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Charge Segregation and Antiferromagnetism in High-Tc Superconductors

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 Added by John M. Tranquada
 Publication date 1999
  fields Physics
and research's language is English




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Local antiferromagnetism coexists with superconductivity in the cuprates. Charge segregation provides a way to reconcile these properties. Direct evidence for modulated spin and charge densities has been found in neutron and X-ray scattering studies of Nd-doped La(2-x)Sr(x)CuO(4). Here we discuss the nature of the modulation, and present some new results for a Zn-doped sample. Some of the open questions concerning the connections between segregation and superconductivity are described.



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157 - Louis Taillefer 2009
The recent observation of quantum oscillations in underdoped high-Tc superconductors, combined with their negative Hall coefficient at low temperature, reveals that the Fermi surface of hole-doped cuprates includes a small electron pocket. This strongly suggests that the large hole Fermi surface characteristic of the overdoped regime undergoes a reconstruction caused by the onset of some order which breaks translational symmetry. Here we consider the possibility that this order is stripe order, a form of charge / spin modulation observed most clearly in materials like Eu-doped and Nd-doped LSCO. In these materials, the onset of stripe order is indeed the cause of Fermi-surface reconstruction. We identify the critical doping where this reconstruction occurs and show that the temperature dependence of transport coefficients at that doping is typical of metals at a quantum critical point. We discuss how the pseudogap phase may be a fluctuating precursor of the stripe-ordered phase.
106 - S.M. Hayden , G. Aeppli , P. Dai 1997
We review recent measurements of the high-frequency dynamic magnetic susceptibility in the high-$T_c$ superconducting systems La$_{2-x}$Sr$_{x}$CuO$_4$ and YBa$_2$Cu$_3$O$_{6+x}$. Experiments were performed using the chopper spectrometers HET and MARI at the ISIS spallation source. We have placed our measurements on an absolute intensity scale, this allows systematic trends to be seen and comparisons with theory to be made. We find that the insulating S=1/2 antiferromagnetic parent compounds show a dramatic renormalization of the spin wave intensity. The effect of doping on the response is to cause broadenings in wave vector and large redistributions of spectral weight in the frequency spectrum.
We survey recent experimental results including quantum oscillations and complementary measurements probing the electronic structure of underdoped cuprates, and theoretical proposals to explain them. We discuss quantum oscillations measured at high magnetic fields in the underdoped cuprates that reveal a small Fermi surface section comprising quasiparticles that obey Fermi-Dirac statistics, unaccompanied by other states of comparable thermodynamic mass at the Fermi level. The location of the observed Fermi surface section at the nodes is indicated by a body of evidence including the collapse in Fermi velocity measured by quantum oscillations, which is found to be associated with the nodal density of states observed in angular resolved photoemission, the persistence of quantum oscillations down to low fields in the vortex state, the small value of density of states from heat capacity and the multiple frequency quantum oscillation pattern consistent with nodal magnetic breakdown of bilayer-split pockets. A nodal Fermi surface pocket is further consistent with the observation of a density of states at the Fermi level concentrated at the nodes in photoemission experiments, and the antinodal pseudogap observed by photoemission, optical conductivity, nuclear magnetic resonance Knight shift, as well as other complementary diffraction, transport and thermodynamic measurements. One of the possibilities considered is that the small Fermi surface pockets observed at high magnetic fields can be understood in terms of Fermi surface reconstruction by a form of small wavevector charge order, observed over long lengthscales in experiments such as nuclear magnetic resonance and x-ray scattering, potentially accompanied by an additional mechanism to gap the antinodal density of states.
In this review article, we show our recent results relating to the undoped (Ce-free) superconductivity in the electron-doped high-Tc cuprates with the so-called T structure. For an introduction, we briefly mention the characteristics of the electron-doped T-cuprates, including the reduction annealing, conventional phase diagram and undoped superconductivity. Then, our transport and magnetic results and results relating to the superconducting pairing symmetry of the undoped and underdoped T-cuprates are shown. Collaborating spectroscopic and nuclear magnetic resonance results are also shown briefly. It has been found that, through the reduction annealing, a strongly localized state of carriers accompanied by an antiferromagnetic pseudogap in the as-grown samples changes to a metallic and superconducting state with a short-range magnetic order in the reduced superconducting samples. The formation of the short-range magnetic order due to a very small amount of excess oxygen in the reduced superconducting samples suggests that the T-cuprates exhibiting the undoped superconductivity in the parent compounds are regarded as strongly correlated electron systems, as well as the hole-doped high-Tc cuprates. We show our proposed electronic structure model to understand the undoped superconductivity. Finally, unsolved future issues of the T-cuprates are discussed.
Electron irradiation has been used to introduce point defects in a controlled way in the CuO2 planes of underdoped and optimally doped YBCO. This technique allows us to perform very accurate measurements of Tc and of the residual resistivity in a wide range of defect contents xd down to Tc=0. The Tc decrease does not follow the variation expected from pair breaking theories. The evolutions of Tc and of the transition width with xd emphasize the importance of phase fluctuations, at least for the highly damaged regime. These results open new questions about the evolution of the defect induced Tc depression over the phase diagram of the cuprates
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