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Delocalized fermions in underdoped cuprates

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 Added by Michael Sutherland
 Publication date 2005
  fields Physics
and research's language is English




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Low temperature heat transport was used to investigate the ground state of high-purity single crystals of the lightly-doped cuprate YBa$_{2}$Cu$_{3}$O$_{6.33}$. Samples were measured on either side of the superconducting phase boundary, in both zero and applied magnetic field. We report the observation of delocalized fermionic excitations at zero energy in the non-superconducting state, which shows that the ground state of underdoped cuprates is metallic. Its low-energy spectrum appears to be similar to that of the d-wave superconductor, i.e. nodal. The insulating ground state observed in underdoped La$_{2-x}$Sr$_{x}$CuO$_4$ is attributed to the competing spin-density-wave order present in that system.

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We study the static charge correlation function in an one-band model on a square lattice. The Hamiltonian consist of effective hoppings of the electrons between the lattice sites and the Heisenberg Hamiltonian. Approximating the irreducible charge correlation function by a single bubble yields the ladder approximation for the charge correlation function. In this approximation one finds in general three charge instabilities, two of them are due to nesting, the third one is the flux phase instability. Since these instabilities cannot explain the experiments in hole-doped cuprates we have included in the irreducible charge correlation function also Aslamasov-Larkin (AL) diagrams where charge fluctuations interact with products of spin fluctuations. We then find at high temperatures a nematic or $d$-wave Pomeranchuk instability with a very small momentum. Its transition temperature decreases roughly linearly with doping in the underdoped region and vanishes near optimal doping. Decreasing the temperature further a secondary axial charge-density wave (CDW) instability appears with mainly $d$-wave symmetry and a wave vector somewhat larger than the distance between nearest neighbor hot spots. At still lower temperatures the diagonal flux phase instability emerges. A closer look shows that the AL diagrams enhance mainly axial and not diagonal charge fluctuations in our one-band model. This is the main reason why axial and not diagonal instabilities are the leading ones in agreement with experiment. The two instabilities due to nesting vanish already at very low temperatures and do not play any major role in the phase diagram. Remarkable is that the nematic and the axial CDW instabilities show a large reentrant behavior.
Pair density waves, identified by Cooper pairs with finite center-of-mass momentum, have recently been observed in copper oxide based high T$_textrm{c}$ superconductors (cuprates). A charge density modulation or wave is also ubiquitously found in underdoped cuprates. Within a general mean-field one-band model we show that the coexistence of charge density waves and uniform superconductivity in $d$-wave superconductors like cuprates, generates an odd-frequency spin-singlet pair density wave, in addition to the even-frequency counterparts. The strength of the induced odd-frequency pair density wave depends on the modulation wave vector of the charge density wave, with the odd-frequency pair density waves even becoming comparable to the even-frequency ones in parts of the Brillouin zone. We show that a change in the modulation wave vector of the charge density wave from bi-axial to uni-axial, can enhance the odd-frequency component of the pair density waves. Such a coexistence of superconductivity and uni-axial charge density wave has already been experimentally verified at high magnetic fields in underdoped cuprates. We further discuss the possibility of an odd-frequency spin-triplet pair density wave generated in the coexistence regime of superconductivity and spin density waves, applicable to the iron-based superconductors. Our work thus presents a route to bulk odd-frequency superconductivity in high T$_c$ superconductors.
275 - Yucel Yildirim , Wei Ku 2010
Despite more than two decades of intensive investigations, the true nature of high temperature (high-$T_c$) superconductivity observed in the cuprates remains elusive to the researchers. In particular, in the so-called `underdoped region, the overall behavior of superconductivity deviates $qualitatively$ from the standard theoretical description pioneered by Bardeen, Cooper and Schrieffer (BCS). Recently, the importance of phase fluctuation of the superconducting order parameter has gained significant support from various experiments. However, the microscopic mechanism responsible for the surprisingly soft phase remains one of the most important unsolved puzzles. Here, opposite to the standard BCS starting point, we propose a simple, solvable low-energy model in the strong coupling limit, which maps the superconductivity literally into a well-understood physics of superfluid in a special dilute bosonic system of local pairs of doped holes. In the prototypical material (La$_{1-delta}$Sr$_delta$)$_2$CuO$_4$, without use of any free parameter, a $d$-wave superconductivity is obtained for doping above $sim 5.2%$, below which unexpected incoherent $p$-wave pairs dominate. Throughout the whole underdoped region, very soft phases are found to originate from enormous mass enhancement of the pairs. Furthermore, a striking mass divergence is predicted that dictates the occurrence of the observed quantum critical point. Our model produces properties of the superfluid in good agreement with the experiments, and provides new insights into several current puzzles. Owing to its simplicity, this model offers a paradigm of great value in answering the long-standing challenges in underdoped cuprates.
In underdoped cuprates, only a portion of the Fermi surface survives as Fermi arcs due to pseudogap opening. In hole-doped La$_{2}$CuO$_4$, we have deduced the coherence temperature $T_{coh}$ of quasi-particles on the Fermi arc above which the broadened leading edge position in angle-integrated photoemission spectra is shifted away from the Fermi level and the quasi-particle concept starts to lose its meaning. $T_{coh}$ is found to rapidly increase with hole doping, an opposite behavior to the pseudogap temperature $T^*$. The superconducting dome is thus located below both $T^*$ and $T_{coh}$, indicating that the superconductivity emerges out of the coherent Fermionic quasi-particles on the Fermi arc. $T_{coh}$ remains small in the underdoped region, indicating that incoherent charge carriers originating from the Fermi arc are responsible for the apparently metallic transport at high temperatures.
The resonating valence bond spin liquid model for the underdoped cuprates has as an essential element, the emergence of a pseudogap. This new energy scale introduces asymmetry in the quasiparticle density of states because it is associated with the antiferromagnetic Brillouin zone. By contrast, superconductivity develops on the Fermi surface and this largely restores the particle-hole symmetry for energies below the superconducting energy gap scale. In the highly underdoped regime, these two scales can be separately identified in the density of states and also partial density of states for each fixed angle in the Brillouin zone. From the total density of states, we find that the pseudogap energy scale manifests itself differently as a function of doping for positive and negative bias. Furthermore, we find evidence from recent scanning tunneling spectroscopy data for asymmetry in the positive and negative bias of the extracted $Delta(theta)$ which is in qualitative agreement with this model. Likewise, the slope of the linear low energy density of states is nearly constant in the underdoped regime while it increases significantly with overdoping in agreement with the data.
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