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Register a new userPhotoinduced superconducting nanowires in Gd-Ba-Cu-O films
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We report the fabrication of high Tc superconducting wires by photodoping a GdBa2Cu3O{6.5} thin film. An optical near-field probe was used to locally excite carriers in the system at room temperature. Trapping of the photogenerated electrons define a confining potential for the conducting holes in the CuO planes. Spatially resolved reflectance measurements show the photogenerated nanowires to be ~ 250 nm wide. Electron diffusion, before electron capture, is believed to be responsible for the observed width of the wires.
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It is known that solid-state reaction in high-pressure oxygen can stabilize high-oxidation phases of Y-Ba-Cu-O superconductors in powder form. We extend this superoxygenation concept of synthesis to thin films which, due to their large surface-to-volume ratio, are more reactive thermodynamically. Epitaxial thin films of $rm{YBa_2Cu_3O_{7-delta}}$ grown by pulsed laser deposition are annealed at up to 700 atm O$_2$ and 900$^circ$C, in conjunction with Cu enrichment by solid-state diffusion. The films show clear formation of $rm{Y_2Ba_4Cu_7O_{15-delta}}$ and $rm{Y_2Ba_4Cu_8O_{16}}$ as well as regions of $rm{YBa_2Cu_5O_{9-delta}}$ and YBa$_2$Cu$_6$O$_{10-delta}$ phases, according to scanning transmission electron microscopy, x-ray diffraction and x-ray absorption spectroscopy. Similarly annealed $rm{YBa_2Cu_3O_{7-delta}}$ powders show no phase conversion. Our results demonstrate a novel route of synthesis towards discovering more complex phases of cuprates and other superconducting oxides.
We have measured the resistance vs. temperature of more than 20 superconducting nanowires with nominal widths ranging from 10 to 22 nm and lengths from 100 nm to 1050 nm. With decreasing cross-sectional areas, the wires display increasingly broad resistive transitions. The data are in very good agreement with a model that includes both thermally activated phase slips close to Tc and quantum phase slips (QPS) at low temperatures, but disagree with an earlier model based on a critical value of R_n/Rq. Our measurements provide strong evidence for QPS in thin superconducting wires.
The structure and physical properties of superconducting compounds Y(La)-Ba(Sr)-Cu-O are studied, the compounds being prepared by the method of cryogenic dispersion of a charge consisting of premix oxides and carbonates. Electrical conductivity and critical current density of the superconductors are measured over a wide temperature range of 10~$mK$ to 300~$K$. Degradation of the superconductor critical parameters in time and structural characteristics, magnetic susceptibility, heat capacity and acoustic properties are studied, and current-voltage characteristics are determined.
Superconductivity is observed in a new nontoxic cuprate system Ga-Ba-Ca-Cu-O, with Tc = 82K for GaBa2Ca5Cu6O14+{delta} (Ga-1256) and Tc = 116K probably for GaBa2Ca3Cu4O10+{delta} (Ga-1234) or GaBa2Ca2Cu3O8+{delta} (Ga-1223), respectively. All compounds are fabricated by solid state reaction method under high pressure and high temperature. Samples are characterized by resistivity, magnetization and X-ray diffraction (XRD) measurements. The temperature dependence of magnetization measured in both zero-field-cooled and field-cooled processes on one sample (S1) shows two superconducting transitions at about 82K and 113K. The estimated shielding fraction for the phase with Tc of 82K is about 67%, while the fraction for another phase with Tc of 113K is quite small. The XRD Rietveld refinement for S1 indicates two main phases existing in the sample, Ga-1256 with fraction of about 58% and non-superconducting Ca0.85CuO2 with fraction of about 42%, respectively. Thus, we can conclude the superconducting phase with transition temperature of 82K is due to Ga-1256. The resistivity measurement also confirms the superconductivity for S1, and the resistivity reaches zero at about 82K. The temperature dependence of magnetization for another sample (S2) shows much higher superconducting shielding fraction for the phase with Tc of 116K, which may be a promising prospective for the synthesis of Ga-1234 or Ga-1223 phase.
We present the fabrication and electrical transport characterization of underdoped YBa$_2$Cu$_3$O$_{7-{delta}}$ nanowires. The nanowires have been realized without any protective capping layer and they show transport properties similar to those of the parent thin film, demonstrating that they have not been damaged by the nanopatterning. The current-voltage characteristics of the underdoped nanowires show large hysteretic voltage switching at the critical current, in contrast to the flux-flow like characteristics of optimally doped nanostructures, indicating the formation of a self-stabilizing hot spot. These results open up new possibilities of using the underdoped nanowires for single photon detection and for exploring the underdoped side of the YBa$_2$Cu$_3$O$_{7-{delta}}$ phase diagram at the nanoscale.
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