Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userComment on Quantum Scattering of Heavy Particles from a 10 K Cu(111) Surface
96
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
In the original paper Althoff et al. (see ibid., vol.79, p.4429 (1997)) reported a study of scattering of thermal Ne, Ar, and Kr atoms from a Cu(111) surface in which they assessed the corresponding Debye-Waller factor (DWF) as a function of the particle mass m in a wide range of substrate temperature T. The experiments were interpreted by the semiclassical DWF theory in which the projectile moves on the classical recoilless trajectory and the surface vibrations are quantized. Siber and Gumhalter claim that the experiments described by Althoff et al. were carried out in the quantum scattering regime in which the semiclassical scalings of Althoff et al. do not hold and the semiclassical DWE significantly deviates from the exact quantum one both in the low and high T limits. Hence, it is claimed, the quantum scattering data of Althoff et al. cannot be reliably interpreted by the semiclassical theory.
rate research
Read More
We study the early time and coarsening dynamics in the Light-Heavy model, a system consisting of two species of particles ($light$ and $heavy$) coupled to a fluctuating surface (described by tilt fields). The dynamics of particles and tilts are coupled through local update rules, and are known to lead to different ordered and disordered steady state phases depending on the microscopic rates. We introduce a generalized balance mechanism in non-equilibrium systems, namely $bunchwise~balance$, in which incoming and outgoing transition currents are balanced between groups of configurations. This allows us to exactly determine the steady state in a subspace of the phase diagram of this model. We introduce the concept of $irreducible~sequences$ of interfaces and bends in this model. These sequences are non-local, and we show that they provide a coarsening length scale in the ordered phases at late times. Finally, we propose a $local$ correlation function ($mathcal{S}$) that has a direct relation to the number of irreducible sequences, and is able to distinguish between several phases of this system through its coarsening properties. Starting from a totally disordered initial configuration, $mathcal{S}$ displays an initial linear rise and a broad maximum. As the system evolves towards the ordered steady states, $mathcal{S}$ further exhibits power law decays at late times that encode coarsening properties of the approach to the ordered phases. Focusing on early time dynamics, we posit coupled mean-field evolution equations governing the particles and tilts, which at short times are well approximated by a set of linearized equations, which we solve analytically. Beyond a timescale set by a lattice cutoff and preceding the onset of coarsening, our linearized theory predicts the existence of an intermediate power-law stretch, which we also find in simulations of the ordered regime of the system.
We present angle-resolved photoemission data from Cu(111). Using a focused 6 eV continuous wave laser for photo-excitation, we achieve a high effective momentum resolution enabling the first detection of the Rashba spin splitting in the Shockley surface state on Cu(111). The magnitude of the spin-splitting of Delta k ~ 0.006 A^-1 is surprisingly large and exceeds values predicted for the analogous surface state on Ag(111) but is reproduced by first principles calculations. We further resolve a kink in the dispersion which we attribute to electron-phonon coupling.
We present a study of graphene/substrate interactions on UHV-grown graphene islands with minimal surface contamination using emph{in situ} low-temperature scanning tunneling microscopy (STM). We compare the physical and electronic structure of the sample surface with atomic spatial resolution on graphene islands versus regions of bare Cu(111) substrate. We find that the Rydberg-like series of image potential states is shifted toward lower energy over the graphene islands relative to Cu(111), indicating a decrease in the local work function, and the resonances have a much smaller linewidth, indicating reduced coupling to the bulk. In addition, we show the dispersion of the occupied Cu(111) Shockley surface state is influenced by the graphene layer, and both the band edge and effective mass are shifted relative to bare Cu(111).
We present a theoretical study of surface states close to 3d transition metal adatoms (Cr, Mn, Fe, Co, Ni and Cu) on a Cu(111) surface in terms of an embedding technique using the fully relativistic Korringa-Kohn-Rostoker method. For each of the adatoms we found resonances in the s-like states to be attributed to a localization of the surface states in the presence of an impurity. We studied the change of the s-like densities of states in the vicinity of the surface state band-edge due to scattering effects mediated via the adatoms d-orbitals. The obtained results show that a magnetic impurity causes spin-polarization of the surface states. In particular, the long-range oscillations of the spin-polarized s-like density of states around an Fe adatom are demonstrated.
We present density-functional results on the lifetime of the (111) surface state of the noble metals. We consider scattering on the Fermi surface caused by impurity atoms belonging to the 3d and 4sp series. The results are analyzed with respect to film thickness and with respect to separation of scattering into bulk or into surface states. While for impurities in the surface layer the overall trends are similar to the long-known bulk-state scattering, for adatom-induced scattering we find a surprising behavior with respect to the adatom atomic number. A plateau emerges in the scattering rate of the 3d adatoms, instead of a peak characteristic of the d resonance. Additionally, the scattering rate of 4sp adatoms changes in a zig-zag pattern, contrary to a smooth parabolic increase following Lindes rule that is observed in bulk. We interpret these results in terms of the weaker charge-screening and of interference effects induced by the lowering of symmetry at the surface.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
