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Register a new userAnomalous Electronic Susceptibility in Bi2sr2cuo6+d
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Added by
Zorica Konstantinovic
Publication date
2002
fields
Physics
and research's language is
English
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We report magnetic susceptibility performed on overdoped Bi2Sr2CuO6+d powders as a function of oxygen doping d and temperature T. The decrease of the spin susceptibility chis with increasing T is confirmed. At sufficient high temperature, chis presents an unusual linear temperature dependence chis=chis0 -chi1T . Moreover, a linear correlation between chi1 and chis0 for increasing hole concentration has been displayed. These non conventional metal features will be discussed in terms of a singular narrow-band structures.
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We report magnetic susceptibility performed on overdoped Bi2Sr2CuO6+d powders as a function of oxygen doping d and temperature T. The decrease of the spin susceptibility with increasing T is confirmed. At sufficient high temperature, the spin susceptibility Chi_s presents an unusual linear temperature dependence Chi_s ~ Chi_s0 -Chi_1 T. Moreover, a linear correlation between Chi_1 and Chi_s0 for increasing hole concentration is displayed. A temperature Tchi, independent of hole doping characterizes this scaling. Comparison with other cuprates of the literature(LSCO, Tl-2201 and Bi-2212), over the same overdoped range, shows similarities with above results. These non conventional metal features will be discussed in terms of a singular narrow-band structure.
We have studied the evolution of the thermoelectric power S(T) with oxygen doping of single-layered Bi2Sr2CuO6+d thin films and ceramics in the overall superconducting (Tc, S290K) phase diagram. While the universal relation between the room-temperature thermopower S290K and the critical temperature is found to hold in the strongly overdoped region (d>0.14), a strong violation is observed in the underdoped part of the phase diagram. The observed behaviour is compared with other cuprates and the different scenarios are discussed.
The evolution of the thermoelectric power S(T) with doping, p, of single-layer Bi2Sr2CuO6+d ceramics in the strongly overdoped region is studied in detail. Analysis in term of drag and diffusion contributions indicates a departure of the diffusion from the T-linear metallic behavior. This effect is increased in the strongly overdoped range (p~0.2-0.28) and should reflect the proximity of some topological change.
Unveiling the driving force for a phase transition is normally difficult when multiple degrees of freedom are strongly coupled. One example is the nematic phase transition in iron-based superconductors. Its mechanism remains controversial due to a complex intertwining among different degrees of freedom. In this paper, we report a method for measuring the nematic susceptibly of FeSe$_{0.9}$S$_{0.1}$ using angle-resolved photoemission spectroscopy (ARPES) and an $in$-$situ$ strain-tuning device. The nematic susceptibility is characterized as an energy shift of band induced by a tunable uniaxial strain. We found that the temperature-dependence of the nematic susceptibility is strongly momentum dependent. As the temperature approaches the nematic transition temperature from the high temperature side, the nematic susceptibility remains weak at the Brillouin zone center while showing divergent behavior at the Brillouin zone corner. Our results highlight the complexity of the nematic order parameter in the momentum space, which provides crucial clues to the driving mechanism of the nematic phase transition. Our experimental method which can directly probe the electronic susceptibly in the momentum space provides a new way to study the complex phase transitions in various materials.
One of the central issues concerning the mechanism of high temperature superconductivity in cuprates is the nature of the ubiquitous charge order and its implications to superconductivity. Here we use scanning tunneling microscopy to investigate the evolution of charge order from the optimally doped to strongly overdoped Bi2Sr2CuO6+{delta} cuprates. We find that with increasing hole concentration, the long-range checkerboard order gradually evolves into short-range glassy patterns consisting of diluted charge puddles. Each charge puddle has a unidirectional nematic internal structure, and exhibits clear pair density modulations as revealed by the spatial variations of superconducting coherence peak and gap depth. Both the charge puddles and the nematicity vanish completely in the strongly overdoped non-superconducting regime, when another type of short-range order with root2 * root2 periodicity emerges. These results shed important new lights on the intricate interplay between the intertwined orders and the superconducting phase of cuprates.
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