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Register a new userDouble metal-insulator transitions and magnetoresistance:An intrinsic feature of Ru substituted La(0.67)Ca(0.33)MnO(3)
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In this paper, we examine the possible influence of extrinsic factors on the electrical and magnetotransport of La(0.67)Ca(0.33)Mn(1-x)Ru(x)O(3) (x < 0.10). These results not only exclude the extrinsic factors, but establishes the fact that the metal transitions both exhibiting MR is intrinsic to Ru substituted La(0.67)Ca(0.33)MnO(3) and the system. These results substantiate our hypothesis that Ru substituted system undergoes a magnetic phase separation involving the co-existence of two ferromagnetic-metallic phases in its ground state.
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This paper is in continuation of our previous work on the structural, electrical and magnetic properties of Ru doped La(0.67)Ca(0.33)MnO(3) compounds (Ref.: L.Seetha Lakshmi et.al, J. Magn. Magn. Mater. 257, 195 (2003)). Here we report the results of magnetotransport measurements on La(0.67)Ca(0.33)Mn(1-x)Ru(x)O(3) (0<x< 0.1) compounds in the light of proposed magnetic phase separation.
We discuss the effects of local structure on the electrical transport and magnetic properties of La(0.67)Ca(0.33)Mn(1-x)Ti(x)O(3) system.Based on the intercomparison of the structure, transport and magnetic properties of the Mn site substituted La(0.67)Ca(0.33)MnO(3) with isovalent diamagnetic and paramagnetic ions, we argue that local structural effects have a decisive role to play, compared to the local spin coupling effects, in the ferromagnetic-metallic ground state of the CMR manganites
We report magnetization experiments in two magnetically isolated ferromagnetic nanotubes of perovskite La$_{0.67}$Ca$_{0.33}$MnO$_3$. The results show that the magnetic anisotropy is determined by the sample shape although the coercive field is reduced by incoherent magnetization reversal modes. The temperature dependence of the magnetization reveals that the magnetic behavior is dominated by grain surface properties. These measurements were acquired using a Silicon micro-mechanical oscillator working in its resonant mode. The sensitivity was enough to measure the magnetic properties of these two samples with a mass lower than 14 picograms and to obtain for the first time the magnetization loop for one isolated nanotube.
Manganites have shown potential in spintronics because they exhibit high spin polarization. Here, by ferromagnetic resonance we have studied the damping properties of La$_{0.67}$Sr$_{0.33}$MnO$_{3}$/Pt bilayers which are prepared by oxide molecular beam epitaxy. The damping coefficient ($alpha$) of La$_{0.67}$Sr$_{0.33}$MnO$_{3}$ (LSMO) single layer is found to be 0.0104. However the LSMO/Pt bilayers exhibit decrease in $alpha$ with increase in Pt thickness. This decrease in the value of $alpha$ is probably due to high anti-damping like torque. Further, we have investigated the angle dependent inverse spin Hall effect (ISHE) to quantify the spin pumping voltage from other spin rectification effects such as anomalous Hall effect and anisotropic magnetoresistance. We have observed high spin pumping voltage ($sim$~20 $ mu V$). The results indicate that both anti-damping and spin pumping phenomena are occuring simultaneously.
Reflectivity as a function of temperature for the La$_{0.67}$Ca$_{0.33}$MnO$_{3}$ (LCMO) film has been measured across the metal-insulator phase transition. The optical properties and their temperature dependence were determined in the infrared and visible range by fits to a Drude-Lorentz model, using exact formula for the thin film optics and the measured properties of the substrate. The phonon modes were identified and verified with lattice dynamical calculations for the ideal and distorted perovskite structure of the material. The optical conductivity shows agreement with the double exchange mechanism in conjunction with the Jahn-Teller distortion term in the Hamiltonian. Low temperature metallic phase is dominated by large polaron dynamics, a key component of electron-orbital coupling in a strongly corrrelated system. Free carrier dynamics in the metallic phase is described in terms of coherent heavy polaronic motion in the DC limit with incoherent and asymmetric polaronic background in the mid-IR range. The strength and line width of Jahn-Teller modes has been discussed across the phase transition and their temperature evolution is qualitatively discussed on account of existing electron-phonon coupling. The localized Holstein polaron formation in the high temperature insulative phase is identified as optical conductivity peaks in the visible range above the critical temperature.
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