Scaling Behavior of the Longitudinal and Transverse Transport in Quasi One-Dimensional Organic Conductors


Abstract in English

We report on dc and microwave experiments of the low-dimensional organic conductors (TMTSF)$_2$PF$_6$ and (TMTSF)$_2$ClO$_4$ along the $a$, $b^{prime}$, and $c^*$ directions. In the normal state of (TMTSF)$_2$PF$_6$ below T=70 K, the dc resistivity follows a power-law with $rho_a$ and $rho_{b^{prime}}$ proportional to $T^2$ while $rho_{c^*}propto T$. Above $T = 100$ K the exponents extracted from the data for the $a$ and $c^*$ axes are consiste1nt with what is to be expected for a system of coupled one-dimensional chains (Luttinger liquid) and a dimensional crossover at a temperature of about 100 K. The $b^prime$ axis shows anomalous exponents that could be attributed to a large crossover between these two regimes. The contactless microwave measurements of single crystals along the $b^{prime}$-axis reveal an anomaly between 25 and 55 K which is not understood yet. The organic superconductor (TMTSF)$_2$ClO$_4$ is more a two-dimensional metal with an anisotropy $rho_a/rho_{b^{prime}}$ of approximately 2 at all temperatures. Such a low anisotropy is unexpected in view of the transfer integrals. Slight indications to one-dimensionality are found in the temperature dependent transport only above 200 K. Even along the least conducting $c^*$ direction no region with semiconducting behavior is revealed up to room temperature.

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