanding the Kondo effect in the triple-quantum-dot structures.
We calculate the nonequilibrium conductance of a system of two capacitively coupled quantum dots, each one connected to its own pair of conducting leads. The system has been used recently to perform pseudospin spectroscopy by controlling independently the voltages of the four leads. The pseudospin is defined by the orbital occupation of one or the other dot. Starting from the SU(4) symmetric point of spin and pseudospin degeneracy in the Kondo regime, for an odd number of electrons in the system, we show how the conductance through each dot varies as the symmetry is reduced to SU(2) by a pseudo-Zeeman splitting, and as bias voltages are applied to any of the dots. We analize the expected behavior of the system in general, and predict characteristic fingerprint features of the SU(4) to SU(2) crossover that have not been observed so far.
We review our recent studies on the Kondo effect in the tunneling phenomena through quantum dot systems. Numerical methods to calculate reliable tunneling conductance are developed. In the first place, a case in which electrons of odd number occupy the dot is studied, and experimental results are analyzed based on the calculated result. Tunneling anomaly in the even-number-electron occupation case, which is recently observed in experiment and is ascribed to the Kondo effect in the spin singlet-triplet cross over transition region, is also examined theoretically.
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