We demonstrate a novel kind of polariton four wave mixing oscillation. Two pump polaritons scatter towards final states that emit two beams of equal intensity, separated both spatially and in polarization with respect to the pumps. The measurement of the intensity fluctuations of the emitted light demonstrates that the final states are strongly correlated.
Microcavity polaritons are composite half-light half-matter quasi-particles, which have recently been demonstrated to exhibit rich physical properties, such as non-equilibrium Bose-Einstein condensation, parametric scattering and superfluidity. At the same time, polaritons have some important advantages over photons for information processing applications, since their excitonic component leads to weaker diffraction and stronger inter-particle interactions, implying, respectively, tighter localization and lower powers for nonlinear functionality. Here we present the first experimental observations of bright polariton solitons in a strongly coupled semiconductor microcavity. The polariton solitons are shown to be non-diffracting high density wavepackets, that are strongly localised in real space with a corresponding broad spectrum in momentum space. Unlike solitons known in other matter-wave systems such as Bose condensed ultracold atomic gases, they are non-equilibrium and rely on a balance between losses and external pumping. Microcavity polariton solitons are excited on picosecond timescales, and thus have significant benefits for ultrafast switching and transfer of information over their light only counterparts, semiconductor cavity lasers (VCSELs), which have only nanosecond response time.
Based on a microscopic many-particle theory, we predict large optical gain in the probe and background-free four-wave mixing directions caused by excitonic instabilities in semiconductor quantum wells. For a single quantum well with radiative-decay limited dephasing in a typical pump-probe setup we discuss the microscopic driving mechanisms and polarization and frequency dependence of these instabilities.
We demonstrate experimentally an unusual behavior of the parametric polariton scattering in semiconductor microcavity under a strong cw resonant excitation. The maximum of the scattered signal above the threshold of stimulated parametric scattering does not shift along the microcavity lower polariton branch with the change of pump detuning or angle of incidence but is stuck around the normal direction. We show theoretically that such a behavior can be modelled numerically by a system of Maxwell and nonlinear Schroedinger equations for cavity polaritons and explained via the competition between the bistability of a driven nonlinear MC polariton and the instabilities of parametric polariton-polariton scattering.
Entanglement generation in microcavity exciton-polaritons is an interesting application of the peculiar properties of these half-light/half-matter quasiparticles. In this paper we theoretically investigate their luminescence dynamics and entanglement formation in single, double, and triple cavities. We derive general expressions and selection rules for polariton-polariton scattering. We evaluate a number of possible parametric scattering schemes in terms of entanglement, and identify the ones that are experimentally most promising.
Non-perturbative phenomena in four-wave mixing spectra of semiconductors are studied using the exact solution of a widely used phenomenological non-linear equation of motion of the exciton polarization. It is shown that Coulomb interaction, included in the nonlinearity, leads to two characteristic effects, which are essentially of dynamical origin, -- a split of the exciton peak and a non-monotonous dependence of the response at the exciton frequency on the magnitude of the external field. Relations between the spectral features and the parameters of the system is obtained. It is found that the transition from perturbative to non-perturbative regimes is controlled by parameters inversely proportional to the decay rate. It implies that the condition of low excitation density does not necessarily warrant applicability of the perturbational approach.
Marco Romanelli
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(2005)
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"Four wave mixing oscillation in a semiconductor microcavity: Generation of two correlated polariton populations"
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Marco Romanelli
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