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Register a new userSuperconducting phase diagram of Li Metal in nearly hydrostatic pressures up to 67 GPa
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The dependence of the superconducting transition temperature T_{c} on nearly hydrostatic pressure has been determined to 67 GPa in an ac susceptibility measurement for a Li sample embedded in helium pressure medium. With increasing pressure, superconductivity appears at 5.47 K for 20.3 GPa, T_{c} rising rapidly to ~ 14 K at 30 GPa. The T_{c}(P)-dependence to 67 GPa differs significantly from that observed in previous studies where no pressure medium was used. Evidence is given that superconductivity in Li competes with symmetry breaking structural phase transitions which occur near 20, 30, and 62 GPa. In the pressure range 20-30 GPa, T_{c} is found to decrease rapidly in a dc magnetic field, the first evidence that Li is a type I superconductor.
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We have constructed a pressure$-$temperature ($P-T$) phase diagram of $P$-induced superconductivity in EuFe$_2$As$_2$ single crystals, via resistivity ($rho$) measurements up to 3.2 GPa. As hydrostatic pressure is applied, an antiferromagnetic (AF) transition attributed to the FeAs layers at $T_mathrm{0}$ shifts to lower temperatures, and the corresponding resistive anomaly becomes undetectable for $P$ $ge$ 2.5 GPa. This suggests that the critical pressure $P_mathrm{c}$ where $T_mathrm{0}$ becomes zero is about 2.5 GPa. We have found that the AF order of the Eu$^{2+}$ moments survives up to 3.2 GPa without significant changes in the AF ordering temperature $T_mathrm{N}$. The superconducting (SC) ground state with a sharp transition to zero resistivity at $T_mathrm{c}$ $sim$ 30 K, indicative of bulk superconductivity, emerges in a pressure range from $P_mathrm{c}$ $sim$ 2.5 GPa to $sim$ 3.0 GPa. At pressures close to but outside the SC phase, the $rho(T)$ curve shows a partial SC transition (i.e., zero resistivity is not attained) followed by a reentrant-like hump at approximately $T_mathrm{N}$ with decreasing temperature. When nonhydrostatic pressure with a uniaxial-like strain component is applied using a solid pressure medium, the partial superconductivity is continuously observed in a wide pressure range from 1.1 GPa to 3.2 GPa.
In this communication, we report the temperature dependence (3 to 300K) of the electrical resistivity of BiS2 based layered PrO0.5F0.5BiS2 superconductor at ambient and hydrostatic pressure of up to 3GPa. It is observed that Tc increases with pressure at the rate of dTc/dP=0.45/GPa for PrO0.5F0.5BiS2 compound. It is envisaged that one may increase the Superconducting transition temperature (Tc) of recently discovered PrO0.5F0.5BiS2 superconductor by applying hydrostatic external or internal chemical pressure via suitable on site substitutions.
Motivated by the recent discovery of near-room temperature superconductivity in high-pressure superhydrides, we investigate from first-principles the high-pressure superconducting phase diagram of the ternary Ca-B-H system, using ab-initio evolutionary crystal structure prediction, and Density Functional Perturbation Theory. We find that below 100 GPa all stable and weakly metastable phases are insulating. This pressure marks the appearance of several new chemically-forbidden phases on the hull of stability, and the first onset of metalization in CaBH$_5$. Metallization is then gradually achieved at higher pressure at different compositions. Among the metallic phases stable in the Megabar regime, we predict two high-$T_c$ superconducting phases with CaBH$_6$ and Ca$_2$B$_2$H$_{13}$ compositions, with critical temperatures of 119 and 89 K at 300 GPa, respectively, surviving to lower pressures. Ternary hydrides will most likely play a major role in superconductivity research in the coming years; our study suggests that, in order to reduce the pressure for the onset of metallicity and superconductivity, further explorations of ternary hydrides should focus on elements less electronegative than boron.
Basal plane resistivity of expanded graphite was studied under simultaneous influence of hydrostatic pressure up to 1.8 GPa and magnetic field 0.8 T in the 77-300 K temperature region. Magnetic field induces negative magnetoresistance in the sample within all temperature and pressure range studied. A change in resistivity of the sample under maximum pressure reaches 80%. Significant change in resistivity dependence on temperature under the pressure of 0.6 GPa suggests for ordering transition in the sample studied. Negative magnetoresistance in the graphite reaches about 15% at 0.6 GPa. Magnetic field acts in the same way as pressure and potentiates the transition formation and further magnetoresistance dynamics. The effects observed are mostly of elastic character according to resistivity of the unloaded sample.
We study the phase diagram of the Hubbard model in the weak-coupling limit for coexisting spin-density-wave order and spin-fluctuation-mediated superconductivity. Both longitudinal and transverse spin fluctuations contribute significantly to the effective interaction potential, which creates Cooper pairs of the quasi-particles of the antiferromagnetic metallic state. We find a dominant $d_{x^2-y^2}$-wave solution in both electron- and hole-doped cases. In the quasi-spin triplet channel, the longitudinal fluctuations give rise to an effective attraction supporting a $p$-wave gap, but are overcome by repulsive contributions from the transverse fluctuations which disfavor $p$-wave pairing compared to $d_{x^2-y^2}$. The sub-leading pair instability is found to be in the $g$-wave channel, but complex admixtures of $d$ and $g$ are not energetically favored since their nodal structures coincide. Inclusion of interband pairing, in which each fermion in the Cooper pair belongs to a different spin-density-wave band, is considered for a range of electron dopings in the regime of well-developed magnetic order. We demonstrate that these interband pairing gaps, which are non-zero in the magnetic state, must have the same parity under inversion as the normal intraband gaps. The self-consistent solution to the full system of five coupled gap equations give intraband and interband pairing gaps of $d_{x^2-y^2}$ structure and similar gap magnitude. In conclusion, the $d_{x^2-y^2}$ gap dominates for both hole and electron doping inside the spin-density-wave phase.
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