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Correlation length in cuprates deduced from the impurity-induced magnetization

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 Added by Bobroff
 Publication date 2003
  fields Physics
and research's language is English




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We report a new multi-nuclei based NMR method which allows us to image the staggered polarization induced by nonmagnetic Li impurities in underdoped O6.6 and slightly overdoped O7 YBa2Cu3O6+y above T_C. The spatial extension of the polarization xi_imp approximately follows a Curie law, increasing up to six lattice constants at T=80K at O6.6 in the pseudogap regime. Near optimal doping, the staggered magnetization has the same shape, with xi_imp reduced by a factor 2. xi_imp is argued to reveal the intrinsic magnetic correlation length of the pure system. It is found to display a smooth evolution through the pseudogap regime.



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The large ($10^2 - 10^5$) and strongly temperature dependent resistive anisotropy $eta = (sigma_{ab}/sigma_c)^{1/2}$ of cuprates perhaps holds the key to understanding their normal state in-plane $sigma_{ab}$ and out-of-plane $sigma_{c}$ conductivities. It can be shown that $eta$ is determined by the ratio of the phase coherence lengths $ell_i$ in the respective directions: $sigma_{ab}/sigma_c = ell_{ab}^2/ell_{c}^2$. In layered crystals in which the out-of-plane transport is incoherent, $ell_{c}$ is fixed, equal to the interlayer spacing. As a result, the T-dependence of $eta$ is determined by that of $ell_{ab}$, and vice versa, the in-plane phase coherence length can be obtained directly by measuring the resistive anisotropy. We present data for hole-doped $YBa_2Cu_3O_y$ ($6.3 < y < 6.9$) and $Y_{1-x}Pr_xBa_2Cu_3O_{7-delta }$ ($0 < x leq 0.55$) and show that $sigma_{ab}$ of crystals with different doping levels can be well described by a two parameter universal function of the in-plane phase coherence length. In the electron-doped $Nd_{2-x}Ce_{x}CuO_{4-y}$, the dependence $sigma_{ab}(eta)$ indicates a crossover from incoherent to coherent transport in the c-direction.
We demonstrate that most features ascribed to strong correlation effects in various spectroscopies of the cuprates are captured by a calculation of the self-energy incorporating effects of spin and charge fluctuations. The self energy is calculated over the full doping range of electron-doped cuprates from half filling to the overdoped system. The spectral function reveals four subbands, two widely split incoherent bands representing the remnant of the split Hubbard bands, and two additional coherent, spin- and charge-dressed in-gap bands split by a spin-density wave, which collapses in the overdoped regime. The incoherent features persist to high doping, producing a remnant Mott gap in the optical spectra, while transitions between the in-gap states lead to pseudogap features in the mid-infrared.
In order to investigate the electronic state of Ce-free and Ce-underdoped high-Tc cuprates with the so-called T structure, we have performed muon-spin-relaxation (muSR) and specific-heat measurements of Ce-free T-La_1.8_Eu_0.2_CuO_4+d_ (T-LECO) polycrystals and Ce-underdoped T-Pr_1.3-x_La_0.7_Ce_x_CuO_4+d_ (T-PLCCO) single crystals with x=0.10. The muSR spectra of the reduced superconducting samples of both T-LECO with Tc=15K and T-PLCCO with x=0.10 and Tc=27K have revealed that a short-range magnetic order coexists with the superconductivity in the ground state. The formation of a short-range magnetic order due to a tiny amount of excess oxygen in the reduced superconducting samples strongly suggest that the Ce-free and Ce-underdoped T-cuprates are regarded as strongly correlated electron systems.
Nematicity is ubiquitous in electronic phases of high-$T_c$ superconductors, particularly in the Fe-based systems. We used inelastic x-ray scattering to extract the temperature-dependent nematic correlation length $xi$ from the anomalous softening of acoustic phonon modes in FeSe, underdoped Ba(Fe$_{0.97}$Co$_{0.03}$)$_2$As$_2$ and optimally doped Ba(Fe$_{0.94}$Co$_{0.06}$)$_2$As$_2$. In all cases, we find that $xi$ is well described by a power law $(T-T_0)^{-1/2}$ extending over a wide temperature range. We attributed this mean-field behavior and the extended fluctuation regime to a sizable nemato-elastic coupling, which may be detrimental to superconductivity.
100 - S. Ouazi , J. Bobroff , H. Alloul 2005
Oxygen NMR is used to probe the local influence of nonmagnetic Zn and magnetic Ni impurities in the superconducting state of optimally doped high Tc YBa2Cu3O7. Zn and Ni induce a staggered paramagnetic polarization, similar to that evidenced above Tc, with a typical extension xi=3 cell units for Zn and xi>=3 for Ni. In addition, Zn is observed to induce a local density of states near the Fermi Energy in its neighbourhood, which also decays over about 3 cell units. Its magnitude decreases sharply with increasing temperature. This allows direct comparison with the STM observations done in BiSCO.
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